English
Related papers

Related papers: On multiphoton absorption by molecules

200 papers

A fundamental issue that limits the efficiency of many photoelectrochemical systems is that the photon absorption length is typically much longer than the electron diffusion length. Various photon management schemes have been developed to…

We study Fermi edge singularities in photo-absorption spectra of generic mesoscopic systems such as quantum dots or nanoparticles. We predict deviations from macroscopic-metallic behavior and propose experimental setups for the observation…

Mesoscale and Nanoscale Physics · Physics 2009-08-12 M. Hentschel , D. Ullmo , H. U. Baranger

We consider theoretically nonlinear effects in a semiconductor quantum well embedded inside a photonic microcavity. Two-photon absorption by a 2p exciton state is considered and investigated; the matrix element of two-photon absorption is…

Mesoscale and Nanoscale Physics · Physics 2016-12-21 A. A. Pervishko , T. C. H. Liew , V. M. Kovalev , I. G. Savenko , I. A. Shelykh

The dynamics of a vibronic system in a lossy two-mode cavity is studied, with the first mode being resonant to the electronic transition and the second one being nearly resonant due to Raman transitions. We derive analytical solutions for…

Quantum Physics · Physics 2011-06-13 P. Grünwald , S. K. Singh , W. Vogel

Rydberg atomic sensors have been adopted for novel radio frequency (RF) measurement technique and the sensing capability for signals in multiple frequencies makes it attractive for multi-user communication. However, unlike traditional…

Signal Processing · Electrical Eng. & Systems 2025-06-27 Hao Wu , Chongwu Xie , Xinyuan Yao , Kang-Da Wu , Shanchi Wu , Rui Ni , Guo-Yong Xiang , Chen Gong

We investigate simultaneous multiphoton-multiatom processes in atomic gases exposed to laser fields under specific frequency conditions, where multiple atoms are simultaneously excited through the absorption of one laser photon each. These…

Atomic Physics · Physics 2025-04-09 Yongle Yu

We study the absorption and dispersion properties of a weak tunable probe field in a four-level Y-type atomic system driven by two strong laser (coupling) fields within the framework of density matrix formalism. It is found that the probe…

Atomic Physics · Physics 2014-03-12 L. Safari , D. Iablonskyi , F. Fratini

We reexamine the invariance of two-photon transition matrix elements and corresponding two-photon Rabi frequencies under the "gauge" transformation from the length to the velocity gauge. It is shown that gauge invariance, in the most…

Quantum Physics · Physics 2017-05-23 U. D. Jentschura

We present a theory for the diffraction of large molecules or nanoparticles at a standing light wave. Such particles can act as a genuine photon absorbers due to their numerous internal degrees of freedom effecting fast internal energy…

Quantum Physics · Physics 2016-10-26 Kai Walter , Stefan Nimmrichter , Klaus Hornberger

Nonlinear optical effects can be enhanced in tapered optical fibers with diameters less than the wavelength of the propagating light. Here we report on the observation of two-photon absorption using tapered fibers in rubidium vapor at power…

Quantum Physics · Physics 2010-10-22 S. M. Hendrickson , M. M. Lai , T. B. Pittman , J. D. Franson

We investigate theoretically the photo absorbtion of the cluster of alkali atoms embedded into a single mode quantum microcavity. We show that when the energy of the giant plasmonic resonance lies close to the energy of the cavity mode, the…

Mesoscale and Nanoscale Physics · Physics 2013-03-15 I. G. Savenko , R. G. Polozkov , I. A. Shelykh

Spectral properties of fluorescent radiation from a two-level quantum system with broken inversion spatial symmetry, which can be described by a model of an one-electron two-level atom whose electric dipole moment operator has permanent…

Quantum Physics · Physics 2024-12-17 Nikolai N. Bogolyubov, , Andrey V. Soldatov

We discuss two-photon physics, taking for illustration the particular but topical case of resonance fluorescence. We show that the basic concepts of interferences and correlations provide at the two-photon level an independent and…

Quantum Physics · Physics 2024-10-10 Eduardo Zubizarreta Casalengua , Fabrice P. Laussy , Elena del Valle

A theoretical and experimental investigation of the intensity noise reduction induced by two-photon absorption in a Er,Yb:Glass laser is reported. The time response of the two-photon absorption mechanism is shown to play an important role…

Optics · Physics 2015-06-15 Abdelkrim El Amili , Gaël Kervella , Mehdi Alouini

Since the mass of the electron is very small relative to atomic masses, Thomson scattering of low-energy photons ($h\nu \ll m_ec^2$) produces thermal Doppler frequency shifts that are much larger than atomic Doppler widths. A method is…

Astrophysics · Physics 2011-05-23 G. B. Rybicki , D. G. Hummer

Multi-photon emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multi-level atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has…

A two-level atom interacting with a single radiation mode is considered, without the rotating-wave approximation, in the strong coupling regime. It is shown that, in agreement with the recent results on Rabi oscillations in a Josephson…

Quantum Physics · Physics 2009-11-07 Marco Frasca

We apply input-output theory with quantum pulses [AH Kiilerich, K M\o lmer, Phys. Rev. Lett. {\bf 123}, 123604 (2019)] to a model of a new type of two-photon detector consisting of one molecule that can detect two photons arriving…

Quantum Physics · Physics 2021-10-20 Saumya Biswas , S. J. van Enk

We investigate quantum beats in the arrival-time distribution of single photons from a single trapped $^{40}$Ca$^+$ ion, revealing their fundamentally different physical origins in two distinct experimental situations: In a $\Lambda$-type…

Quantum Physics · Physics 2014-08-19 Michael Schug , Christoph Kurz , Pascal Eich , Jan Huwer , Philipp Müller , Jürgen Eschner

In this paper we consider a general model of an atom with n energy levels interacting with n-1 external (laser) fields which is a natural extension in the two and three level systems. We exactly solve the Schr{\" o}dinger equation to obtain…

Quantum Physics · Physics 2007-05-23 Kazuyuki Fujii , Kyoko Higashida , Ryosuke Kato , Yukako Wada