English

Quantum dynamics of incoherently driven V-type system: Analytic solutions beyond the secular approximation

Chemical Physics 2016-07-27 v2 Atomic Physics Quantum Physics

Abstract

We present closed-form analytic solutions to non-secular Bloch-Redfield master equations for quantum dynamics of a V-type system driven by weak coupling to a thermal bath. We focus on noise-induced Fano coherences among the excited states induced by incoherent driving of the V-system initially in the ground state. For suddenly turned-on incoherent driving, the time evolution of the coherences is determined by the damping parameter ζ=12(γ1+γ2)/Δp\zeta=\frac{1}{2}(\gamma_1+\gamma_2)/\Delta_p, where γi\gamma_i are the radiative decay rates of the excited levels i=1,2i=1,2, and Δp=Δ2+(1p2)γ1γ2\Delta_p=\sqrt{\Delta^2 + (1-p^2)\gamma_1\gamma_2} depends on the excited-state level splitting Δ>0\Delta>0 and the angle between the transition dipole moments in the energy basis. The coherences oscillate as a function of time in the underdamped limit (ζ1\zeta\gg1), approach a long-lived quasi-steady state in the overdamped limit (ζ1\zeta\ll 1), and display an intermediate behavior at critical damping (ζ=1\zeta= 1). The sudden incoherent turn-on generates a mixture of excited eigenstates e1|e_1\rangle and e2|e_2\rangle and their in-phase coherent superposition ϕ+=12rˉ(r1e1+r2e2)|\phi_+\rangle = \frac{1}{\sqrt{2\bar{r}}}(\sqrt{r_1} |e_1\rangle + \sqrt{r_2}|e_2\rangle), which is remarkably long-lived in the overdamped limit (where r1r_1 and r2r_2 are the incoherent pumping rates). Formation of this coherent superposition {\it enhances} the decay rate from the excited states to the ground state. In the strongly asymmetric V-system where the coupling strengths between the ground state and the excited states differ significantly, we identify additional asymptotic quasistationary coherences, which arise due to slow equilibration of one of the excited states. Finally, we demonstrate that noise-induced Fano coherences are maximized with respect to populations when r1=r2r_1=r_2 and the transition dipole moments are fully aligned.

Keywords

Cite

@article{arxiv.1509.03399,
  title  = {Quantum dynamics of incoherently driven V-type system: Analytic solutions beyond the secular approximation},
  author = {Amro Dodin and Timur V. Tscherbul and Paul Brumer},
  journal= {arXiv preprint arXiv:1509.03399},
  year   = {2016}
}

Comments

revised version

R2 v1 2026-06-22T10:54:19.752Z