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We numerically study the collective excitations present in isotropic superconductors including a screened Coulomb interaction. By varying the screening strength, we analyze its impact on the system. We use a formulation of the effective…

Superconductivity · Physics 2025-09-10 Joshua Althüser , Götz S. Uhrig

We investigate the nonlinear optical susceptibilities of Mott insulators with the dynamical mean field approximation. The two-photon absorption (TPA) and the third-harmonic generation (THG) spectra are calculated, and the classification by…

Strongly Correlated Electrons · Physics 2009-11-13 Takanobu Jujo

We study the contribution of the Higgs amplitude mode on the nonlinear optical response of superconductors beyond the BCS approximation by taking into account the retardation effect in the phonon-mediated attractive interaction. To evaluate…

Superconductivity · Physics 2017-01-02 Naoto Tsuji , Yuta Murakami , Hideo Aoki

Motivated by the gigantic nonlinear optical response in the halogen-bridged Ni-compounds, the underlying electronic states of the compounds are examined in the one-dimensional two-band Hubbard model, by studying the current-current…

Strongly Correlated Electrons · Physics 2009-11-10 H. Matsueda , T. Tohyama , S. Maekawa

We present a calculation of Third Harmonic Generation (THG) for two-band systems using the length gauge that avoids unphysical divergences otherwise present in the evaluation of the third order current density response. The calculation is…

Mesoscale and Nanoscale Physics · Physics 2018-01-31 F. Hipolito , T. G. Pedersen

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

Optics · Physics 2022-03-03 Davis M. Welakuh , Prineha Narang

We show that the charge transfer excitons in a Hubbard model system including nearest neighbor Coulomb interactions effectively attain some charge in doped systems and become visible in photoelectron and inverse photoelectron…

Strongly Correlated Electrons · Physics 2009-10-30 J. van den Brink , R. Eder , G. A. Sawatzky

A manifestation of electron-hole pairing in nonlinear electromagnetic response of a double layer graphene system is studied. It is shown that the pairing causes the appearance of a number of peaks in the frequency dependence of the…

Strongly Correlated Electrons · Physics 2017-10-20 K. V. Germash , D. V. Fil

The scattering and recombination processes between two triplet excitons in conjugated polymers are investigated by using a nonadiabatic evolution method, based on an extended Su-Schrieffer-Heeger model including interchain interactions. Due…

Chemical Physics · Physics 2010-10-05 Y. Meng , B. Di , X. J. Liu , Y. D. Wang , Z. An

We investigate the high-order harmonic generation (HHG) in doped semiconductors. The HHG is simulated with the single-electron time-dependent Schr\"{o}dinger equation (TDSE). The results show that the high-order harmonics in the second…

Optics · Physics 2017-11-22 Tengfei Huang , Xiaosong Zhu , Liang Li , Xi Liu , Pengfei Lan , Peixiang Lu

We study optical harmonic generation on the 1S exciton-polariton in the semiconductor ZnSe. Intense and spectrally narrow exciton resonances are found in optical second (SHG), third (THG), and fourth (FHG) harmonic generation spectra. The…

Optics · Physics 2020-07-29 Johannes Mund , Dmitri R. Yakovlev , Marina A. Semina , Manfred Bayer

The efficient optical second-harmonic generation (SHG) of two-dimensional (2D) crystals, coupled with their atomic thickness that circumvents the phase-match problem, has garnered considerable attention. While various 2D heterostructures…

Materials Science · Physics 2023-10-31 Wontaek Kim , Gyouil Jeong , Juseung Oh , Jihun Kim , Kenji Watanabe , Takashi Taniguchi , Sunmin Ryu

Molecular exciton effects in the neutral and maximally doped C60 (C70) are considered using a tight binding model with long-range Coulomb interactions and bond disorder. By comparing calculated and observed optical spectra, we conclude that…

chem-ph · Physics 2008-02-03 Kikuo Harigaya , Shuji Abe

We report on a comprehensive experimental and theoretical study of optical third harmonic generation (THG) on the exciton-polariton resonances in the zinc-blende semiconductors GaAs, CdTe, and ZnSe subject to an external magnetic field,…

The nonlinear optical response of an excitonic insulator coupled to lattice degrees of freedom is shown to depend in strong and characteristic ways on whether the insulating behavior originates primarily from electron-electron or…

Strongly Correlated Electrons · Physics 2021-01-04 Denis Golez , Zhiyuan Sun , Yuta Murakami , Antoine Georges , Andrew J. Millis

We explore the two-dimensional extended Hubbard model on the triangular lattice in the high doping regime. On-site and nearest-neighbour repulsive interactions are treated in a non-perturbative way by means of Extended Dynamical Mean Field…

Strongly Correlated Electrons · Physics 2017-09-26 Sophie Chauvin , Thomas Ayral , Lucia Reining , Silke Biermann

We investigate second harmonic generation (SHG) from hexagonal periodic arrays of triangular nano-holes of aluminum using a self-consistent methodology based on the hydrodynamics-Maxwell-Bloch approach. It is shown that angular polarization…

Optics · Physics 2021-07-07 Maxim Sukharev , Adi Salomon , Joseph Zyss

We theoretically investigate the effects of Coulomb interaction, at the level of unscreened Hartree-Fock approximation, on third harmonic generation of undoped graphene in an equation of motion framework. The unperturbed electronic states…

Mesoscale and Nanoscale Physics · Physics 2020-01-01 J. L. Cheng , J. E. Sipe , Chunlei Guo

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…