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Here we a present a density functional theory study of pentacene ultra-thin films on flat [(111)] and vicinal [(455)] Au surfaces. We have performed crystal and electronic structure calculations by using PBE and optB86b-vdW functionals and…

Materials Science · Physics 2020-05-20 Ersen Mete , Mehmet Fatih Danisman

A new model for the intermediate compound of the hydrogen evolution reaction (HER) is proposed, for the electrochemical reduction of hydrogen in the presence of bisulfate on platinum(111). The formation of this compound, a regular 2…

Chemical Physics · Physics 2007-05-23 L. Blum , Dale A. Huckaby

Defects in crystalline silicon consisting of a silicon self-interstitial atom and one, two, three, or four hydrogen atoms are studied within density-functional theory (DFT). We search for low-energy defects by starting from an ensemble of…

Materials Science · Physics 2010-02-11 Andrew J. Morris , Chris J. Pickard , R. J. Needs

Ab initio random structure searching with density functional theory was used to determine the zero-temperature structures of atomic metallic hydrogen from 500 GPa to 5 TPa. Including zero point motion in the harmonic approximation, we…

Materials Science · Physics 2015-05-20 Jeffrey M. McMahon , David M. Ceperley

Orbital relaxation of the core region is a primary source of error in the computation of core ionization and core excitation energies. Recently, Transition-Potential Coupled Cluster (TP-CC) methods have been used to explicitly treat orbital…

Chemical Physics · Physics 2025-03-17 Alexis A. A. Delgado , Devin A. Matthews

Titanium borates show promissing hydrogen storage characteristics. Structural relaxation around individual hydrogen atoms and the binding energies are studied by means of the density functional theory methods for a number of hydrogenated…

Materials Science · Physics 2011-08-02 R. Žitko , H. J. P. Van Midden , E. Zupanič , A. Prodan , S. S. Makridis , D. Niarchos , A. K. Stubos

Density Functional Theory (DFT) calculations show a weak interaction between hydrogen and helium in iron, in contrast to previous reports of a strong trapping of hydrogen at helium. The strong preference of He and H to occupy regions with…

Materials Science · Physics 2012-10-22 C. J. Ortiz , R. Vila , J. M. Pruneda

Several commonly observed physical and biological systems are arranged in shapes that closely resemble an honeycomb cluster, that is, a tessellation of the plane by regular hexagons. Although these shapes are not always the direct product…

Optimization and Control · Mathematics 2025-01-10 Marco Caroccia , Kenneth DeMason , Francesco Maggi

We report ground state energies and structural properties for small helium clusters (4He) containing an H- impurity computed by means of variational and diffusion Monte Carlo methods. Except for 4He_2H- that has a noticeable contribution…

Atomic and Molecular Clusters · Physics 2009-10-31 M. Casalegno , M. Mella , G. Morosi , D. Bressanini

Density-functional theory based global geometry optimization is used to scrutinize the possibility of using endohedrally-doped hydrogenated Si clusters as building blocks for constructing highly magnetic materials. In contrast to the known…

Materials Science · Physics 2013-07-26 Dennis Palagin , Karsten Reuter

Experimental progress finally reached the metallic solid hydrogen phase, which was predicted by Wigner and Huntington over 80 years ago. However, the different structures in the phase diagram are still been debated due to the difficulty of…

Materials Science · Physics 2022-01-03 Tom Ichibha , Yunwei Zhang , Kenta Hongo , Ryo Maezono , Fernando A. Reboredo

Recently, the successful synthesis of the pentagonal form of PdTe$_{2}$ monolayer (\emph{p}-PdTe$_{2}$) was reported [Liu~\emph{et al.}, Nature Materials \textbf{23}, 1339 (2024)]. In this work, we present an extensive first-principles…

Materials Science · Physics 2025-01-07 Poonam Sharma , Vaishali Roondhe , Alok Shukla

We study the $z=0$ properties of clusters (and large groups) of galaxies within the context of interacting and non-interacting quintessence cosmological models, using a series of adiabatic SPH simulations. Initially, we examine the average…

Cosmology and Nongalactic Astrophysics · Physics 2015-06-18 Edoardo Carlesi , Alexander Knebe , Geraint F. Lewis , Gustavo Yepes

Using density-functional-theory calculations, we have identified new stable configurations for tri-, tetra-, and penta-vacancies in silicon. These new configurations consist of combinations of a ring-hexavacancy with three, two, or one…

Materials Science · Physics 2009-11-10 D. V. Makhov , Laurent J. Lewis

We have investigated the structural and electronic properties of phosphorescent planar platinum(II) complexes at the interface of Au(111) with submolecular resolution using combined scanning tunneling microscopy and spectroscopy as well as…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Pascal R. Ewen , Jan Sanning , Nikos L. Doltsinis , Matteo Mauro , Cristian A. Strassert , Daniel Wegner

We investigate the properties of clusters formed from two connected $\mathrm{Ge_{m}}$ cage-like clusters, such as experimentally synthesized $\mathrm{Au_3Ge_{18}^{5-}}$, using first-principles DFT methods. We focus particularly on…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 Danielle McDermott , Kathie E. Newman

In this work, we foresee the structure of a new class of borophenes with smaller 2D densities of atoms than those explored so far for 2D boron crystals. Boron atoms in the porous borophenes tend to be $5$-coordinated in contrast to commonly…

Materials Science · Physics 2021-11-25 T. Tarkowski , M. Marchwiany , N. Gonzalez Szwacki

Metallic solids are a challenging target for wavefunction-based electronic structure theories and have not been studied in great detail by such methods. Here, we use coupled-cluster theory with single and double excitations (CCSD) to study…

Materials Science · Physics 2022-04-05 Verena A. Neufeld , Hong-Zhou Ye , Timothy C. Berkelbach

The activity and stability of a platinum nanoparticle (NP) is not only affected by its size but additionally depends on its shape. To this end, simulations can identify structure-property relationships to make a priori decisions on the most…

Chemical Physics · Physics 2022-03-25 Björn Kirchhoff , Christoph Jung , Hannes Jónsson , Donato Fantauzzi , Timo Jacob

Electrical and structural characterization of nano-particles are very important steps to determine their potential applications in microelectronics. In this paper, we adress the crystallographic and electric transport properties of…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 B. C. Camargo , B. Lassagne , R. Arenal , C. Gatel , T. Blon , G. Viau , L-M Lacroix , W. Escoffier
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