Related papers: On multiphoton absorption by molecules
Quantum networks require flying qubits that transfer information between the nodes. This may be implemented by means of single atoms (the nodes) that emit and absorb single photons (the flying qubits) and requires full control of photon…
We analyze a system composed of a superconducting flux qubit coupled to a transmission-line resonator driven by two signals with frequencies close to the resonator's harmonics. The first strong signal is used for exciting the system to a…
We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…
An analytical microscopic theory for the resonant multiple scattering of light by cold atoms with arbitrary internal degeneracy is presented. It permits to calculate the average amplitude and the average intensity for one-photon states of…
Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…
This paper is concerned with two rather basic phenomena: the incoherent fluorescence spectrum of an atom driven by an intense laser field and the coupling of the atom to the (empty) modes of the radiation field. The sum of the many-photon…
We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS's photon absorption spectrum. Tuning and controlling the emission and the absorption is of much interest e.g.\ for the…
Photoinduced biological processes occur via one photon absorption in natural light, which is weak, CW and incoherent, but are often studied in the laboratory using pulsed coherent light. Here we compare the response of a molecule to these…
We present a non-Hermitian theory of atomic and molecular absorption, which enables computing the absorption spectrum of multi-electron atoms and molecules without using any fitting parameters. We propose a method for optically inducing…
We present combined measurements of the spatially-resolved optical spectrum and the total excited-atom number in an ultracold gas of three-level atoms under electromagnetically induced transparency conditions involving high-lying Rydberg…
The rotational echo response of molecules is found to strongly depend on the delay between the two ultrashort laser pulses, as opposed to two-level systems. We study this dependence experimentally and theoretically and show that by…
The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…
By extending the Berry--Robnik approach for the nearly integrable quantum systems,\cite{[1]} we propose one possible scenario of the energy level spacing distribution that deviates from the Berry--Robnik distribution. The result described…
Absorption spectroscopy is a fundamental tool for probing molecular structure. However, performing absorption spectroscopy on individual molecules is challenging due to the low signal-to-noise ratio. Here, we report on a nondestructive…
We investigate the effect of a laser shining perpendicularly to a waveguide channeling two-level atoms. For weak transversal coupling the excitation of transverse atomic levels occurs at avoided crossings associated with "Rabi resonances"…
We study resonance flourescence in a four level ladder system and illustrate some novel features due to quantum interference and atomic coherence effects. We find that under three photon resonant conditions, in some region of the parameter…
The three level photon echo has been described in different works by using rotating wave approximation but none of them did not get results which show the effects of field's frequencies on frequency of ground level of system. In this work,…
A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field…
We determine the energy loss spectrum per time-interval of a relativistic charge traversing a dispersive medium. Polarization and absorption effects in the medium are modelled via a complex index of refraction. We find that the spectrum…
It is shown that the absorption of photons at energies > 1 TeV (much higher than the mass of the Higgs boson ~ 100 GeV) is a multi-channel one as opposed to the purely electron pair like absorption at lower energies. The observation on…