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We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

Monolayers of transition metal dichacogenides show strong second-order nonlinearity and symmetry-driven selection rules from their three-fold lattice symmetry. This process resembles the valley-contrasting selection rules for…

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…

We report on the experimental and theoretical investigation of magnetic-field-induced second harmonic generation (SHG) and two-photon absorption (TPA) of excited exciton states ($n \geq 3$) of the yellow series in Cu$_2$O. In this…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 A. Farenbruch , J. Mund , D. Fröhlich , D. R. Yakovlev , M. Bayer , M. A. Semina , M. M. Glazov

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…

Second-harmonic generation (SHG) is a fundamental tool in modern laser technology, enabling coherent frequency conversion to remote optical bands, serving as the basis for self-referenced femtosecond lasers and quadrature-squeezed light…

Optics · Physics 2025-12-10 Nikolai Kuznetsov , Zihan Li , Tobias J. Kippenberg

High harmonic generation (HHG) in solids could enable attosecond and ultraviolet light sources with high compactness, great controllability and rich functions. However, the HHG process is accompanied by a quite large wavevector mismatch…

LMTO calculations are presented for the frequency dependent second harmonic generation (SHG) in the polytypes 2H, 4H, 6H, 15R and 3C of SiC. All independent tensor components are calculated. The spectral features and the ratios of the 333…

Condensed Matter · Physics 2009-10-30 Sergey N. Rashkeev , Walter R. L. Lambrecht , Benjamin Segall

High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

High harmonic generation (HHG) in solids results from an interplay between intraband acceleration and electron-hole recombination driven by a high-intensity laser pulse. Here, we theoretically reveal that the driving pulse duration can play…

Optics · Physics 2026-03-06 Alba de las Heras , Ofer Neufeld , Angel Rubio

Nonlinear topological photonics, which explores topics common to the fields of topological phases and nonlinear optics, is expected to open up a new paradigm in topological photonics. Here, we demonstrate second-harmonic generation (SHG)…

Optics · Physics 2021-04-28 Zhihao Lan , Jian Wei You , Qun Ren , Wei E. I. Sha , Nicolae C. Panoiu

The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…

Second harmonic generation (SHG) extensively employs periodically poled nonlinear crystals through forward quasi-phase-matching to achieve efficient frequency conversion. As poling periods approach sub-micrometers, backward…

Optics · Physics 2024-07-15 Fengyan Yang , Juanjuan Lu , Mohan Shen , Guangcanlan Yang , Hong X. Tang

We investigate second harmonic generation (SHG) from hexagonal periodic arrays of triangular nano-holes of aluminum using a self-consistent methodology based on the hydrodynamics-Maxwell-Bloch approach. It is shown that angular polarization…

Optics · Physics 2021-07-07 Maxim Sukharev , Adi Salomon , Joseph Zyss

Second harmonic generation (SHG) on the pyrochlore metal Cd2Re2O7 indicates the presence of three order parameters setting in below an inversion breaking transition. Here, we explore a possible structural explanation and relate it not only…

Strongly Correlated Electrons · Physics 2020-01-15 M. R. Norman

Second-order nonlinearity gives rise to many distinctive physical phenomena, e.g., second-harmonic generation, which plays an important role in fundamental science and various applications. Lithium niobate, one of the most widely used…

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

The in-plane anisotropic properties of two-dimensional (2D) group IV monochalcogenides provide an additional degree of freedom which can be used in future optoelectronic devices. Here, it is shown that the third harmonic generation (THG)…