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Understanding ultrafast x-ray 'echoes' diffracted from single crystals

Materials Science 2026-04-03 v1 Optics

Abstract

Multiple x-ray beams generated by interference processes in perfect crystals were imaged with a resolution of about 100nm using tele-ptychography in the diffraction direction. These multiple wave-fields, also known as x-ray diffraction echoes, are related to the process known as the Pendelloesung effect and are described by dynamical diffraction theory. The echoes are produced by the constructive interference of diffracted x-rays at the exit surface of the crystal sample. In the imaged diffraction peak, we observed 10 echoes maxima with a total signal length of 78 um. Which translates into a total temporal delay in the signal of less than 108 fs.This makes the echoes of high importance for x-ray optics at x-ray Free Electron Laser sources, as the effect could be used for future ultrafast x-ray beam splitters. In addition to this application, echoes can be exploited to follow ultrafast processes in single crystal micro-structures such as melting or strain propagation.

Keywords

Cite

@article{arxiv.2604.01784,
  title  = {Understanding ultrafast x-ray 'echoes' diffracted from single crystals},
  author = {Angel Rodriguez-Fernandez and Dmitry Karpov and Steven Leake and Dina Carbone and Ana Diaz},
  journal= {arXiv preprint arXiv:2604.01784},
  year   = {2026}
}
R2 v1 2026-07-01T11:50:36.067Z