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We report the results of molecular dynamics simulation of a spatiotemporal evolution of the locally photoexcited electrons and holes localized in two separate layers. It is shown that the ring-shaped spatial pattern of luminescence forms…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 A. V. Paraskevov , S. E. Savel'ev

Understanding the fine structure of excitons is crucial for optoelectronic and quantum photonic applications of lead halide perovskites. It is demonstrated that polarization-sensitive photon echo spectroscopy in magnetic field provides a…

We examine the multiple exciton population dynamics in PbS quantum dots by ultrafast spectrally-resolved supercontinuum transient absorption (SC-TA). We simultaneously probe the first three excitonic transitions over a broad spectral range.…

Mesoscale and Nanoscale Physics · Physics 2016-09-21 F. Gesuele , M. Y. Sfeir , W. -K. Koh , C. B. Murray , T. F. Heinz , C. W. Wong

The elementary optical excitations of a two-dimensional electron or hole system have been identified as exciton-Fermi-polarons. Nevertheless, the connection between the bound state of an exciton and an electron, termed trion, and…

Mesoscale and Nanoscale Physics · Physics 2020-06-30 Atac Imamoglu , Ovidiu Cotlet , Richard Schmidt

The problem of an electron-hole system interacting through a contact potential and moving in a one-dimensional quantum ring threaded by an Aharonov-Bohm flux is considered, both with respect to the system's energetics as well as its optical…

Mesoscale and Nanoscale Physics · Physics 2011-03-07 A. V. Ghazaryan , A. P. Djotyan , K. Moulopoulos , A. A. Kirakosyan

We study the texture of the exciton condensate at low temperatures in an independently gated electron-hole bilayer system. A model Hamiltonian is solved in real space within a mean-field approximation. It is found that, with increased…

Strongly Correlated Electrons · Physics 2015-05-14 Jian-Xin Zhu , A. R. Bishop

Long-lived indirect excitons (IXs) exhibit a rich phase diagram, including a Bose-Einstein condensate (BEC), a Wigner crystal, and other exotic phases. Recent experiments have hinted at a new, "classical" liquid of IXs above the BEC…

Mesoscale and Nanoscale Physics · Physics 2022-09-07 Paul R. Wrona , Eran Rabani , Phillip L. Geissler

he properties of excitons formed in spherical quantum dots are studied using the $\mathbf{k}\cdot\mathbf{p}$ method within the Hartree approximation. The spherical quantum dots considered have a central core and several concentric layers of…

Mesoscale and Nanoscale Physics · Physics 2019-10-11 Mariano Garagiola , Omar Osenda

The negatively charged quasi-two-dimensional exciton ($X^-$) is studied numerically in the presence of a uniform B-field and various in-plane confinements. The corresponding photoluminescence (PL) spectra, including shakeup processes, are…

Condensed Matter · Physics 2009-10-30 J. R. Chapman , N. F. Johnson , V. N. Nicopoulos

Two-dimensional (2D) monolayer phosphorene, a 2D system with quasi-one-dimensional (quasi-1D) excitons, provides a unique 2D platform for investigating the dynamics of excitons in reduced dimensions and fundamental many-body interactions.…

Materials Science · Physics 2016-02-03 Renjing Xu , Jiong Yang , Ye Win Myint , Jiajie Pei , Han Yan , Fan Wang , Yuerui Lu

Exciton-exciton interactions are fundamental to the light-emitting properties of semiconductors, influencing applications from lasers to quantum light sources. In this study, we investigate the spectroscopic signatures and binding energy of…

Long lasting coherence in photosynthetic pigment-protein complexes has been observed even at physiological temperatures. Experiments have demonstrated quantum coherent behaviour in the long-time operation of the D-Wave quantum computer as…

Chemical Physics · Physics 2016-05-23 D. Drakova , G. Doyen

Nonlinear optical processes in low dimensional materials are often weak or symmetry forbidden, limiting their use in nanoscale light sources and on chip frequency conversion. Here, we show that combining two weakly nonlinear systems,…

Indirect excitons -- pairs of electrons and holes spatially separated in semiconductor bilayers or quantum wells -- are known to undergo Bose-Einstein condensation and to form a quantum fluid. Here we show that this superfluid may…

Quantum Gases · Physics 2015-03-17 J. Boening , A. Filinov , M. Bonitz

The attraction between electrons and holes in semiconductors forms excitons, which largely determine the optical properties of the hosting material, and hence the device performance, especially for low-dimensional systems. Mono- and…

Mesoscale and Nanoscale Physics · Physics 2018-03-20 Guowei Zhang , Andrey Chaves , Shenyang Huang , Fanjie Wang , Qiaoxia Xing , Tony Low , Hugen Yan

The evolution of excitons from 2D to 3D is of great importance in photo-physics, yet the layer-dependent exciton polarizability has not been investigated in 2D semiconductors. Here, we determine the exciton polarizabilities for 3- to…

Simulating the irreversible quantum dynamics of exciton and electron transfer problems poses a nontrivial challenge. Because the irreversibility of the system dynamics is a result of quantum thermal activation and dissipation caused by the…

Chemical Physics · Physics 2021-03-30 Seiji Ueno , Yoshitaka Tanimura

The Rabi model, a two-level atom coupled to a harmonic oscillator, can undergo a second-order quantum phase transition (QPT) [M. -J. Hwang et al, Phys. Rev. Lett. 115, 180404 (2015)]. Here we show that the Rabi QPT accompanies critical…

Quantum Physics · Physics 2016-08-24 Ricardo Puebla , Myung-Joong Hwang , Martin B. Plenio

Excitons - the particle-hole bound states - composed of localized electron-hole states in semiconducting systems are crucial to explaining the optical spectrum. Spectroscopic measurements can contain signatures of these two particle bound…

Mesoscale and Nanoscale Physics · Physics 2018-06-19 Avinash Rustagi , Alexander F. Kemper

Recent experiments on two-dimensional exciton systems have shown the excitons collect in shallow in-plane traps. We find that Bose condensation in a trap results in a dramatic change of the exciton photoluminescence (PL) angular…

Condensed Matter · Physics 2007-05-23 Jonathan Keeling , L. S. Levitov , P. B. Littlewood