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In this paper, we report an experimental realization of quantum switch using nuclear spins and magnetic resonant pulses. The nuclear spins of H and C in carbon-13 labelled chloroform are used to carry the information, then nuclear magnetic…

Quantum Physics · Physics 2007-05-23 I. M. Tsai , S. Y. Kuo , S. L. Huang , Y. C. Lin , T. T. Chen

Nuclear spins interact weakly with their environment. In particular, they are generally insensitive to mechanical vibrations. Here, we successfully demonstrate the coherent coupling of mechanics to a single nuclear spin. This coupling is…

Geometric phases have been used in NMR, to implement controlled phase shift gates for quantum information processing, only in weakly coupled systems in which the individual spins can be identified as qubits. In this work, we implement…

Quantum Physics · Physics 2009-11-13 T. Gopinath , Anil Kumar

The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…

Strongly Correlated Electrons · Physics 2012-05-31 Rina Takagi , Kazuya Miyagawa , Kazushi Kanoda , Biao Zhou , Akiko Kobayashi , Hayao Kobayashi

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with…

Quantum Physics · Physics 2017-03-06 Zhen-Yu Wang , Jorge Casanova , Martin B. Plenio

The main part of this review is devoted to the comprehensive description of coherent radiation by nuclear spins. The theory of nuclear spin superradiance is developed and the experimental observations of this phenomenon are considered. The…

Statistical Mechanics · Physics 2007-05-23 V. I. Yukalov , E. P. Yukalova

We propose a mechanism for very slow coherent oscillations of current and nuclear spins in a quantum dot system, that may qualitatively explain some recent experimental observations. We concentrate on an experimentally relevant double dot…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Sigurdur I. Erlingsson , Oleg N. Jouravlev , Yuli V. Nazarov

The substitution of one metal ion in a Cr-based molecular ring with dominant antiferromagnetic couplings allows to engineer its level structure and ground-state degeneracy. Here we characterize a Cr7Ni molecular ring by means of…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 F. Troiani , A. Ghirri , M. Affronte , S. Carretta , P. Santini , G. Amoretti , S. Piligkos , G. Timco , R. E. P. Winpenny

We study the effect of contact hyperfine interaction on the nuclear spin diffusion coefficients in semiconductor quantum dots. The diffusion coefficients are calculated with both the method of moment and density matrix. We show that nuclear…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Changxue Deng , Xuedong Hu

The ability to sense and control nuclear spins near solid-state defects might enable a range of quantum technologies. Dynamically Decoupled Radio-Frequency (DDRF) control offers a high degree of design flexibility and long electron-spin…

The detection of nuclear spins using individual electron spins has enabled new opportunities in quantum sensing and quantum information processing. Proof-of-principle experiments have demonstrated atomic-scale imaging of nuclear-spin…

We experimentally demonstrate the use of a single electronic spin to measure the quantum dynamics of distant individual nuclear spins from within a surrounding spin bath. Our technique exploits coherent control of the electron spin,…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Shimon Kolkowitz , Quirin P. Unterreithmeier , Steven D. Bennett , Mikhail D. Lukin

Quantum simulators are controllable systems that can be used to simulate other quantum systems. Here we focus on the dynamics of a chain of molecular qubits with interposed antiferromagnetic dimers. We theoretically show that its dynamics…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 P. Santini , S. Carretta , F. Troiani , G. Amoretti

Theoretical study of the indirect coupling of nuclear spins (qubits) embedded into a mesoscopic ring and in a finite length quantum wire in a magnetic field is presented. It is found that the hyperfine interaction, via the conduction…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Yu. V. Pershin , I. D. Vagner , P. Wyder

Quantum computing promises to provide machine learning with computational advantages. However, noisy intermediate-scale quantum (NISQ) devices pose engineering challenges to realizing quantum machine learning (QML) advantages. Recently, a…

Quantum Physics · Physics 2022-07-22 Rodrigo Araiza Bravo , Khadijeh Najafi , Xun Gao , Susanne F. Yelin

A method of switching a controlled-NOT gate in a solid-stae NMR quantum computer is presented. Qubits of I=1/2 nuclear spins are placed periodically along a quantum spin chain (1-D antiferromagnet) having a singlet ground state with a…

Quantum Physics · Physics 2009-11-07 Atsushi Goto , Tadashi Shimizu , Kenjiro Hashi , Hideaki Kitazawa

Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the…

Quantum Physics · Physics 2015-11-25 Ashok Ajoy , Ulf Bissbort , Mikhail D. Lukin , Ronald L. Walsworth , Paola Cappellaro

Multiple quantum (MQ) NMR methods \cite{Baum} are applied to the analysis of various problems of quantum information processing. It is shown that the two-spin/two-quantum Hamiltonian \cite{Baum} describing MQ NMR dynamics is related to the…

Quantum Physics · Physics 2017-01-16 G. A. Bochkin , S. I. Doronin , S. G. Vasil'ev , A. V. Fedorova , E. B. Fel'dman

Achieving high energy resolution in spin systems is important for fundamental physics research and precision measurements, with alkali-noble-gas comagnetometers being among the best available sensors. We found a new relaxation mechanism in…

Atomic Physics · Physics 2023-02-22 Kai Wei , Tian Zhao , Xiujie Fang , Zitong Xu , Chang Liu , Qian Cao , Arne Wickenbrock , Yanhui Hu , Wei Ji , Dmitry Budker

Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…

Mesoscale and Nanoscale Physics · Physics 2026-04-10 Elia Turco , Fupeng Wu , Annika Bernhardt , Nils Krane , Ji Ma , Roman Fasel , Michal Juriček , Xinliang Feng , Pascal Ruffieux