English

Electronic correlation determining correlated plasmons in Sb-doped Bi$_2$Se$_3$

Materials Science 2019-09-09 v1

Abstract

Electronic correlation is believed to play an important role in exotic phenomena such as insulator-metal transition, colossal magneto resistance and high temperature superconductivity in correlated electron systems. Recently, it has been shown that electronic correlation may also be responsible for the formation of unconventional plasmons. Herewith, using a combination of angle-dependent spectroscopic ellipsometry, angle resolved photoemission spectroscopy and Hall measurements all as a function of temperature supported by first-principles calculations, the existence of low-loss high-energy correlated plasmons accompanied by spectral weight transfer, a fingerprint of electronic correlation, in topological insulator (Bi0.8_{0.8}Sb0.2_{0.2})2_2Se3_3 is revealed. Upon cooling, the density of free charge carriers in the surface states decreases whereas those in the bulk states increase, and that the newly-discovered correlated plasmons are key to explaining this phenomenon. Our result shows the importance of electronic correlation in determining new correlated plasmons and opens a new path in engineering plasmonic-based topologically-insulating devices.

Keywords

Cite

@article{arxiv.1909.02703,
  title  = {Electronic correlation determining correlated plasmons in Sb-doped Bi$_2$Se$_3$},
  author = {P. K. Das and T. J. Whitcher and M. Yang and X. Chi and Y. P. Feng and W. Lin and J. S. Chen and I. Vobornik and J. Fujii and K. A. Kokh and O. E. Tereshchenko and C. Z. Diao and Jisoo Moon and Seongshik Oh and A. H. Castro-Neto and M. B. H Breese and A. T. S. Wee and A. Rusydi},
  journal= {arXiv preprint arXiv:1909.02703},
  year   = {2019}
}
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