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Cooling of systems to sub-kelvin temperatures is usually done using either a cold bath of particles or spontaneous photon scattering from a laser field; in either case, cooling is driven by interaction with a well-ordered, cold (i.e. low…

Quantum Physics · Physics 2023-05-19 Amanda Younes , Wesley C. Campbell

We demonstrate millikelvin thermometry of laser cooled trapped ions with high-resolution imaging. This equilibrium approach is independent of the cooling dynamics and has lower systematic error than Doppler thermometry, with \pm5 mK…

Quantum Physics · Physics 2011-06-10 B. G. Norton , E. W. Streed , M. J. Petrasiunas , A. Jechow , D. Kielpinski

We propose the application of laser cooling to a number of transition-metal atoms, allowing numerous bosonic and fermionic atomic gases to be cooled to ultra-low temperatures. The non-zero electron orbital angular momentum of these atoms…

Atomic Physics · Physics 2020-12-03 Scott Eustice , Kayleigh Cassella , Dan Stamper-Kurn

We provide a theoretical analysis for a recently demonstrated cooling method. Two-level particles undergo successive adiabatic transfers upon interaction with counter-propagating laser beams that are repeatedly swept over the transition…

Over the past decade, tremendous progress has been made to extend the tools of laser cooling and trapping to molecules. Those same tools have recently been applied to polyatomic molecules (molecules containing three or more atoms). In this…

We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and…

Atomic Physics · Physics 2019-07-24 L. Caldwell , J. A. Devlin , H. J. Williams , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…

Chemical Physics · Physics 2018-12-04 X. Wu , T. Gantner , M. Zeppenfeld , S. Chervenkov , G. Rempe

We demonstrate rotational cooling of the silicon monoxide cation via optical pumping by a spectrally filtered broadband laser. Compared with diatomic hydrides, SiO\+ is more challenging to cool because of its smaller rotational interval.…

Most ions lack the fast, cycling transitions that are necessary for direct laser cooling. In most cases, they can still be cooled sympathetically through their Coulomb interaction with a second, coolable ion species confined in the same…

We investigate rotational state changes in a single collision of diatomic molecular ions, polar or apolar, with an atomic ion. Rotational state changes may occur since the angular degree of freedom of the molecular ions interacts with the…

Quantum Physics · Physics 2026-04-20 J. Martin Berglund , Michael Drewsen , Christiane P. Koch

A mixed system of cooled and trapped, ions and atoms, paves the way for ion assisted cold chemistry and novel many body studies. Due to the different individual trapping mechanisms, trapped atoms are significantly colder than trapped ions,…

Atomic Physics · Physics 2012-11-01 K. Ravi , Seunghyun Lee , Arijit Sharma , G. Werth , S. A. Rangwala

Sympathetic cooling with ultracold atoms and atomic ions enables ultralow temperatures in systems where direct laser or evaporative cooling is not possible. It has so far been limited to the cooling of other microscopic particles, with…

Cold molecular ions are promising candidates in various fields ranging from precision spectroscopy and test of fundamental physics to ultra-cold chemistry. Control of internal and external degrees of freedom is a prerequisite for many of…

Quantum Physics · Physics 2015-05-06 Yong Wan , Florian Gebert , Fabian Wolf , Piet O. Schmidt

High-fidelity quantum logic operations in trapped ions often require the ions' collective motion to be cooled to near the ground state. Since cooling the ions' motion typically involves dissipative processes such as spontaneous photon…

Quantum Physics · Physics 2026-05-28 Kavyashree Ranawat , Jiyong Yu , Andrew Van Horn , Jacob Whitlow , Kenneth R Brown , Jungsang Kim

We study laser cooling of atomic gases by collisional redistribution, a technique applicable to ultradense atomic ensembles at a pressure of a few hundred bar. Frequent collisions of an optically active atom with a buffer gas shift atoms…

Quantum Gases · Physics 2014-10-30 Anne Saß , Ulrich Vogl , Martin Weitz

Recently a new wave of interest to spectroscopy of radioactive compounds has raised due to successful applications of the new experimental ISOL/CRIS technique to optical spectroscopy of radium monofluoride molecules. This opens great…

Chemical Physics · Physics 2022-10-19 Timur Isaev , Dmitrii Makinski , Andrei Zaitsevski

Efficient cooling of trapped charged particles is essential to many fundamental physics experiments, to high-precision metrology, and to quantum technology. Until now, sympathetic cooling has required close-range Coulomb interactions, but…

The ability to cool single ions, atomic ensembles, and more recently macroscopic degrees of freedom down to the quantum groundstate has generated considerable progress and perspectives in Basic and Technological Science. These major…

Mesoscale and Nanoscale Physics · Physics 2016-02-17 A. Niguès , A. Siria , P. Verlot

We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we…

Quantum Physics · Physics 2015-10-02 M. Guggemos , D. Heinrich , O. A. Herrera-Sancho , R. Blatt , C. F. Roos

It is shown that the translational degrees of freedom of a large variety of molecules, from light diatomic to heavy organic ones, can be cooled sympathetically and brought to rest (crystallized) in a linear Paul trap. The method relies on…

Quantum Physics · Physics 2009-11-10 S. Schiller , C. Laemmerzahl