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Praseodymium (Pr$^{3+}$) ions doped in the site 1 of yttrium orthosilicate (Y$_2$SiO$_5$) has been widely employed as the photonic quantum memory due to their excellent optical coherence and spin coherence. While praseodymium ions occupying…

Quantum Physics · Physics 2020-05-26 Yi-Xin Xiao , Zong-Quan Zhou , Yu Ma , Tian-Shu Yang , You-Zhi Ma , Chuan-Feng Li , Guang-Can Guo

In many important situations the dominant dephasing mechanism in cryogenic rare-earth-ion doped systems is due to magnetic field fluctuations from spins in the host crystal. Operating at a magnetic field where a transition has a zero…

Atomic Physics · Physics 2015-06-03 D. L. McAuslan , J. G. Bartholomew , M. J. Sellars , J. J. Longdell

Rare-earth ions in dielectric crystals are interesting candidates for storing quantum states of photons. A limiting factor on the optical density and thus the conversion efficiency is the distortion introduced in the crystal by doping…

The spin coherence time of $^{151}$Eu$^{3+}$ which substitutes the yttrium at site 1 in Y$_2$SiO$_5$ crystal has been extended to 6 hours in a recent work [\textit{Nature} \textbf{517}, 177 (2015)]. To make this long-lived spin coherence…

We characterize the Europium (Eu$^{3+}$) hyperfine interaction of the excited state ($^5$D$_0$) and determine its effective spin Hamiltonian parameters for the Zeeman and quadrupole tensors. An optical free induction decay method is used to…

Rovibrational energies, wave functions, and Raman transition moments are reported for the lowest-energy states of the H$_3^+$ molecular ion including the magnetic couplings of the proton spins and molecular rotation in the presence of a…

Chemical Physics · Physics 2024-10-29 Gustavo Avila , Ayaki Sunaga , Stanislav Komorovsky , Edit Matyus

We investigate the decoherence of Er$^{3+}$ in Y$_2$SiO$_5$ at low magnetic fields using the photon-echo technique. We reproduce accurately a variety of the decay curves with a unique coherence time by considering the so-called…

Quantum Physics · Physics 2020-09-16 B. Car , J. -L. Le Gouët , T. Chanelière

We report measurements of the branching fraction, hyperfine constant, and second-order Zeeman coefficient of the D$_{5/2}$ level in $^{171}$Yb$^+$ with up to two orders-of-magnitude improvement in precision compared to previously reported…

Atomic Physics · Physics 2021-08-04 T. R. Tan , C. L. Edmunds , A. R. Milne , M. J. Biercuk , C. Hempel

We report precise measurement of the hyperfine splitting and calculation of the Zeeman coefficients of the $^{171}$Yb$^+$ ground state. The absolute hyperfine splitting frequency is measured using high-resolution laser-microwave…

Atomic Physics · Physics 2023-09-12 J. Z. Han , B. Q. Lu , N. C. Xin , Y. M. Yu , H. R. Qin , S. T. Chen , Y. Zheng , J. G. Li , J. W. Zhang , L. J. Wang

The decoherence times of orthogonally phased components of the optical transition dipole moment in a two-level system have been observed to differ by an order of magnitude. This phase anisotropy is observed in coherent transient experiments…

Quantum Physics · Physics 2008-11-26 G. J. Pryde , M. J. Sellars , N. B. Manson

A sequence of optical holeburning pulses is used to isolate transitions between hyperfine levels, which are initially buried within an inhomogeneously broadened absorption line. Using this technique selected transitions can be studied with…

Other Condensed Matter · Physics 2009-11-10 Mattias Nilsson , Lars Rippe , Robert Klieber , Dieter Suter , Stefan Kroll

We demonstrate experimentally a robust quantum memory using a magnetic-field-independent hyperfine transition in 9Be+ atomic ion qubits at a magnetic field B ~= 0.01194 T. We observe that the single physical qubit memory coherence time is…

We demonstrate the preparation and probing of the coherence between the hyperfine ground states |5S_{1/2}, F=1> and |5S_{1/2}, F=2> of the Rubidium 87 isotope. The effect of various coherence control techniques, i.e. fractional Stimulated…

Quantum Physics · Physics 2009-11-13 Martin Oberst , Frank Vewinger , A. I. Lvovsky

The hyperfine structure of the ground state of erbium doped yttrium orthosilicate is analyzed with the use of electron paramagnetic resonance experiments in a tunable microwave resonator. This work was prompted by the disagreement between…

Optically trapped ensembles are of crucial importance for frequency measurements and quantum memories, but generally suffer from strong dephasing due to inhomogeneous density and light shifts. We demonstrate a drastic increase of the…

We report on the development and application of a parametrized crystal-field model for both C$_{1}$ symmetry centers in trivalent erbium-doped Y$_{2}$SiO$_{5}$. High resolution Zeeman and temperature dependent absorption spectroscopy was…

Materials Science · Physics 2022-06-22 N. L. Jobbitt , J. -P. R. Wells , M. F. Reid , S. P. Horvath , P. Goldner , A. Ferrier

Coherent manipulation of lattice vibrations using ultrafast light pulses enables access to nonequilibrium 'hidden' phases with designed functionalities in quantum materials. However, expanding the understanding of nonlinear light-phonon…

We show that crystal-field calculations for $C_1$ point-group symmetry are possible, and that such calculations can be performed with sufficient accuracy to have substantial utility for rare-earth based quantum information applications. In…

Precision determination of the hyperfine splitting of cadmium ions is essential to study space-time variation of fundamental physical constants and isotope shifts. In this work, we present the precision frequency measurement of the…

Atomic Physics · Physics 2025-01-24 Ying Zheng , Yanmei Yu , Yiting Chen , Shengnan Miao , Wenxin Shi , Jianwei Zhang , Lijun Wang

We study the effect of an external magnetic field on coherent backscattering of light from a cool rubidium vapor. We observe that the backscattering enhancement factor can be {\it increased} with $B$. This surprising behavior shows that the…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Olivier Sigwarth , Guillaume Labeyrie , Thibaut Jonckheere , Dominique Delande , Robin Kaiser , Christian Miniatura
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