English

Anomalous electric conductions in KSbO3-type metallic rhenium oxides

Materials Science 2009-11-13 v1

Abstract

Single crystals of KSbO3-type rhenium oxides, La4Re6O19,Pb6Re6O19,Sr2Re3O9andBi3Re3O11,weresynthesizedbyahydrothermalmethod.TheircrystalstructurescanberegardedasanetworkofthreedimensionalorthogonaldimerlatticeofedgesharedReO6octahedra.AllofthemexhibitsmallmagnitudeofPauliparamagnetism,indicatingmetallicelectronicstateswithoutstrongelectroncorrelations.Theresistivityoftheserhenates,exceptBi3Re3O11,haveatemperaturedependenceof19, Pb6Re6O19, Sr2Re3O9 and Bi3Re3O11, were synthesized by a hydrothermal method. Their crystal structures can be regarded as a network of three-dimensional orthogonal-dimer lattice of edge-shared ReO6 octahedra. All of them exhibit small magnitude of Pauli paramagnetism, indicating metallic electronic states without strong electron correlations. The resistivity of these rhenates, except Bi3Re3O11, have a temperature dependence of rho(T)=\rho_{0}+AT^{n} (n \approx 1.6)$ in a wide temperature range between 5 K and 300 K, which is extraordinary for three-dimensional metals without strong electron correlations. The resistivity of Bi3Re3O11 shows an anomaly around at 50 K, where the magnetic susceptibility also detects a deviation from ordinary Pauli paramagnetism.

Keywords

Cite

@article{arxiv.cond-mat/0702451,
  title  = {Anomalous electric conductions in KSbO3-type metallic rhenium oxides},
  author = {Hirotake Suzuki and Hiromi Ozawa and Hirohiko Sato},
  journal= {arXiv preprint arXiv:cond-mat/0702451},
  year   = {2009}
}

Comments

13 pages, 7 figures. J. Phys. Soc. Japan, in press