Related papers: Reaching optimally oriented molecular states by la…
Proposals to reach the next generation of laser intensities through Raman or Brillouin backscattering have centered on optical frequencies. Higher frequencies are beyond the range of such methods mainly due to the wave damping that…
Adaptive methods of laser irradiation of plasmas are proposed consisting of deterministic, `on-off' amplitude modulations in time, and intermittently changing speckle-patterns. These laser pulses consist of a series of picosecond time-scale…
We show that a topological investigation of the phase space of a Semiconductor Ring Laser can be used to devise switching schemes which are alternative to optical pulse injection of counter-propagating light. To provide physical insight in…
The capability to control molecular rotation for field-free orientation, which arranges molecules in specific spatial directions without external fields, is crucial in physics, chemistry, and quantum information science. However,…
A general consideration on the phase rotations in quantum searching algorithm is taken in this work. As four phase rotations on the initial state, the marked states, and the states orthogonal to them are taken account, we deduce a phase…
The tomographic imaging of arbitrary molecular orbitals via high-order harmonic generation requires that electrons recollide from one direction only. Within a semi-classical model, we show that extremely short phase-stabilized laser pulses…
The time-optimal technique of spatial localization of the random pulsed-point source that has the uniform distribution density on search interval and indicating itself by generation of the instant impulses (delta functions) at random time…
The field of attosecond science was first enabled by nonlinear compression of intense laser pulses to a duration below two optical cycles. Twenty years later, creating such short pulses still requires state-of-the-art few-cycle laser…
A common approach to reduce the linewidth of a laser is an increase of its resonator length. In large gas lasers, however, the frequency spacing between longitudinal modes of the resonator easily becomes significantly smaller than the…
We study the control by electromagnetic fields of molecular alignment and orientation, in a linear, rigid rotor model. With the help of a monotonically convergent algorithm, we find that the optimal field is in the microwave part of the…
A short overview of laser-plasma acceleration of ions is presented. The focus is on some recent experimental results and related theoretical work on advanced regimes. These latter include in particular target normal sheath acceleration…
Controlling molecular reactivity by shaped laser pulses is a long-standing goal in chemistry. Here we suggest a direct optimal control approach which combines external pulse optimization with other control parameters arising in the upcoming…
We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…
Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of…
In this paper we study the problem of designing periodic orbits for a special class of hybrid systems, namely mechanical systems with underactuated continuous dynamics and impulse events. We approach the problem by means of optimal control.…
We analyze the simultaneous time-optimal control of two-spin systems. The two non coupled spins which differ in the value of their chemical offsets are controlled by the same magnetic fields. Using an appropriate rotating frame, we restrict…
We investigate theoretically the ability of an optical centrifuge - a laser pulse whose linear polarization is rotating at an accelerated rate, to control molecular rotation in the regime when the rigid-rotor approximation breaks down due…
Optimal control experiments can readily identify effective shaped laser pulses, or "photonic reagents", that achieve a wide variety of objectives. For many practical applications, an important criterion is that a particular photonic reagent…
Laser plasma acceleration at kilohertz repetition rate has recently been shown to work in two different regimes, with pulse lengths of either 30 fs or 3.5 fs. We now report on a systematic study in which a large range of pulse durations and…
We propose a method for achieving highly efficient transfer between the vibrational states in a diatomic molecule. The process is mediated by strong laser pulses and can be understood in terms of light-induced potentials. In addition to…