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We propose an alternative to the usual time--independent Born--Oppenheimer approximation that is specifically designed to describe molecules with non--symmetrical hydrogen bonds. In our approach, the masses of the hydrogen nuclei are scaled…

Mathematical Physics · Physics 2009-11-13 George A. Hagedorn , Alain Joye

The analytic Born-Oppenheimer (B-O) potential curve for the ground state $X^1\Sigma^+$ of the molecule (H,D,T)Cl is constructed for the whole range of internuclear distances $R \in [0,\infty)$ with an accuracy of 3-5 figures in comparison…

Chemical Physics · Physics 2023-08-15 Horacio Olivares-Pilón , Alexander V. Turbiner

We study the ground state properties of a quasi one dimensional electron gas, interacting via an effective potential with a harmonic transversal confinement and long range Coulomb tail. The exact correlation energy has been calculated for a…

Strongly Correlated Electrons · Physics 2013-05-29 Michele Casula , Sandro Sorella , Gaetano Senatore

Analytical formulas for the excitation energies as well as for the electric quadrupole reduced transition probabilities in the ground, beta and gamma bands were derived within the coherent state model for the near vibrational and well…

Nuclear Theory · Physics 2015-05-30 A. A. Raduta , R. Budaca , Amand Faessler

We show, in several important and general cases, that a low variational energy density of a trial state is possible even when the trial state represents a different phase from the ground state. Specifically, we ask whether the ground state…

Strongly Correlated Electrons · Physics 2015-06-22 Leon Balents

A simple method of variational calculations of the electronic structure of a two-electron atom/ion, primarily near the nucleus, is proposed. The method as a whole consists of a standard solution of a generalized matrix eigenvalue equation,…

Atomic Physics · Physics 2024-10-08 Evgeny Z. Liverts

A system of N interacting bosons or fermions in a two-dimensional harmonic potential (or, equivalently, magnetic field) whose states are projected onto the lowest Landau level is considered. Generic expressions are derived for matrix…

Mesoscale and Nanoscale Physics · Physics 2011-12-12 Stefan Mashkevich , Sergey Matveenko , Stéphane Ouvry

A new electronic structure model is developed in which the ground state energy of a molecular system is given by a Hartree-Fock-like expression with parametrized one- and two-electron integrals over an extended (minimal + polarization) set…

Chemical Physics · Physics 2014-02-11 Dimitri N. Laikov

Electron-electron correlation forms the basis of difficulties encountered in many-body physics. Accurate treatment of the correlation problem is likely to unravel some nice physical properties of matter embedded in the correlation. In an…

Atomic Physics · Physics 2021-03-17 E. Jobunga

The ground state energy of a system of electrons and nuclei is proven to be a variational functional of the conditional electronic density $n_R(\mathbf{r})$, the nuclear wavefunction $\chi(R)$ and an induced vector potential $A_{\mu}(R)$…

Chemical Physics · Physics 2016-11-08 Ryan Requist , E. K. U. Gross

We consider asymptotics of the ground state energy of heavy atoms and molecules in the self-generatedl magnetic field. Namely, we consider $$ H=((D-A)\cdot\boldsymbol{\sigma})^2-V $$ with $$V=\sum_{1\le m\le M} \frac{Z_m}{|x-y_m|}$$ and a…

Mathematical Physics · Physics 2014-01-03 Victor Ivrii

Accurate $EF{}^1\Sigma^+_g-X{}^1\Sigma^+_g$ transition energies in molecular hydrogen were determined for transitions originating from levels with highly-excited vibrational quantum number, $v=11$, in the ground electronic state.…

Atomic Physics · Physics 2016-09-23 T. Madhu Trivikram , M. L. Niu , P. Wcisło , W. Ubachs , E. J. Salumbides

The leading terms in the large-$R$ asymptotics of the functional of the one-electron reduced density matrix for the ground-state energy of the H$_2$ molecule with the internuclear separation $R$ is derived thanks to the solution of the…

Chemical Physics · Physics 2023-03-14 Jerzy Cioslowski , Christian Schilling , Rolf Schilling

Ground state properties of finite nuclei ($^{16}$O and $^{40}$Ca) are evaluated from realistic nucleon-nucleon interactions. The calculations are based on the Brueckner-Hartree-Fock approximation. Special attention is paid to the role of…

Nuclear Theory · Physics 2011-07-19 Kh. Gad , H. Müther

In this article, we derived a rigorous lower bound on the ground-state energy for a class of one-dimensional quantum systems in deformed space with minimal coordinate and momentum uncertainties, representing the absolute minimum energy that…

Quantum Physics · Physics 2026-05-05 Arsen Panas , Volodymyr Tkachuk

For a hydrogen atom subject to a constant magnetic field, we report a numerical realization of the two-dimensional Non-Linearization Procedure (NLP) to estimate the accuracy of the variational energy associated with a given trial function.…

Atomic Physics · Physics 2024-07-31 J. C. del Valle

Recent years have shown steady progress in research towards molecular electronics [1,2], where molecules have been investigated as switches [3-5], diodes [6], and electronic mixers [7]. In much of the previous work a Scanning Tunnelling…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. H. M. Smit , Y. Noat , C. Untiedt , N. D. Lang , M. van Hemert , J. M. van Ruitenbeek

Thanks to an algebraic duality property of reduced states, the Schmidt best approximation theorems have important corollaries in the rigorous theory of two-electron moleculae. In turn, the "harmonium mode" or "Moshinsky atom" constitutes a…

Chemical Physics · Physics 2012-06-01 Kurusch Ebrahimi-Fard , Jose M. Gracia-Bondia

The electron-electron correlation term in two-atomic collision is the most important, most difficult term to obtain the effective interatomic potential. Generally the H and H collision is a four center problem. It is extremely difficult to…

Atomic Physics · Physics 2013-11-14 Hasi Ray

The static and dynamic electric multipolar polarizabilities and second hyperpolarizabilities of the H$_2^+$, D$_2^+$, and HD$^+$ molecular ions in the ground and first excited states are calculated nonrelativistically using explicitly…

Atomic Physics · Physics 2014-09-23 Li-Yan Tang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb
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