English

Disorder-mediated linear and nonlinear magnetotransport in the charge-density-wave material ${\rm Ta_2NiSe_7 }$

Materials Science 2025-12-10 v1 Mesoscale and Nanoscale Physics

Abstract

We report disorder-mediated first-order linear and higher-order nonlinear (magneto-)transport of Ta2_2NiSe7_7 (TNS) in the charge-density-wave (CDW) regime. CDW transition temperature (TCDWT_{CDW}) and carrier density are proportional and inversely proportional to residual resistance ratio of samples, respectively. Such relation helps to understand the unique CDW order therein. High-TCDWT_{CDW} TNS exhibits negative first-harmonic magnetoresistance (MR1ω^{1\omega}) under a magnetic field (BB) parallel to the direction of alternating current (IωI^{\omega}), which may arise from the anomalous velocity induced by the Berry curvature of three-dimensional topological bands near the Fermi level. As TCDWT_{CDW} drops, a positive-to-negative MR1ω^{1\omega} transition is observed with decreasing perpendicular BB, which is likely due to the contribution of Zeeman effect on current pathways in the disordered system. Moreover, interestingly, the second-harmonic nonlinear signals are suppressed, while the third-harmonic signals are significant and sensitive to both BB and TCDWT_{CDW}. Such observations, together with scaling analysis, suggest the quantum geometry quadrupole at play and the modulation of disorder on third-order nonlinearity. Our results pave an avenue for tailoring distinct-order magnetoresistive phases in disordered topological materials.

Keywords

Cite

@article{arxiv.2512.08373,
  title  = {Disorder-mediated linear and nonlinear magnetotransport in the charge-density-wave material ${\rm Ta_2NiSe_7 }$},
  author = {Xiaodong Sun and Jiabin Qiao and Yuanzhe Li and Wanli He and Jiali Chen and Jinjin Liu and Yuxiang Chen and Yuchen Ma and Meiling Jin and Jianlin Luo and Jie Chen and Wei Wu and Zhiwei Wang and Wei Jiang and Xiang Li and Yugui Yao},
  journal= {arXiv preprint arXiv:2512.08373},
  year   = {2025}
}