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We predict that it is possible to cool rotational, vibrational and translational degrees of freedom of molecules by coupling a molecular dipole transition to an optical cavity. The dynamics is numerically simulated for a realistic set of…

Quantum Physics · Physics 2007-08-13 Giovanna Morigi , Pepijn W. H. Pinkse , Markus Kowalewski , Regina de Vivie-Riedle

A general scheme for rotational cooling of diatomic heteronuclear molecules is proposed. It uses a superconducting microwave cavity to enhance the spontaneous decay via Purcell effect. Rotational cooling can be induced by sequentially…

Quantum Physics · Physics 2009-11-10 C. H. Raymond Ooi

Gas-phase multiply charged proteins have been sympathetically cooled to translational temperatures below 1 K by Coulomb interaction with laser-cooled barium ions in a linear ion trap. In one case, an ensemble of 53 cytochrome c molecules…

Atomic Physics · Physics 2008-12-01 D. Offenberg , C. B. Zhang , Ch. Wellers , B. Roth , S. Schiller

A laser cooling method for trapped atoms is described which achieves ground state cooling by exploiting quantum interference in a driven Lambda-shaped arrangement of atomic levels. The scheme is technically simpler than existing methods of…

Quantum Physics · Physics 2010-03-26 Giovanna Morigi , Juergen Eschner , Christoph H. Keitel

A novel type of particle "cooling", called Ionization Cooling, is applicable to slow (v of the order of 0.1c) ions stored in a small ring. The many traversals through a thin foil enhance the nuclear reaction probability, in a steady…

High Energy Physics - Phenomenology · Physics 2011-05-18 C. Rubbia , A. Ferrari , Y. Kadi , V. Vlachoudis

We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…

We theoretically analyze the cooling dynamics of an atom which is tightly trapped inside a high-finesse optical resonator. Cooling is achieved by suitably tailored scattering processes, in which the atomic dipole transition either scatters…

Quantum Physics · Physics 2012-11-08 Marc Bienert , Giovanna Morigi

Cooling the motion of trapped ions to near the quantum ground state is crucial for many applications in quantum information processing and quantum metrology. However, certain motional modes of trapped-ion crystals can be difficult to cool…

We propose a general method to cool the translational motion of molecules. Our method is an extension of single photon atomic cooling which was successfully implemented in our laboratory. Requiring a single event of absorption followed by a…

Chemical Physics · Physics 2015-05-13 Edvardas Narevicius , S. Travis Bannerman , Mark G. Raizen

We propose a scheme for laser cooling of negatively charged molecules. We briefly summarise the requirements for such laser cooling and we identify a number of potential candidates. A detailed computation study with C$\_2^-$, the most…

Atomic Physics · Physics 2015-06-23 Pauline Yzombard , Mehdi Hamamda , Sebastian Gerber , Michael Doser , Daniel Comparat

A lightsail can be accelerated to ultra-high speed by the radiation pressure of a laser having an intensity of the order of GW/m$^2$, which though presents a critical challenge in the thermal management of lightsails. In this letter, we…

Optics · Physics 2022-06-14 Weiliang Jin , Wei Li , Chinmay Khandekar , Meir Orenstein , Shanhui Fan

We propose a method of stimulated laser cooling of diatomic molecules by counter-propagating $\pi$-trains of ultrashort laser pulses. The cooling cycles occur on the rovibrational transitions inside the same ground electronic manifold, thus…

Atomic Physics · Physics 2015-03-13 Ekaterina Ilinova , Jonathan Weinstein , Andrei Derevianko

The trapped-ion quantum charge-coupled device (QCCD) architecture is a leading candidate for advanced quantum information processing. In current QCCD implementations, imperfect ion transport and anomalous heating can excite ion motion…

The study of cold and controlled molecular ions is pivotal for fundamental research in modern physics and chemistry. Investigations into cooling molecular anions, in particular, have proven to be of key consequence for the production of…

We propose a new method for the production of ultracold molecular ions. This method utilizes sympathetic cooling due to the strong collisions between appropriately chosen molecular ions and laser-cooled neutral atoms to realize ultracold,…

Atomic Physics · Physics 2009-11-13 Eric R. Hudson

Cooling down a trapped ion into its motional ground state is a central step for trapped ions based quantum information processing. State of the art cooling schemes often work under a set of optimal cooling conditions derived analytically…

Quantum Physics · Physics 2021-10-12 Xie-Qian Li , Shuo Zhang , Jie Zhang , Wei Wu , Chu Guo , Ping-Xing Chen

We present detailed calculations at the basis of our recent proposal for simultaneous cooling the rotational, vibrational and external molecular degrees of freedom. In this method, the molecular rovibronic states are coupled by an intense…

Quantum Physics · Physics 2007-12-10 Markus Kowalewski , Giovanna Morigi , Pepijn W. H. Pinkse , Regina de Vivie-Riedle

We study laser cooling of atomic gases by collisional redistribution of fluorescence. In a high pressure buffer gas regime, frequent collisions perturb the energy levels of alkali atoms, which allows for the absorption of a far red detuned…

We investigate laser cooling of an ensemble of atoms in an optical cavity. We demonstrate that when atomic dipoles are sychronized in the regime of steady-state superradiance, the motion of the atoms may be subject to a giant frictional…

Quantum Physics · Physics 2016-04-20 Minghui Xu , Simon B. Jäger , S. Schütz , J. Cooper , Giovanna Morigi , M. J. Holland

We present state-selected measurements of rotational cooling and excitation rates of CH$^+$ molecular ions by inelastic electron collisions. The experiments are carried out at the Cryogenic Storage Ring, making use of a monoenergetic…