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Related papers: Variational calculations on the hydrogen molecular…

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The main motivation for this work is the exploration of rotational-vibrational states corresponding to electronic excitations in a pre-Born-Oppenheimer quantum theory of molecules. These states are often embedded in the continuum of the…

Chemical Physics · Physics 2018-10-15 Edit Mátyus

Potential energy curves and matrix elements of radial non-adiabatic couplings of 2{\Sigma}+ and 2{\Pi} states of the NeH molecule are calculated using the electronic structure package MOLPRO, in view of the study of the reactive collisions…

Instrumentation and Methods for Astrophysics · Physics 2025-01-31 R. Hassaine , D. Talbi , R. P. Brady , J. Zs. Mezei , J. Tennyson , and Ioan F. Schneider

The energies of the lowest $^2P_u$, $^4P_g$ and $2D_g$ states of the boron atom are calculated with $\mu$hartree accuracy, in the basis of symmetrized, explicitly correlated Gaussian lobe functions. Finite nuclear mass and scalar…

Chemical Physics · Physics 2020-11-18 Krzysztof Strasburger

In this paper we report calculations of potential energy curves in the $1.2 a.u.\le R\le100 a.u.$ range at Multireference Configuration Interaction (MRCI) level for doubly excited states of the H$_2$ molecule. We have focused on the $Q_2$…

A basis set of generalized nonspherical Gaussian functions (GGTOs) is presented and discussed. As a first example we report on Born-Oppenheimer energies of the hydrogen molecule. Although accurate results have been obtained, we conclude…

Chemical Physics · Physics 2009-10-31 T. Detmer , P. Schmelcher , L. S. Cederbaum

We report \textit{ab initio} calculations of the X $^2 \Sigma_{u}^+$, A $^2\Pi_u$ and B $^2 \Sigma_{g}^+$ states of the Ca$_{2}^+$ dimer. All electron CAS+MRCI calculations are performed for the X $^2 \Sigma_{u}^+$ and B $^2 \Sigma_{g}^+$…

Chemical Physics · Physics 2015-06-05 Sandipan Banerjee , John A. Montgomery , Jason N. Byrd , H. Harvey Michels , Robin Côté

A variational calculation of the energy levels of a class of PT-invariant quantum mechanical models described by the non-Hermitian Hamiltonian H= p^2 - (ix)^N with N positive and x complex is presented. Excellent agreement is obtained for…

Quantum Physics · Physics 2009-10-31 Carl Bender , Fred Cooper , Peter Meisinger , Van M. Savage

Using the effective rotational Hamiltonian method, we have conducted an analysis of the D218O ground and the first excited vibration state rotational energy levels. The analysis was based on the effective Hamiltonians represented in several…

Chemical Physics · Physics 2021-01-18 I. A. Vasilenko , O. V. Naumenko , E. R. Polovtseva , A. D. Bykov

Our previous studies of dissociative recombination, and vibrational excitation/de-excitation of the BeH$^+$ ion, based on the multichannel quantum defect theory, are extended to collision energies above the dissociation threshold, taking…

The simplest molecules in nature, molecular hydrogen ions in the form of H2+ and HD+, provide an important benchmark system for tests of quantum electrodynamics in complex forms of matter. Here, we report on such a test based on a frequency…

Atomic Physics · Physics 2016-02-03 J. Biesheuvel , J. -Ph. Karr , L. Hilico , K. S. E. Eikema , W. Ubachs , J. C. J. Koelemeij

In this work we report the results concerning calculations for quantum-mechanical rotational transitions in molecular hydrogen, H$_2$, induced by an ultra-cold ground state anti-hydrogen atom $\bar{H}_{1s}$. The calculations are…

Atomic Physics · Physics 2015-05-14 Renat A. Sultanov , Sadhan K. Adhikari , Dennis Guster

The article presents calculated dissociative recombination (DR) rate coefficients for H+3 . The previous theoretical work on H+3 was performed using the adiabatic hyperspherical approximation to calculate the target ion vibrational states…

Atomic Physics · Physics 2007-08-22 Samantha Fonseca dos Santos , Viatcheslav Kokoouline , Chris H. Greene

The translational motion of molecular ions can be effectively cooled sympathetically to translational temperatures below 100 mK in ion traps through Coulomb interactions with laser-cooled atomic ions. The ro-vibrational degrees of freedom,…

Atomic Physics · Physics 2009-11-10 I. S. Vogelius , L. B. Madsen , M. Drewsen

Recently we reported a high precision optical frequency measurement of the (v,L):(0,2)->(8,3) vibrational overtone transition in trapped deuterated molecular hydrogen (HD+) ions at 10 mK temperature. Achieving a resolution of 0.85…

Atomic Physics · Physics 2017-02-20 J. Biesheuvel , J. -Ph. Karr , L. Hilico , K. S. E. Eikema , W. Ubachs , J. C. J. Koelemeij

Heavy polar molecules offer a great sensitivity to the electron Electric Dipole Moment(EDM). To guide emerging searches for EDMs with molecular ions, we estimate the EDM-induced energy corrections for hydrogen halide ions $\mathrm{HBr}^{+}$…

High Energy Physics - Experiment · Physics 2011-08-11 Boris Ravaine , Sergey G. Porsev , Andrei Derevianko

The mass corrections to the bound state energies of the three-body muonic molecular ions $pp\mu, pd\mu, pt\mu, dd\mu, dt\mu$ and $tt\mu$ are determined numerically from the results of highly accurate computations. The total energies and…

Atomic Physics · Physics 2015-06-03 Alexei M. Frolov

The ground state energy of hydrogen molecular ion H2+ confined by a hard prolate spheroidal cavity is calculated. The case in which the nuclear positions are clamped at the foci is considered. Our calculations are based on using the…

Atomic and Molecular Clusters · Physics 2016-05-25 S. B. Doma , F. N. El-Gammal , A. A. Amer

A procedure for calculation of rotation-vibration states of medium sized molecules is presented. It combines the advantages of variational calculations and perturbation theory. The vibrational problem is solved by diagonalizing a…

Chemical Physics · Physics 2015-04-13 A. I. Pavlyuchko , S. N. Yurchenko , Jonathan Tennyson

We investigated transition strengths from ultracold weakly bound 41K87Rb molecules produced via the photoassociation of laser-cooled atoms. An accurate potential energy curve of the excited state (3)1Sigma+ was constructed by carrying out…

Atomic Physics · Physics 2015-05-20 K. Aikawa , D. Akamatsu , M. Hayashi , J. Kobayashi , M. Ueda , S. Inouye

The electronic structure of the hydrogen molecule is investigated for the parallel configuration. The ground states of the Sigma manifold are studied for ungerade and gerade parity as well as singlet and triplet states covering a broad…

Chemical Physics · Physics 2009-10-30 T. Detmer , P. Schmelcher , F. K. Diakonos , L. S. Cederbaum