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We present ab initio perturbed ion calculations on the structures and relative stabilities of doubly charged [(NaCl)_m(Na)_2]2+ cluster ions. The obtained stabilities show excellent agreement with experimental abundances obtained from mass…

Atomic and Molecular Clusters · Physics 2007-05-23 Andres Aguado

In this paper we show that 1-electron properties such as Compton profiles and structure factors of crystals can be asymptotically retrieved through cluster-based calculations, followed by an appropriate partition of the 1-electron reduced…

Chemical Physics · Physics 2015-06-26 Sebastien Ragot , Jean-Michel Gillet , Pierre J Becker

We investigate noncollinear effects in antiferromagnetically coupled clusters using the general, rotationally invariant form of local spin-density theory. The coupling to the electronic degrees of freedom is treated with relativistic…

Atomic and Molecular Clusters · Physics 2009-10-31 C. Kohl , G. F. Bertsch

Finite magnesium oxide nanotubes are investigated. Stacks of four parallel squares, hexagons, octagons, and decagons are constructed and studied by the pseudopotential density functional theory within the local-density approximation.…

Materials Science · Physics 2009-11-10 G. Bilalbegovic

Context Mixed-metal clusters have long been studied because of their peculiar properties and how they change with cluster size, composition and charge state and their potential roles in catalysis. The characterization of these clusters is…

Chemical Physics · Physics 2024-04-30 Paulo H. Acioli

The analytic properties of Nilsson's Modified Oscillator (MO), which was first introduced in nuclear structure, and of the recently introduced, based on quantum algebraic techniques, 3-dimensional q-deformed harmonic oscillator (3-dim q-HO)…

Condensed Matter · Physics 2009-11-07 Dennis Bonatsos , D. Lenis , P. P. Raychev , P. A. Terziev

Extensive first-principle calculations on embedded clusters containing few O, Y, Ti, and Cr atoms as well as vacancies are performed to obtain interaction parameters to be applied in Metropolis Monte Carlo simulations, within the framework…

Materials Science · Physics 2014-11-05 M. Posselt , D. Murali , B. K. Panigrahi

Density functional and quantum Monte Carlo calculations challenge the existence of a unique ground state structure for certain Si clusters. For Si clusters with more than a dozen atoms the lowest ten isomers are close in energy and for some…

Materials Science · Physics 2009-11-11 W. Hellmann , R. Hennig , S. Goedecker , C. Umrigar , B. Delley , T. Lenosky

We have investigated the crystal, electronic, and magnetic structure of Mn5O8 by means of state of-the-art density functional theory calculations and neutron powder diffraction (NPD) measurements. This compound stabilizes in the monoclinic…

Materials Science · Physics 2016-09-12 M. R. Ashwin Kishore , H. Okamoto , Lokanath Patra , R. Vidya , Anja O. Sjastad , H. Fjellvag , P. Ravindran

In this work we have applied the recently formulated self-compressed inhomogeneous stabilized jellium model [M. Payami and T. Mahmoodi, Can. J. Phys. {\bf 89}, 967 (2011)] to describe the equilibrium electronic and geometric properties of…

Materials Science · Physics 2017-09-22 M. Payami , T. Mahmoodi

We investigate the properties of clusters formed from two connected $\mathrm{Ge_{m}}$ cage-like clusters, such as experimentally synthesized $\mathrm{Au_3Ge_{18}^{5-}}$, using first-principles DFT methods. We focus particularly on…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 Danielle McDermott , Kathie E. Newman

Ionization potentials, excitation energies, transition properties, and hyperfine structure constants of the low-lying $3p^6 3d^{9} \ ^2D_{5/2}$, $3p^6 3d^{9} \ ^2D_{3/2}$, $3p^5 3d^{10} \ ^2P_{3/2}$ and $3p^5 3d^{10} \ ^2P_{1/2}$ atomic…

Atomic Physics · Physics 2021-12-01 Dillip K. Nandy , B. K. Sahoo

The equilibrium structure and exchange constants of CaMnO$_3$ and LaMnO$_3$ have been investigated using total energy unrestricted Hartree-Fock (UHF) and localised orbital configuration interaction (CI) calculations on the bulk compounds…

Strongly Correlated Electrons · Physics 2009-11-07 M. Nicastro , C. H. Patterson

We present a detailed theoretical investigation on the magnetic properties of small single-layered Fe, Co and Ni clusters deposited on Ir(111), Pt(111) and Au(111). For this a fully relativistic {\em ab-initio} scheme based on density…

Materials Science · Physics 2015-06-04 S. Bornemann , O. Šipr , S. Mankovsky , S. Polesya , J. B. Staunton , W. Wurth , H. Ebert , J. Minár

First-principles, density-functional based electronic structure calculations are carried out for MgC(Ni_{1-x}Co_{x})_{3} alloys over the concentration range 0\leq x\leq1, using Korringa-Kohn-Rostoker coherent-potential approximation (KKR…

Materials Science · Physics 2009-11-11 P. Jiji Thomas Joseph , Prabhakar P. Singh

X-ray observations of galaxy clusters reveal a large range of morphologies with various degrees of disturbance, showing that the assumptions of hydrostatic equilibrium and spherical shape which are used to determine the cluster mass from…

Cosmology and Nongalactic Astrophysics · Physics 2012-12-11 A. Weißmann , H. Böhringer , R. Suhada , S. Ameglio

The chemical flexibility of metal-organic frameworks (MOFs) offers an ideal platform to tune structure and composition for specific applications, from gas sensing to catalysis and from photoelectric conversion to energy storage. This…

Materials Science · Physics 2024-02-13 Joshua Edzards , Holger-Dietrich Saßnick , Julia Santana Andreo , Caterina Cocchi

We systematically investigate the structural, electronic and magnetic properties of Mn$_n$ clusters ($n =$ 2$-$20) within the {\it ab-initio} pseudopotential plane wave method using generalized gradient approximation for the…

Atomic and Molecular Clusters · Physics 2008-06-12 Mukul Kabir , Abhijit Mookerjee , D. G. Kanhere

We present a comprehensive density functional theory (DFT) study of Mo-doped silver clusters Ag$_n$Mo ($n=1$-14), focusing on their structural, electronic, and bonding properties. Global optimization reveals an evolution from planar and…

Materials Science · Physics 2025-09-04 Samantha Ortega-Flores , Peter Ludwig Rodríguez-Kessler

Nuclei at both the neutron- and proton-drip lines are studied. In the cluster-core model, the halo-structure of all the observed and proposed cases of neutron- or proton-halos is investigated in terms of simple potential energy surfaces…

Nuclear Theory · Physics 2011-11-09 Raj K. Gupta , Sushil Kumar , M. Balasubramaniam , G. Munzenberg , Werner Scheid