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A scheme is proposed for preparing delocalised mesoscopic states of the motion of two or more atoms trapped at distantly-separated locations. Generation of entanglement is achieved using interactions in cavity quantum electrodynamics which…

Quantum Physics · Physics 2007-05-23 A. S. Parkins

We propose a state-sensitive scheme to optically detect a single molecule without a closed transition, through strong coupling to a high-Q whispering-gallery mode high-Q resonator. A background-free signal can be obtained by detecting a…

Atomic Physics · Physics 2020-09-02 Ming Zhu , Yan-Cheng Wei , Chen-Lung Hung

A full density-matrix simulation is performed for optical deflection of a barium monofluoride ($^{138}$Ba$^{19}$F) beam using the bichromatic force, which employs pairs of counter-propagating laser beams that are offset in frequency. We…

Atomic Physics · Physics 2023-07-26 A. Marsman , M. Horbatsch , E. A. Hessels

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

Atomic Physics · Physics 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

The simple structure of the BH molecule makes it an excellent candidate for direct laser cooling. We measure the branching ratios for the decay of the ${\rm A}^{1}\Pi (v'=0)$ state to vibrational levels of the ground state, ${\rm…

Atomic Physics · Physics 2014-08-06 R. J. Hendricks , D. A. Holland , S. Truppe , B. E. Sauer , M. R. Tarbutt

We propose an alternative scenario for the generation of entanglement between rotational quantum states of two polar molecules. This entanglement arises from dipole-dipole interaction, and is controlled by a sequence of laser pulses…

Quantum Physics · Physics 2016-08-16 Eric Charron , Pérola Milman , Arne Keller , Osman Atabek

We demonstrate the conversion of cold Cs_{2} molecules initially distributed over several vibrational levels of the lowest triplet state a^{3}\Sigma_{u}^{+} into the singlet ground state X^{1}\Sigma_{g}^{+}. This conversion is realized by a…

Sympathetic cooling of trapped ions has been established as a powerful technique for manipulation of non-laser-coolable ions (Raizen1992,Waki1992,Bowe1999,Barrett2003). For molecular ions, it promises vastly enhanced spectroscopic…

Quantum Physics · Physics 2018-06-06 Soroosh Alighanbari , Michael Georg Hansen , Vladimir Korobov , Stephan Schiller

Confocal microscopy of fluorescent labeled particles has been used to study the dynamical and structural properties of colloidal and granular matter in real space. Localization algorithms allow for a fully automatized determination of the…

Soft Condensed Matter · Physics 2011-12-08 Marcel Roth , Michael Franzmann , Maria D'Acunzi , Max Kreiter , Günter K. Auernhammer

We establish that matter-wave interference at near-resonant ultraviolet optical gratings can be used to spatially separate individual conformers of complex molecules. Our calculations show that the conformational purity of the prepared beam…

Precise measurement of the particle number, spatial distribution and internal state is fundamental to all proposed experiments with ultracold molecules both in bulk gases and optical lattices. Here, we demonstrate in-situ detection of…

Accurate low and high-lying bound states of Tietz-Hua oscillator potential are presented. The radial Schr\"odinger equation is solved efficiently by means of the generalized pseudospectral method that enables optimal spatial discretization.…

Chemical Physics · Physics 2014-09-10 Amlan K. Roy

We present a method for the deterministic generation of all the electronic Bell states of two trapped ions. It involves the combination of a purely dispersive with a resonant laser excitation of vibronic transitions of the ions. In contrast…

Quantum Physics · Physics 2014-11-18 E. Solano , R. L. de Matos Filho , N. Zagury

The present work proposes a self-consistent reduced-order NLTE kinetic model for radiating plasmas such as are found in the outer layers of stellar atmospheres. Starting from the most up-to-date set of ab-initio and experimental data, the…

Solar and Stellar Astrophysics · Physics 2017-04-12 A. Munafo , N. Mansour , M. Panesi

We employ heterodyne interferometry to investigate the effect of a single organic molecule on the phase of a propagating laser beam. We report on the first phase-contrast images of individual molecules and demonstrate a single-molecule…

Quantum Physics · Physics 2015-05-27 M. Pototschnig , Y. Chassagneux , J. Hwang , G. Zumofen , A. Renn , V. Sandoghdar

We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…

We present a mechanism for cooling atoms by a laser beam reflected from a single mirror. The cooling relies on the dipole force and thus in principle applies to arbitrary refractive particles including atoms, molecules, or dielectric…

Quantum Physics · Physics 2009-08-05 André Xuereb , Peter Horak , Tim Freegarde

A method for specular reflection of polar molecules is proposed. Electrostatatic potentials and forces are calculated for a low-field-seeking molecule near a series of long cylindrical electrodes of radius $r$ with dc potentials of $+V$ and…

The low-temperature properties of glasses present important differences with respect to crystalline matter. In particular, models such as the Debye model of solids, which assume the existence of an underlying regular lattice, predict that…

Disordered Systems and Neural Networks · Physics 2023-01-03 Matteo Baggioli , Rico Milkus , Alessio Zaccone

We propose a theoretical scheme for coupling a nanomechanical resonator to a single diatomic molecule via microwave cavity mode of a driven LC resonator. We describe the diatomic molecule by a Morse potential and find the corresponding…

Quantum Physics · Physics 2015-03-03 M. Eghbali-Arani , Sh. Barzanjeh , H. Yavari , M. A. Shahzamanian