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Motivated by a revision of the classical equations of electromagnetism that allow for the inclusion of solitary waves in the solution space, the material collected in these notes examines the consequences of adopting the modified model in…

General Physics · Physics 2019-09-27 Daniele Funaro

We present an experiment where a single molecule strongly affects the amplitude and phase of a laser field emerging from a subwavelength aperture. We achieve a visibility of -6% in direct and +10% in cross-polarized detection schemes. Our…

Quantum Physics · Physics 2007-05-23 I. Gerhardt , G. Wrigge , P. Bushev , G. Zumofen , R. Pfab , V. Sandoghdar

We provide a theory of the deflection of polar and non-polar rotating molecules by inhomogeneous static electric field. Rainbow-like features in the angular distribution of the scattered molecules are analyzed in detail. Furthermore, we…

Chemical Physics · Physics 2015-05-20 E. Gershnabel , I. Sh. Averbukh

We study a system of two distant quantum emitters coupled via a one-dimensional waveguide where the electromagnetic field has a direction-dependent velocity. As a consequence, the onset of collective emission is non-simultaneous and, for…

Quantum Physics · Physics 2022-05-04 P. Solano , P. Barberis-Blostein , K. Sinha

We study spontaneous emission from an atom under the action of laser fields. We consider two different energy level diagrams. The first one consists of two levels resonantly driven by laser radiation where either of levels may decay to a…

Quantum Physics · Physics 2007-05-23 V. O. Chaltykyan , A. D. Gazazyan , Y. T. Pashayan

We employ heterodyne interferometry to investigate the effect of a single organic molecule on the phase of a propagating laser beam. We report on the first phase-contrast images of individual molecules and demonstrate a single-molecule…

Quantum Physics · Physics 2015-05-27 M. Pototschnig , Y. Chassagneux , J. Hwang , G. Zumofen , A. Renn , V. Sandoghdar

A theoretical study of the rotational dynamics of a linear polar molecule in a two-color non-resonant cw laser field is presented. By systematically considering the interactions of this field with the electric dipole moment, polarizability…

Quantum Physics · Physics 2020-08-26 David Mellado-Alcedo , Niurka R. Quintero , Rosario González-Férez

Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…

Atomic Physics · Physics 2019-07-23 Xueping Long , Scarlett S. Yu , Andrew M. Jayich , Wesley C. Campbell

A photon echo experiment has been performed using accumulated highly attenuated laser pulses. We show experimentally that the photon echo process can be performed with, on the average, less than one photon in each pair of excitation pulses.…

Quantum Physics · Physics 2009-11-10 Nicklas Ohlsson , Mattias Nilsson , Stefan Kroll

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

The production of single photons using rephased amplified spontaneous emission is examined. This process produces single photons on demand with high efficiency by detecting the spontaneous emission from an atomic ensemble, then applying a…

Single dye molecules at cryogenic temperatures display many spectroscopic phenomena known from free atoms and are thus promising candidates for fundamental quantum optical studies. However, the existing techniques for the detection of…

Quantum Physics · Physics 2008-02-12 Gert Wrigge , Ilja Gerhardt , Jaesuk Hwang , Gert Zumofen , Vahid Sandoghdar

For nearly a decade, it has been a mystery why the small average number of photons absorbed per atom from an ultrashort laser pulse is able to induce a strong magnetization within a few hundred femtoseconds. Here we resolve this mystery by…

Optics · Physics 2015-05-18 M. S. Si , G. P. Zhang

Superradiance in an ensemble of atoms leads to the collective enhancement of radiation in a particular mode shared by the atoms in their spontaneous decay from an excited state. The quantum aspects of this phenomenon are highlighted when…

We study light-mediated interactions between spatially separated molecules using real-time quantum electrodynamical time-dependent density functional theory based on the Pauli-Fierz Hamiltonian. An ultrashort delta-kick excitation…

Chemical Physics · Physics 2026-01-22 Yetmgeta Aklilu , Tiany Yang , Cody Covington , Kalman Varga

The dynamics of spontaneous emission of an atomic system is studied in the framework of an open quantum system. The resulting quantum master equation for the atomic system is non hermitian. The generator $\mathcal{L}$ can possess…

Quantum Physics · Physics 2016-03-23 Morag Am-Shallem , Ronnie Kosloff , Nimrod Moiseyev

Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…

Atomic and Molecular Clusters · Physics 2011-05-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

Revivals of optical coherence of molecular photoassociation driven by two ultrashort laser pulses are addressed in the Condon approach. Based on textbook examples and numerical simulation of KrF excimer molecules, a prediction is made about…

Atomic Physics · Physics 2015-06-26 Alexander G. Rudavets , Alexander M. Dykhne

Echo is a ubiquitous phenomenon found in many physical systems, ranging from spins in magnetic fields to particle beams in hadron accelerators. It is typically observed in inhomogeneously broadened ensembles of nonlinear objects, and is…

We show how an initial localized radiative excitation in a two-dimensional array of cold atoms can be converted into highly-directional coherent emission of light by protecting the spreading of the excitation across the array in a…

Quantum Gases · Physics 2020-05-06 K. E. Ballantine , J. Ruostekoski