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Recent improvements in experimental techniques for preparing ultracold molecules that contain alkali atoms (e.g., Li, Na, and K) have been reported. Based on these advances in ultracold molecules, new searches for the electric dipole moment…

Atomic Physics · Physics 2020-01-08 A. Sunaga , M. Abe , V. S. Prasannaa , T. Aoki , M. Hada

Parity- and time-reversal-symmetry violating interaction constants required for the interpretation of a recent measurement (arXiv:1704.07928 [physics.atom-ph]) of corresponding symmetry violations in the $\Omega=1$ (${^3\Delta}_1$) science…

Atomic Physics · Physics 2017-10-18 Timo Fleig

It has been shown that the crystal-field interactions can produce a non- magnetic singlet ground state for the highly-correlated d6 system situated in the quasi-octahedral crystal field (CEF) surrounding provided the spin-orbit interactions…

Strongly Correlated Electrons · Physics 2009-10-31 R. J. Radwanski , Z. Ropka

The best upper limit for the electron electric dipole moment was recently set by the ACME collaboration. This experiment measures an electron spin-precession in a cold beam of ThO molecules in their metastable $H~(^3\Delta_1)$ state.…

We report on the results of a search for the electron electric dipole moment $d_e$ using paramagnetic ferroelectric Eu$_{0.5}$Ba$_{0.5}$TiO$_3$. The electric polarization creates an effective electric field that makes it energetically…

Atomic Physics · Physics 2012-11-28 S. Eckel , A. O. Sushkov , S. K. Lamoreaux

The Electric Dipole Moment of the electron (eEDM) is typically investigated in experiments using paramagnetic molecules. However, the physical observable in these searches consists in a linear combination of CP-violating interactions,…

High Energy Physics - Phenomenology · Physics 2025-03-31 Marco Ardu , Nicola Valori

The a(1) state of PbO can be used to measure the electric dipole moment of the electron d_e. We discuss a semiempirical model for this state, which yields an estimate of the effective electric field on the valence electrons in PbO. Our…

Atomic Physics · Physics 2007-05-23 M. G. Kozlov , D. DeMille

The electronic structures of element cerium under high pressure remain unclear all the time. We tried to calculate the electronic structures of $\alpha'$, $\alpha"$, and $\epsilon$-Ce which only exist in the presence of pressure, by using…

Strongly Correlated Electrons · Physics 2018-11-02 Haiyan Lu , Li Huang

Heavy polar diatomic molecules are the primary tools for searching for the T-violating permanent electric dipole moment of the electron (eEDM). Valence electrons in some molecules experience extremely large effective electric fields due to…

Atomic Physics · Physics 2015-06-11 V. S. Prasannaa , A. C. Vutha , M. Abe , B. P. Das

The NL-eEDM collaboration is building an experimental setup to search for the permanent electric dipole moment of the electron in a slow beam of cold barium fluoride molecules [Eur. Phys. J. D, 72, 197 (2018)]. Knowledge of molecular…

The ACME collaboration has recently reported a new bound on the electric dipole moment (EDM) of the electron, $|d_e|< 1.1 \times 10^{-29}\, {\rm e\cdot cm}$ at 90$\%$ confidence level, reaching an unprecedented accuracy level. This can…

High Energy Physics - Phenomenology · Physics 2021-11-05 Giuliano Panico , Alex Pomarol , Marc Riembau

An accurate determination of the effective electric field (Eeff) in YbF is important, as it can be combined with the results of future experiments to give an improved new limit for the electric dipole moment of the electron. We report a…

Atomic Physics · Physics 2015-06-19 M. Abe , G. Gopakumar , M. Hada , B. P. Das , H. Tatewaki , D. Mukherjee

To describe excited states, the electron density alone being insufficient, we use the noninteracting reference density matrix $\gamma_{s}({\bf x},{\bf x}')$ based on the recently established foundation for the $\Delta SCF$ theory, in which…

Chemical Physics · Physics 2024-08-20 Weitao Yang , Yichen Fan

Electric field gradients (EFG's) were calculated for the $CeIn_3$ compound at both $^{115}In$ and $^{140}Ce$ sites. The calculations were performed within the density functional theory (DFT) using the augmented plane waves plus local…

Strongly Correlated Electrons · Physics 2009-11-13 S. Jalali Asadabadi

This paper describes the results of the most recent measurement of the permanent electric dipole moment (EDM) of neutral $^{199}$Hg atoms. Fused silica vapor cells containing enriched $^{199}$Hg are arranged in a stack in a common magnetic…

Atomic Physics · Physics 2017-08-21 B. Graner , Y. Chen , E. G. Lindahl , B. R. Heckel

We investigate an extension of excited state mean-field theory in which the energy expression is augmented with density functional components in an effort to include the effects of weak electron correlations. The approach remains…

Chemical Physics · Physics 2020-02-05 Luning Zhao , Eric Neuscamman

Ensemble density functional theory (EDFT) is a promising alternative to time-dependent density functional theory for computing electronic excitation energies. Using coordinate scaling, we prove several fundamental exact conditions in EDFT…

Strongly Correlated Electrons · Physics 2023-07-04 Thais R. Scott , John Kozlowski , Steven Crisostomo , Aurora Pribram-Jones , Kieron Burke

In order to realize more sensitive eEDM measurement, it would be worthwhile to find some new laser-cooled molecules with larger internal effective electric field (E$_{eff}$), higher electric polarizability and longer lifetime of the eEDM…

Atomic Physics · Physics 2019-03-13 Zhenghai Yang , Jing Li , Qinning Lin , Liang Xu , Hailing Wang , Tao Yang , Jianping Yin

Several new aspects of the subtle interplay between electronic correlations and disorder are reviewed. First, the dynamical mean-field theory (DMFT)together with the geometrically averaged ("typical") local density of states is employed to…

Strongly Correlated Electrons · Physics 2015-05-18 K. Byczuk , W. Hofstetter , U. Yu , D. Vollhardt

We have completed a new precision measurement of the electron's electric dipole moment using trapped HfF$^+$ in rotating bias fields. We report on the accuracy evaluation of this measurement, describing the mechanisms behind our systematic…