English

Critical fluctuations in the spin-orbit Mott insulator Sr$_3$Ir$_2$O$_7$

Strongly Correlated Electrons 2019-03-27 v2

Abstract

X-ray magnetic critical scattering measurements and specific heat measurements were performed on the perovskite iridate Sr3_3Ir2_2O7_7. We find that the magnetic interactions close to the N\'{e}el temperature TNT_N = 283.4(2) K are three-dimensional. This contrasts with previous studies which suggest two-dimensional behaviour like Sr2_2IrO4_4. Violation of the Harris criterion (dν>2d\nu>2) means that weak disorder becomes relevant. This leads a rounding of the antiferromagnetic phase transition at TNT_N, and modifies the critical exponents relative to the clean system. Specifically, we determine that the critical behaviour of Sr3_3Ir2_2O7_7 is representative of the diluted 3D Ising universality class.

Keywords

Cite

@article{arxiv.1812.08682,
  title  = {Critical fluctuations in the spin-orbit Mott insulator Sr$_3$Ir$_2$O$_7$},
  author = {J. G. Vale and S. Boseggia and H. C. Walker and R. S. Springell and E. C. Hunter and R. S. Perry and S. P. Collins and D. F. McMorrow},
  journal= {arXiv preprint arXiv:1812.08682},
  year   = {2019}
}

Comments

Accepted in Journal of Physics: Condensed Matter