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Critical behavior in itinerant ferromagnet SrRu$_{1-x}$Ti$_x$O$_3$

Strongly Correlated Electrons 2018-08-01 v1

Abstract

SrRuO3_3 presents a rare example of ferromagnetism among the 4dd based oxides. While the nature of magnetic state in SrRuO3_3 is mostly believed to be of itinerant type, recent studies suggest a coexistence of both itinerant and localized model of magnetism in this material. Here, we have investigated the evolution of magnetic state in doped SrRu1x_{1-x}Tix_xO3_3 through studying the critical behavior using standard techniques such as, modified Arrott plot, Kouvel-Fisher plot and critical isotherm analysis across the magnetic transition temperature TcT_c. The substitution of nonmagnetic Ti4+^{4+} (3d0d^{0}) for Ru4+^{4+} (4d4d^4) would simply dilute the magnetic system apart from modifying the electron correlation effect and the density of states at Fermi level. Surprisingly, TcT_c does not change with xx. Moreover, our analysis show the exponent β\beta related to spontaneous magnetization increases while the exponents γ\gamma and δ\delta related to initial inverse susceptibility and critical magnetization, respectively decrease with Ti substitution. The estimated exponents do not match with any established theoretical models for universality classes, however, the exponent obey the Widom relation and the scaling behavior. Interestingly, this particular evolution of exponents in present series has similarity with that in isoelectronic doped Sr1x_{1-x}Cax_xRuO3_3. We believe that site dilution by Ti leads to formation magnetic clusters which causes this specific changes in critical exponents.

Keywords

Cite

@article{arxiv.1807.01445,
  title  = {Critical behavior in itinerant ferromagnet SrRu$_{1-x}$Ti$_x$O$_3$},
  author = {Renu Gupta and Imtiaz Noor Bhatti and A. K. Pramanik},
  journal= {arXiv preprint arXiv:1807.01445},
  year   = {2018}
}

Comments

10 pages, 9 figures