Long-lived quantum coherent dynamics of a $\Lambda$-system driven by a thermal environment
Abstract
We present a theoretical study of quantum coherent dynamics of a three-level system driven by a thermal environment (such as blackbody radiation), which serves as an essential building block of photosynthetic light-harvesting models and quantum heat engines. By solving the nonsecular Bloch-Redfield master equations, we obtain analytical results for the ground-state population and coherence dynamics and classify the dynamical regimes of the incoherently driven -system as underdamped and overdamped depending on whether the ratio is greater or less than one, where is the ground-state energy splitting, is the incoherent pumping rate, and is a function of the transition dipole alignment parameter . In the underdamped regime, we observe long-lived coherent dynamics that lasts for , even though the initial state of the -system contains no coherences in the energy basis. In the overdamped regime for , we observe the emergence of coherent quasi-steady states with the lifetime , which have low von Neumann entropy compared to the conventional thermal states. We propose an experimental scenario for observing noise-induced coherent dynamics in metastable He atoms driven by x-polarized incoherent light. Our results suggest that thermal excitations can generate experimentally observable long-lived quantum coherent dynamics in the ground-state subspace of atomic and molecular systems in the absence of coherent driving.
Cite
@article{arxiv.2108.07457,
title = {Long-lived quantum coherent dynamics of a $\Lambda$-system driven by a thermal environment},
author = {Suyesh Koyu and Timur V. Tscherbul},
journal= {arXiv preprint arXiv:2108.07457},
year = {2022}
}