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We employ a first-principles lattice-gas Hamiltonian (LGH) approach to determine the lateral interactions between O atoms adsorbed on the Pd(100) surface. With these interactions we obtain an ordering behavior at low coverage that is in…

Materials Science · Physics 2009-11-13 Yongsheng Zhang , Volker Blum , Karsten Reuter

The hydration free energies of ions exhibit an approximately quadratic dependence on the ionic charge, as predicted by the Born model. We analyze this behavior using second-order perturbation theory. This provides effective methods to…

chem-ph · Physics 2008-02-03 Gerhard Hummer , Lawrence R. Pratt , Angel E. Garcia

The Casimir-Polder potential for interaction between an excited atom and a ground-state one in the retarded case obtained with the help of perturbation technique drops as R^-2 with the distance between the atoms [E.A. Power,…

Quantum Physics · Physics 2007-05-23 Yury Sherkunov

The Lagrangian proposed by York et al. and the covariant first order Lagrangian for General Relativity are introduced to deal with the (vacuum) gravitational field on a reference background. The two Lagrangians are compared and we show that…

General Relativity and Quantum Cosmology · Physics 2014-11-17 L. Fatibene , M. Ferraris , M. Francaviglia , M. Raiteri

The random-phase approximation with exchange (RPAE) is used with a $B$-spline basis to compute dynamic dipole polarizabilities of noble-gas atoms and several other closed-shell atoms (Be, Mg, Ca, Zn, Sr, Cd, and Ba). From these, values of…

Atomic Physics · Physics 2015-07-08 A. R. Swann , J. A. Ludlow , G. F. Gribakin

Using molecular dynamics (MD) simulations we study the interactions between elongated colloidal particles (length to breath ratio > 1) in a nematic host. The simulation results are compared to the results of a Landau-de Gennes elastic free…

Soft Condensed Matter · Physics 2009-11-10 D. Andrienko , M. Tasinkevych , P. Patricio , M. P. Allen , M. M. Telo da Gama

Variational and perturbative relativistic energies are computed and compared for two-electron atoms and molecules with low nuclear charge numbers. In general, good agreement of the two approaches is observed. Remaining deviations can be…

Chemical Physics · Physics 2022-09-21 Dávid Ferenc , Péter Jeszenszki , Edit Mátyus

The onset of retardation effects in atom-wall interactions is studied. It is shown that the transition range from the 1/z^3 short-range (van der Waals) interaction to the 1/z^4 long-range (Casimir) retarded interaction critically depends on…

Other Condensed Matter · Physics 2024-03-18 T. Das , C. A. Ullrich , U. D. Jentschura

Strong correlations between equilibrium fluctuations of the configurational parts of pressure and energy are found in the Lennard-Jones liquid and other simple liquids, but not in hydrogen-bonding liquids like methanol and water. The…

Statistical Mechanics · Physics 2009-11-13 Ulf R. Pedersen , Nicholas Bailey , Thomas B. Schrøder , Jeppe C. Dyre

We study A-B reaction kinetics at a fixed interface separating A and B bulks. Initially, the number of reactions ${\cal R}_t \sim t n_A^\infty n_B^\infty$ is 2nd order in the far-field densities $n_A^\infty,n_B^\infty$. First order…

Soft Condensed Matter · Physics 2009-10-31 Ben O'Shaughnessy , Dimitrios Vavylonis

The neglected quantum effect On CuO2 plane--the transition of electron between neighbored ions is studied. To study this affection, an ideal square lattice composed of triangle unit is proposed and studied. Every unit in the square lattice…

Superconductivity · Physics 2013-08-14 Dong Hang

Path-integral molecular dynamics simulations based on density functional theory employing exchange-correlation density functionals capable of treating nonlocal van der Waals (vdW) interactions self-consistently provide a remarkably accurate…

Chemical Physics · Physics 2014-02-13 Jeffrey M. McMahon , Miguel A. Morales , Brian Kolb , Timo Thonhauser

We employ {\it{ab-initio}} calculations to investigate the charge density waves in single-layer NbSe$_2$, and we explore how they are affected by transition metal atoms. Our calculations reproduce the observed orthorhombic phase in…

This work addresses non-classically damped coupled oscillators with closely spaced modes focusing on the physics of modal interactions. Considering the simplest representative example in the form of an impulsively excited…

First principles phase diagram calculations, that included van der Waals interactions, were performed for the bulk transition metal dichalcogenide system $(1-X) \cdot WS_{2} - (X) \cdot WTe_{2}$. To obtain a converged phase diagram, a…

Materials Science · Physics 2017-12-01 B. P. Burton

The accurate treatment of long-range energy terms such as van der Waals interactions is crucial for reliable free energy calculations in molecular simulations. Methods like force switching, potential switching, potential shifting, and Ewald…

Chemical Physics · Physics 2025-04-21 Lindsey M. Whitmore , Yalda Ramezani , Sumit Sharma , Michael R. Shirts

We consider the the van der Waals force involving excited atoms in general environments, constituted by magnetodielectric bodies. We develop a dynamical approach studying the dynamics of the atoms and the field, mutually coupled. When only…

Quantum Physics · Physics 2017-02-24 Pablo Barcellona , Roberto Passante , Lucia Rizzuto , Stefan Yoshi Buhmann

The quantum electrodynamics formalism to treat the interelectronic-interaction correction of first order in $1/Z$ to the two-electron part of the nuclear recoil effect on binding energies in atoms and ions is developed. The nonperturbative…

Atomic Physics · Physics 2019-07-24 A. V. Malyshev , I. S. Anisimova , D. V. Mironova , V. M. Shabaev , G. Plunien

An influence of the repulsive interactions on matter properties is considered within the excluded volume van der Waals hadron-resonance gas model. Quantitative results are presented for matter at the chemical freeze-out in central…

Nuclear Theory · Physics 2013-08-28 V. V. Begun , M. Gaździcki , M. I. Gorenstein

The electrostatic interaction between an excited atom and a diatomic ground state molecule in an arbitrary rovibrational level at large mutual separations is investigated with a general second-order perturbation theory, in the perspective…

Quantum Physics · Physics 2017-04-11 M. Lepers , R. Vexiau , N. Bouloufa , O. Dulieu , V. Kokoouline
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