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Nuclear magnetic resonance (NMR) spectroscopy is a powerful technique for analyzing the structure and function of molecules, and for performing three-dimensional imaging of the spin density. At the heart of NMR spectrometers is the…

Quantum Physics · Physics 2019-04-15 K. S. Cujia , J. M. Boss , K. Herb , J. Zopes , C. L. Degen

Nuclear magnetic resonance imaging (MRI) at the atomic scale offers exciting prospects for determining the structure and function of individual molecules and proteins. Quantum defects in diamond have recently emerged as a promising platform…

Quantum Physics · Physics 2022-04-06 K. S. Cujia , K. Herb , J. Zopes , J. M. Abendroth , C. L. Degen

We study the nuclear spin population in a GaAs quantum well structure and demonstrate its initialization using an all-electrical nuclear magnetic resonance (NMR) device. In our device, nuclear spins are dynamically polarized in a sub-micron…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. Ota , G. Yusa , N. Kumada , S. Miyashita , Y. Hirayama

Due to their long coherence times, nuclear spins have gained considerable attention as physical qubits. Two-qubit gates between nuclear spins of distinct resonance frequencies can be mediated by electron spins, usually employing a sequence…

Quantum Physics · Physics 2021-01-26 Benedikt Tratzmiller , Jan F. Haase , Zhenyu Wang , Martin B. Plenio

We describe a technique for quantum information processing based on localized en sembles of nuclear spins. A qubit is identified as the presence or absence of a collective excitation of a mesoscopic ensemble of nuclear spins surrounding a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. M. Taylor , G. Giedke , H. Christ , B. Paredes , J. I. Cirac , P. Zoller , M. D. Lukin , A. Imamoglu

Optically active spin defects in solids offer promising platforms to investigate nuclear spin clusters with high sensitivity and atomic-site resolution. To leverage near-surface defects for molecular structure analysis in chemical and…

The measurement of single quanta in a collection of coherently interacting objects is transformative in the investigations of emergent quantum phenomena. An isolated nuclear-spin ensemble is a remarkable platform owing to its coherence, but…

We have considered the $S=1/2$ antiferromagnetic Heisenberg model in two dimensions, with an additional Ising \nnn interaction. Antiferromagnetic \nnn interactions will lead to frustration, and the system responds with flipping the spins…

Strongly Correlated Electrons · Physics 2015-06-25 J. Hove , A. Sudbø

We demonstrate a five-bit nuclear-magnetic-resonance quantum computer that distinguishes among various functions on four bits, making use of quantum parallelism. Its construction draws on the recognition of the sufficiency of linear…

Quantum Physics · Physics 2007-05-23 R. Marx , A. F. Fahmy , J. M. Myers , W. Bermel , S. J. Glaser

Atomic comagnetometers are used in searches for anomalous spin-dependent interactions. Magnetic field gradients are one of the major sources of systematic errors in such experiments. Here we describe a comagnetometer based on the nuclear…

Atomic Physics · Physics 2018-07-18 Teng Wu , John W. Blanchard , Derek F. Jackson Kimball , Min Jiang , Dmitry Budker

The coupling between the spin degrees of freedom and macroscopic mechanical motions, including striction, shearing, and rotation, has attracted wide interest with applications in actuation, transduction, and information processing.…

Selective control of qubits in a quantum register for the purposes of quantum information processing represents a critical challenge for dense spin ensembles in solid state systems. Here we present a protocol that achieves a complete set of…

Quantum Physics · Physics 2016-09-28 J. Casanova , Z. -Y. Wang , M. B. Plenio

We introduce a method for solving the problem of an externally controlled electron spin in a quantum dot interacting with host nuclei via the hyperfine interaction. Our method accounts for generalized (non-unitary) evolution effected by…

Mesoscale and Nanoscale Physics · Physics 2011-07-21 Edwin Barnes , Sophia E. Economou

We demonstrate ionization of a molecule with the bias voltage of a Scanning Tunnelling Microscope (STM) resulting in a coexistence of a neutral and ionic molecules, i.e. radical (paramagnetic) and non-radical (diamagnetic) states. This…

Mesoscale and Nanoscale Physics · Physics 2024-04-02 Yishay Manassen , Michael Averbukh , Zion Hazan , Yahel Tzuriel , Pino Boscolo , Alexsander Shnirman , Baruch Horovitz

We propose a mechanism of long-range coherent coupling between nuclear spins to be used as qubits in solid-state semiconductor-heterojunction quantum information processing devices. The coupling is via localized donor electrons which in…

Mesoscale and Nanoscale Physics · Physics 2010-09-22 Dima Mozyrsky , Vladimir Privman , M. Lawrence Glasser

Advanced atomic magnetometers have made it possible to acquire nuclear magnetic resonance spectra in zero to ultralow magnetic fields. This regime carries the benefit of compact, low-cost instrumentation with reduced spin relaxation effects…

Quantum Physics · Physics 2026-04-10 Justin E. Elenewski , Christina M. Camara , Amir Kalev

Coherent dynamics of localized spins in semiconductors is limited by spectral diffusion arising from dipolar fluctuation of lattice nuclear spins. Here we extend the semiclassical theory of spectral diffusion for nuclear spins I=1/2 to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Rogerio de Sousa , Neil Shenvi , K. Birgitta Whaley

Spin dynamics is considered in ferromagnets consisting of electron and nuclear subsystems interacting with each other through hyperfine forces. In addition, the ferromagnetic sample is coupled with a resonance electric circuit. Under these…

Condensed Matter · Physics 2009-10-31 V. I. Yukalov , M. G. Cottam , M. R. Singh

The algebraic reformulation of molecular Quantum Electrodynamics (mQED) at finite temperatures is applied to Nuclear Magnetic Resonance (NMR) in order to provide a foundation for the reconstruction of much more detailed molecular…

Quantum Physics · Physics 2020-09-25 Kolja Them

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh