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We develop a Hamiltonian formalism to study energy and position/momentum correlations between a single Stokes photon and a single material excitation that are created as a pair in the spontaneous Raman scattering process. Our approach…

Quantum Physics · Physics 2020-01-16 Kai Shinbrough , Yanting Teng , Bin Fang , Virginia O. Lorenz , Offir Cohen

The photochemistry of a molecular ensemble coupled to a resonance cavity and triggered by a femtosecond laser pulse is investigated from a real-time, quantum dynamics perspective with the multi-configuration time-dependent Hartree method.…

Chemical Physics · Physics 2018-06-20 Oriol Vendrell

The propagation of polarized photons in optical media can be effectively modeled by means of quantum dynamical semigroups. These generalized time evolutions consistently describe phenomena leading to loss of phase coherence and dissipation…

Quantum Physics · Physics 2009-11-07 F. Benatti , R. Floreanini

The general expressions for the time development of the ensemble averages of E^- and E^-E^+ are found for N two level molecules (TLMs) interacting with a single mode electromagnetic field. The TLMs are assumed to be at equivalent mode…

Quantum Physics · Physics 2015-06-12 Michael T. Tavis , Frederick W. Cummings

Modification of spontaneous decay in space and time is a central topic of quantum physics. It has been predominantly investigated in the context of cavity quantum electrodynamics (QED), gaining new interest recently in the domain of…

Quantum Physics · Physics 2022-03-01 Stefan Richter , Sebastian Wolf , Joachim von Zanthier , Ferdinand Schmidt-Kaler

A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…

Chemical Physics · Physics 2009-11-13 F. Shikerman , E. Barkai

Multi-photon absorption is a well-known phenomenon. With atom lasers a similar process could take place for massive particles, the ionization of an atom or molecule by the successive interaction with various particles. This process would…

Quantum Physics · Physics 2009-11-13 Pedro Sancho

As a contribution to quantum optics in the vicinity of surfaces we study the single atom spontaneous emission in a linear chain of two-level atoms. The electromagnetic field is thereby treated with the help of integro-differential equations…

Quantum Physics · Physics 2009-10-30 Konstantin Krutitsky , Juergen Audretsch

In the present work the model of a single-atom laser generating in the regime when incoherent pumping rate coincides with the cavity decay rate is theoretically investigated. Using the stationary equation for the phase averaged Glauber P…

Quantum Physics · Physics 2020-11-09 Nikolay Larionov

We study the photon blockade at exceptional points for a non-Hermitian optomechanical system coupled to the driven whispering-gallery-mode microresonator with two nanoparticles under the weak optomechanical coupling approximation, where…

Quantum Physics · Physics 2024-04-19 J. Y. Sun , H. Z. Shen

We study a general problem of the translational/rotational/vibrational/electronic dynamics of a diatomic molecule exposed to an interaction with an arbitrary external electromagnetic field. The theory developed in this paper is relevant to…

Quantum Physics · Physics 2016-09-28 Milan Sindelka , Nimrod Moiseyev

For photo-dissociation of a single hydrogen molecule (H2) with combined XUV and IR laser pulses, we demonstrate optical control of the emission direction of the photoelectron with respect to the outgoing neutral fragment (the H-atom).…

The emission of the hard photon by the initial state is considered. The nucleon polarization and the differential cross sections for some experimental conditions have been calculated. The case of the emission of the collinear (with respect…

High Energy Physics - Phenomenology · Physics 2018-03-23 G. I. Gakh , N. P. Merenkov , M. I. Konchatnij , A. G. Gakh

The decay of photoexcited quantum systems (examples are photodissociation of molecules and autoionization of atoms) can be viewed as a half-collision process (an incoming photon excites the system which subsequently decays by dissociation…

Disordered Systems and Neural Networks · Physics 2009-11-10 T. Gorin , B. Mehlig , W. Ihra

We observe the buildup of a frequency-shifted reverse light field in a unidirectionally pumped high-$Q$ optical ring cavity serving as a dipole trap for cold atoms. This effect is enhanced and a steady state is reached, if via an optical…

Quantum Physics · Physics 2009-11-10 D. Kruse , C. von Cube , C. Zimmermann , Ph. W. Courteille

A sequence of single photons is emitted on demand from a single three-level atom strongly coupled to a high-finesse optical cavity. The photons are generated by an adiabatically driven stimulated Raman transition between two atomic ground…

Quantum Physics · Physics 2009-11-07 Axel Kuhn , Markus Hennrich , Gerhard Rempe

The Thomson backscattering of an electron moving in combined fields is studied by a dynamically assisted mechanism. The combined fields are composed of two co-propagating laser fields and a magnetic field, where the first laser field is…

Optics · Physics 2019-05-07 Zhijing Chen , Li Zhao , Chun Jiang , Haibo Sang , Bai-Song Xie

We demonstrate fast and accurate control of the evolution of collective atomic coherences in an Erbium doped solid using external electric fields. This is achieved by controlling the inhomogeneous broadening of Erbium ions emitting at 1536…

There are many ways of calculating photon statistics in quantum optics in general and single molecule spectroscopy in particular such as the generating function method, the quantum jump approach or time ordering methods. In this paper…

Optics · Physics 2007-10-30 Faina Shikerman , Yong He , Eli Barkai

We present an \emph{ab-initio} approach for computing the photoionization spectrum near autoionization resonances in multi-electron systems. While traditional (Hermitian) theories typically require computing the continuum states, which are…

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