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High-order harmonic generation (HHG) from atoms is a coherent light source that opens up attosecond physics, but it is the application of HHG to solids that brings much of excitement for the last decade. Here we report a completely new kind…

Materials Science · Physics 2019-08-28 G. P. Zhang , Y. H. Bai

Integrated waveguides exhibiting efficient second-order nonlinearities are crucial to obtain compact and low power optical signal processing devices. Silicon nitride (SiN) has shown second harmonic generation (SHG) capabilities in resonant…

A theoretical optimization method of high-harmonic-generation (HHG) is developed in the framework of optimal-control-theory (OCT). The target of optimization is the emission radiation of a particular frequency. The OCT formulation includes…

Quantum Physics · Physics 2020-02-19 Ido Schaefer , Ronnie Kosloff

We demonstrate that high-harmonic generation (HHG) in solids dominantly originates from strongly localized surface states through non-perturbative processes. Measurements reveal that HHG from bulk states is suppressed by at least 1-2 orders…

Optics · Physics 2018-05-02 J. Seres , E. Seres , C. Serrat , T. Schumm

We investigate harmonic generation (HG) from ground-state Ar+ aligned with M=1 at a laser wavelength of 390-nm and intensity of 4x10(14) Wcm-2. Using time-dependent R-matrix theory, we find that an initial state with magnetic quantum number…

Atomic Physics · Physics 2013-10-01 A. C. Brown , Hugo W. van der Hart

High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Joel D. Cox , Andrea Marini , F. Javier García de Abajo

An effective self-consistent model is derived and used to study the dynamics of an electron gas confined in a nonparabolic and anisotropic quantum well. This approach is based on the equations of quantum hydrodynamics, which incorporate…

Mesoscale and Nanoscale Physics · Physics 2016-05-11 Jerome Hurst , Kevin Leveque-Simon , Paul-Antoine Hervieux , Giovanni Manfredi , Fernando Haas

A manifestation of electron-hole pairing in nonlinear electromagnetic response of a double layer graphene system is studied. It is shown that the pairing causes the appearance of a number of peaks in the frequency dependence of the…

Strongly Correlated Electrons · Physics 2017-10-20 K. V. Germash , D. V. Fil

We experimentally observe longer than long trajectory influence in high order harmonic generation (HHG) by varying the peak intensity of the driving laser field through either direct attenuation, or by chirping the laser pulse. Using a…

When a continuous symmetry of a physical system is spontaneously broken, two types of collective modes typically emerge: the amplitude and phase modes of the order-parameter fluctuation. For superconductors, the amplitude mode is recently…

Superconductivity · Physics 2020-03-19 Ryo Shimano , Naoto Tsuji

We investigate enhanced harmonic generation processes in gain-assisted, near-zero permittivity metamaterials composed of spherical plasmonic nanoshells. We report the presence of narrow-band features in transmission, reflection and…

Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…

High harmonic generation (HHG) takes place in all phases of matter. In gaseous atomic and molecular media, it has been extensively studied and is very well-understood. In solids research is ongoing, but a consensus is forming for the…

Chemical Physics · Physics 2022-06-22 Ofer Neufeld , Zahra Nourbakhsh , Nicolas Tancogne-Dejean , Angel Rubio

From the famous classical "simple man" model to the recent multichannel model for polyatomic molecules, this tutorial will guide you through the several landmarks in our understanding of high harmonic generation and high harmonic…

Atomic Physics · Physics 2013-04-10 Olga Smirnova , Misha Ivanov

Using a high-frequency field superposed to a linearly polarized bichromatic laser field composed by a wave with frequency $\omega $ and a wave with frequency $2\omega $, we show it is possible to enhance the intensity of a group of high…

Atomic Physics · Physics 2009-11-06 C. Figueira de Morisson Faria , M. L. Du

Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…

Optics · Physics 2013-09-17 B. U. Felderhof , G. Marowsky

High-gain optical parametric amplification is an important nonlinear process used both as a source of coherent infrared light and as a source of nonclassical light. In this work, we experimentally demonstrate an approach to optical…

High-quality crystals without inversion symmetry are the conventional platform to achieve optical frequency conversion via three wave-mixing. In bulk crystals, efficient wave-mixing relies on phase-matching configurations, while at the…

We use a hybrid strategy to obtain anharmonic frequency shifts and lifetimes of phonon quasi-particles from first principles molecular dynamics simulations in modest size supercells. This approach is effective irrespective of crystal…

Materials Science · Physics 2015-06-18 Dong-Bo Zhang , Tao Sun , Renata M. Wentzcovitch

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets