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We present extensive molecular dynamics simulations of a liquid of symmetric dumbbells, for constant packing fraction, as a function of temperature and molecular elongation. For large elongations, translational and rotational degrees of…

Soft Condensed Matter · Physics 2009-11-11 Angel J. Moreno , Song-Ho Chong , Walter Kob , Francesco Sciortino

We propose a novel computational strategy to study the glass transition of molecular fluids. Our approach combines the construction of simple yet realistic models with the development of Monte Carlo algorithms to accelerate equilibration…

Statistical Mechanics · Physics 2026-03-31 Romain Simon , Jean-Louis Barrat , Ludovic Berthier

Laser cooling by collisional redistribution of radiation has been successfully applied in the past for cooling dense atomic gases. Here we report on progress of work aiming at the demonstration of redistribution laser cooling in a molecular…

Atomic Physics · Physics 2013-03-22 Philipp Simon , Peter Moroshkin , Lars Weller , Anne Sass , Martin Weitz

Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population…

We present a laser cooling scheme for trapped ions and atoms using a combination of laser couplings and a magnetic gradient field. In a Schrieffer-Wolff transformed picture, this setup cancels the carrier and blue sideband terms completely…

Quantum Physics · Physics 2011-03-18 Andreas Albrecht , Alex Retzker , Christof Wunderlich , Martin B. Plenio

In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…

Quantum Physics · Physics 2007-05-23 Christiane P. Koch , José P. Palao , Ronnie Kosloff , Françoise Masnou-Seeuws

We investigate the effect of a single heat treatment cycle on the potential energy states and mechanical properties of metallic glasses using molecular dynamics simulations. We consider the three-dimensional binary mixture, which was…

Soft Condensed Matter · Physics 2019-06-14 Nikolai V. Priezjev

We propose and experimentally demonstrate a method for laser cooling an oscillator based on sequences of spin-state-dependent displacements followed by spin repumping. For a thermal state with mean occupation $\bar{n}\gg 1$ the method…

A laser cooling scheme for trapped ions is presented which is based on the fast dynamical Stark shift gate, described in [Jonathan etal, PRA 62, 042307]. Since this cooling method does not contain an off resonant carrier transition, low…

Quantum Physics · Physics 2009-11-13 A. Retzker , M. B. Plenio

We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…

Atomic Physics · Physics 2017-09-13 Chien-Yu Lien , Scott R. Williams , Brian Odom

We show that it is possible to cool interacting pairs of atoms by a lin $\perp$ lin Sisyphus-like laser cooling scheme using counter-propagating photoassociation (PA) lasers. It is shown that the center-of-mass motion (c.m.) of atom pairs…

Atomic and Molecular Clusters · Physics 2016-09-12 Subrata Saha , Somnath Naskar , Bimalendu Deb

Analogous to the extension of laser cooling techniques from two-level to three-level atoms, Doppler cooling of molecules with an intermediate electronic state is considered. In particular, we use a rate-equation approach to simulate cooling…

Atomic Physics · Physics 2015-03-17 J. H. V. Nguyen , B. Odom

Doppler cooling is a widely used technique to laser cool atoms and nanoparticles exploiting the Doppler shift involved in translational transformations. The rotational Doppler effect arising from rotational coordinate transformations should…

Optics · Physics 2019-08-22 Deng Pan , Hongxing Xu , F. Javier García de Abajo

The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…

Laser cooling of alkali atoms typically requires time-varying magnetic fields, introducing unwanted coupling between atom preparation and coherent operations. Here we demonstrate sub-Doppler laser cooling and optical transport of alkali…

Conventional techniques for laser cooling, by coherent scattering off of internal states or through an optical cavity mode, have so far proved inefficient on mechanical oscillators heavier than a few nanograms. That is because larger…

Quantum Physics · Physics 2022-05-05 Kentaro Komori , Dominika Ďurovčíková , Vivishek Sudhir

In a recent paper, we have proposed a novel laser cooling scheme for reducing collisional energy of a pair of atoms by using photoassociative transitions. In that paper, we considered two atoms in free space, that is we have not considered…

Atomic Physics · Physics 2017-03-22 Somnath Naskar , Subrata Saha , Partha Goswami , Arpita pal , Bimalendu Deb

We develop a mathematically simple yet accurate model for the single-pulse non-resonant impulsive alignment of thermal ensembles of linear molecules. We find that our molecular alignment model not only provides a simplification for…

Optics · Physics 2023-06-08 A. Löhr , M. Ivanov , M. Khokhlova

I propose a method to remove the axial motional excitation from an ion qubit within a few oscillation periods of a harmonic trap. The principle is to prepare another coolant ion in its motional ground state, and then apply a phonon beam…

Quantum Physics · Physics 2014-12-10 Hoi-Kwan Lau

We study a single incoherently pumped atom moving within an optical high-Q resonator in the strong coupling regime. Using a semiclassical description for the atom and field dynamics, we derive a closed system of differential equations to…

Quantum Physics · Physics 2007-12-18 Thomas Salzburger , Peter Domokos , Helmut Ritsch