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Room-temperature multistage metastability in a moir\'e superstructure

Strongly Correlated Electrons 2026-04-22 v1 Materials Science

Abstract

Metastability is fundamental not only to phase ordering and transitions, but also to a broad range of modern technologies, from memory devices to metallic glasses. In condensed-matter physics, charge density waves (CDWs) offer versatile platforms for accessing metastable states due to their sensitivity to external stimuli. However, most metastable CDW states are stabilized only at low temperatures, limiting their practical utility. In this study, we report the observation of electrically driven, room-temperature, nonvolatile metastable states in the bulk form of EuTe4_4, a recently discovered compound that hosts an innate moir\'e superlattice characterized by the stacking of incommensurate monolayer and bilayer CDWs. Systematic transport measurements reveal discrete resistivity plateaus and strong electric-field sensitivity, with a large number of metastable states readily induced across a wide temperature window within a giant hysteresis loop, making them well-suited for high-temperature, multi-bit memory applications. By integrating photoemission spectroscopy, diffraction, and in-situ transport measurements, we uncover that these metastable states do not stem from conventional mechanisms such as the emergence of new ordered phases or changes in incommensurate periodicity. Instead, they are characterized by a suppression of the original CDW amplitude and a reduction in correlation length, pointing to a unique electric-field-induced switching of out-of-plane CDW phases in the moir\'e superstructure. Our findings not only provide critical insights into metastable phenomena in moir\'e systems with stacked electronic orders but also establish EuTe4_4 as a promising platform for developing room-temperature, multi-bit memory devices.

Keywords

Cite

@article{arxiv.2604.18998,
  title  = {Room-temperature multistage metastability in a moir\'e superstructure},
  author = {B. Q. Lv and Yifan Su and Alfred Zong and Karna Morey and Bryan T. Fichera and Qiaomei Liu and Dong Wu and Yongchang Ma and Dupeng Zhang and Faran Zhou and Makoto Hashimoto and Dong-Hui Lu and Donald A. Walko and Haidan Wen and Jiarui Li and Suchismita Sarker and Jacob P. C. Ruff and N. L. Wang and Nuh Gedik},
  journal= {arXiv preprint arXiv:2604.18998},
  year   = {2026}
}

Comments

11 pages, 4 figures

R2 v1 2026-07-01T12:27:35.836Z