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Related papers: Nonlinear optical response in doped conjugated pol…

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Exciton effects on conjugated polymers are investigated in soliton lattice states. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration-…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice states. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions for electrons. The third-harmonic…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

Exciton effects on conjugated polymers are investigated in the soliton lattice system. We use the Su-Schrieffer-Heeger model with long-range Coulomb interactions treated by the single-excitation configuration-interaction method. The soliton…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya , Yukihiro Shimoi , Shuji Abe

Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice systems. The magnitude of the THG at the 10 percent doping increases by the factor about 10^2 from that of the neutral…

Condensed Matter · Physics 2016-08-31 Kikuo Harigaya

Exciton effects on soliton and bipolaron lattice states are investigated using an electron-lattice Peierls model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration- interaction…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya , Yukihiro Shimoi , Shuji Abe

Exciton effects on soliton and bipolaron lattice states are investigated using an electron-lattice Peierls model with long-range Coulomb interactions. The Hartree-Fock (HF) approximation and the single-excitation configuration-interaction…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya , Yukihiro Shimoi , Shuji Abe

We examine the third-order non-linear optical response of a one-dimensional Mott insulator coupled with phonons. The Mott insulator is described by an extended Hubbard-Holstein model. The third harmonic generation (THG) of the model is…

Strongly Correlated Electrons · Physics 2015-04-17 Shigetoshi Sota , Seiji Yunoki , Takami Tohyama

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron

Using the one-dimensional Hubbard model, which is commonly used for describing, e.g., high-$T_c$ superconducting cuprates, we study high-harmonic generation (HHG) from doped, correlated materials. Doping is modeled by changing the number of…

Strongly Correlated Electrons · Physics 2023-01-04 Thomas Hansen , Lars Bojer Madsen

We compute and analyze the dependence of excitonic second- and third-harmonic generation (SHG/THG) as a function of the optical excitation intensity in the presence of static electric fields by solving the semiconductor Bloch equations. Our…

Mesoscale and Nanoscale Physics · Physics 2025-11-10 Ruixin Zuo , Matthias Reichelt , Cong Ngo , Xiaohong Song , Weifeng Yang , Torsten Meier

Electronic structures and optical excitations in Moebius conjugated polymers are studied theoretically. Periodic and Moebius boundary conditions are applied to the tight binding model of poly(para-phenylene), taking into account of the…

Materials Science · Physics 2007-05-23 Kikuo Harigaya

Charge-transfer (CT) exciton effects are investigated for the optical absorption spectra of crosslinked C60 systems by using the intermediate exciton theory. We consider the C60-dimers, and the two (and three) molecule systems of the…

chem-ph · Physics 2008-02-03 K. Harigaya

We have studied the exciton states in two coupled conjugated polymer chains which are modeled individually by the Su-Schrieffer-Heeger Hamiltonian and coupled by an interchain electron-transfer term. Both the intra- and inter-chain long…

Soft Condensed Matter · Physics 2009-10-30 Z. G. Yu , M. W. Wu , X. S. Rao , X. Sun , A. R. Bishop

The optical excitations in C$_{60}$ and higher fullerenes, including isomers of C$_{76}$, C$_{78}$, and C$_{84}$, are theoretically investigated. We use a tight binding model with long-range Coulomb interactions, treated by the Hartree-Fock…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

Charge-transfer (CT) exciton effects are investigated for the optical absorption spectra of crosslinked C60 systems by using the intermediate exciton theory. We consider the C60-dimers, and the two (and three) molecule systems of the…

Condensed Matter · Physics 2007-05-23 Kikuo Harigaya

A theory of optical excitations by using a tight binding model with long-range Coulomb interactions is developed. The model is applied to a C60 molecule and a cluster, and is treated by the Hartree-Fock approximation followed by a…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya , Shuji Abe

We investigate the effect of exciton coupling on the optical absorption spectrum of polymer molecules under conditions of strong inhomogeneous broadening. We demonstrate that the dependence of the maximum in the rescaled absorption spectrum…

Chemical Physics · Physics 2009-11-13 A. L. Burin , J. A. Dickman , D. B. Uskov , C. F. F. Hebbard , G. C. Schatz

Electronic structures and optical excitations in Moebius conjugated polymers are studied theoretically. Periodic and Moebius boundary conditions are applied to the tight binding model of poly(para-phenylene), taking exciton effects into…

Materials Science · Physics 2007-05-23 Kikuo Harigaya

Using the Hubbard model we study how the process of high-order harmonic generation (HHG) is modified by beyond mean-field electron-electron correlation for both finite and bulk systems. A finite-size enhancement of the HHG signal is found…

Atomic Physics · Physics 2022-06-01 Thomas Hansen , Simon Vendelbo Bylling Jensen , Lars Bojer Madsen

Nonlinear optical phenomena are at the heart of various technological domains such as high-speed data transfer, optical logic applications, and emerging fields such as non-reciprocal optics and photonic time crystal design. However,…

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