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Electronic properties in itinerant ferromagnet SrRu$_{1-x}$Ti$_x$O$_3$

Strongly Correlated Electrons 2020-09-02 v1

Abstract

Here, we study the electrical transport and specific heat in 4dd based ferromagnetic material SrRuO3_3 and its Ti substituted SrRu1x_{1-x}Tix_xO3_3 series (xx \le 0.7). The SrRuO3_3 is a metal and shows itinerant ferromagnetism with transition temperature TcT_c \sim 160 K. The nonmagnetic Ti4+^{4+} (3d0d^0) substitution would not only weaken the active Ru-O-Ru channel but is also expected to tune the electronic density and electron correlation effect. A metal to insulator transition has been observed around xx \sim 0.4. The nature of charge transport in paramagnetic-metallic state (xx \leq 0.4) and in insulating state (xx >> 0.4) follows modified Mott's variable range hopping model. In ferromagnetic-metallic state, resistivity shows a T2T^2 dependence below TcT_c which though modifies to T3/2T^{3/2} dependence at low temperature. In Ti substituted samples, temperature range for T3/2T^{3/2} dependence extends to higher temperature. Interestingly, this T3/2T^{3/2} dependence dominates in whole ferromagnetic regime in presence of magnetic field. This evolution of electronic transport behavior can be explained within the framework of Fermi liquid theory and electron-magnon scattering mechanism. The negative magnetoresistance exhibits a hysteresis and a crossover between negative and positive value with magnetic field which is connected with magnetic behavior in series. The decreasing electronic coefficient of specific heat with xx supports the increasing insulating behavior in present series. We calculate a high Kadowaki-Woods ratio (xx \leq 0.3) for SrRuO3_3 which increases with substitution concentration. This signifies an increasing electronic correlation effect with substitution concentration.

Keywords

Cite

@article{arxiv.2009.00076,
  title  = {Electronic properties in itinerant ferromagnet SrRu$_{1-x}$Ti$_x$O$_3$},
  author = {Renu Gupta and R. Rawat and A. K. Pramanik},
  journal= {arXiv preprint arXiv:2009.00076},
  year   = {2020}
}

Comments

21 pages, 10 figures