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Molybdenum borides were studied theoretically using first-principles calculations, empirical total energy model and global optimization techniques to determine stable crystal structures. Our calculations reveal the structures of known Mo-B…

Materials Science · Physics 2020-03-10 Dmitry V. Rybkovskiy , Alexander G. Kvashnin , Yulia A. Kvashnina , Artem R. Oganov

A recent experimental work on palladium hydrides suggested that metastable structures with hydrogen atoms occupying tetrahedral sites could lead to superconductivity above 50 K, a huge increase compared to the 10 K critical temperature of…

Superconductivity · Physics 2023-01-25 Antonella Meninno , Ion Errea

Context Mixed-metal clusters have long been studied because of their peculiar properties and how they change with cluster size, composition and charge state and their potential roles in catalysis. The characterization of these clusters is…

Chemical Physics · Physics 2024-04-30 Paulo H. Acioli

We present a comprehensive first-principles investigation of carbon self-interstitial defects in diamond, ranging from mono- to hexa-interstitial complexes. By quantum mechanical density functional theory, empowered by interatomic potential…

Materials Science · Physics 2026-05-01 Nima Ghafari Cherati , Arsalan Hashemi , Ádám Gali

The atomic orbital basis and atomic pseudopotential for electron-ion interaction in framework of density function theory used to calculate C70H84 spin polarized diamond cluster with neutral vacancy. The band gap has been found to be 1.70…

Materials Science · Physics 2012-02-28 S. Sheikholeslami , A. Shafiekhani

Almost all the polymer crystals have several polymorphic modifications. Their structure and existence conditions, as well as transitions between them are not understood even in the case of the 'model' polymer polyethylene (PE). For analysis…

Materials Science · Physics 2011-09-06 Elena A. Zubova , Alexander V. Savin , Nikolay K. Balabaev

Dense polyhedron packings are useful models of a variety of condensed matter and biological systems and have intrigued scientists mathematicians for centuries. Recently, organizing principles for the types of structures associated with the…

Soft Condensed Matter · Physics 2011-09-28 Yang Jiao , Sal Torquato

The energetic ground state of gold clusters with up to 314 atoms consists of rather complicated geometries that have only a weak resemblance to the perfect icosahedra, decahedra and octahedra that are encountered for some magic numbers. The…

Materials Science · Physics 2008-10-14 Kuo Bao , Stefan Goedecker , Kenji Koga , Frederic Lancon , Alexey Neelov

Unlike covalent two-dimensional (2D) materials like graphene, 2D metals have non-layered structures due to their non-directional, metallic bonding. While experiments on 2D metals are still scarce and challenging, density-functional theory…

Materials Science · Physics 2023-01-06 Kameyab Raza Abidi , Pekka Koskinen

This is a follow-up of our recently proposed work on pseudopotential calculation (Ref. [21]) of atoms and molecules within DFT framework, using cartesian coordinate grid. Detailed results are presented to demonstrate the usefulness,…

Chemical Physics · Physics 2015-05-18 Amlan K. Roy

Noble metals adopt close-packed structures at ambient pressure and rarely undergo structural transformation at high pressures. Platinum (Pt), in particular, is normally considered to be unreactive and is therefore not expected to form…

Superconductivity · Physics 2015-03-19 Duck Young Kim , Ralph H. Scheicher , Chris J. Pickard , R. J. Needs , R. Ahuja

A series of electronic and structural transitions are predicted in molten lithium from first principles. A new phase with tetrahedral local order characteristic of $sp^3$ bonded materials and poor electrical conductivity is found at…

Materials Science · Physics 2009-07-09 Isaac Tamblyn , Jean-Yves Raty , Stanimir A. Bonev

The structural and electronic properties of germanium clathrates Ge$_{46}$ and K$_8$Ge$_{46}$ are studied by first principles calculations within the local density approximation. The equilibrium structures are obtained by {\em ab initio}…

Condensed Matter · Physics 2009-10-31 Jijun Zhao , Alper Buldum , Jianping Lu , C. Y. Fong

The structural, electronic, mechanical, optical, thermodynamic properties of plutonium monoxide monohydride (PuOH) are studied by density-functional calculations within the framework of LDA/GGA and LDA/GGA+U.From the total energy…

Materials Science · Physics 2020-01-14 Ruizhi Qiu , Haiyan Lu , Bingyun Ao , Tao Tang , Piheng Chen

As a second part of a previous paper, here the calculated electronic band structure of ideal Pt(100) and Pt(110) surfaces, studied using density functional theory and the empirical tight-binding method, is presented. A detailed discussion…

Materials Science · Physics 2015-03-17 H. J. Herrera-Suarez , A. Rubio-Ponce , D. Olguin

In this work, we employ density functional theory (DFT) to explore the structure of boron clusters doped with two aluminium atoms (B$_7$Al$_2$ or Al$_2$B$_7$). The results show that the most stable structure is a bipyramidal configuration…

Materials Science · Physics 2024-09-30 Peter Ludwig Rodríguez-Kessler

We use density functional theory to quantify finite size and shape effects for gold nanoclusters. We concentrate on the computation of binding energy as a function of bond length for icosahedral and cuboctohedral clusters. We find that the…

Mesoscale and Nanoscale Physics · Physics 2009-12-31 Michael McGuigan , J. W. Davenport

In this paper we analyze the band-structure of two-dimensional (2D) halide perovskites by considering structures related to the simpler case of the series, (BA)$_2$PbI$_4$, in which PbI$_4$ layers are intercalated with butylammonium…

Materials Science · Physics 2023-07-24 Efstratios Manousakis

Properties of point defects resulting from the incorporation of inert-gas atoms in bcc tungsten are investigated systematically using first-principles density functional theory (DFT) calculations. The most stable configuration for the…

Materials Science · Physics 2015-10-29 Duc Nguyen-Manh , S. L. Dudarev

We study the electronic structure and correlated phases of twisted bilayers of platinum diselenide using large-scale ab initio simulations combined with the functional renormalization group. PtSe$_2$ is a group-X transition metal…

Strongly Correlated Electrons · Physics 2022-01-27 Lennart Klebl , Qiaoling Xu , Ammon Fischer , Lede Xian , Martin Claassen , Angel Rubio , Dante M. Kennes