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Related papers: Cold Molecule Spectroscopy for Constraining the Ev…

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We demonstrate the long-term ($<$ 1 minute) trapping of Stark-decelerated OH radicals in their $X~^{2}\Pi _{3/2}~(\nu = 0,~J = 3/2,~M_{J} = 3/2,~f)$ state in a permanent magnetic trap. The trap environment was cryogenically cooled to a…

Chemical Physics · Physics 2019-08-05 Dominik Haas , Claudio von Planta , Thomas Kierspel , Dongdong Zhang , Stefan Willitsch

The Stark deceleration of OH radicals in both low-field-seeking and high-field-seeking levels of the rovibronic ${}^2\Pi_{3/2},v=0,J=3/2$ ground state is demonstrated using a single experimental setup. Applying alternating-gradient…

Chemical Physics · Physics 2008-09-18 Kirstin Wohlfart , Frank Filsinger , Fabian Grätz , Jochen Küpper , Gerard Meijer

Recently, the extremely sensitive torsion-rotation transitions in methanol have been used to set a tight constraint on a possible variation of the proton-to-electron mass ratio over cosmological time scales. In order to improve this…

Cold, neutral hydroxyl radicals are Stark decelerated and confined within a magnetic trap consisting of two permanent ring magnets. The OH molecules are trapped in the ro-vibrational ground state at a density of $\sim10^{6}$ cm$^{-3}$ and…

Atomic Physics · Physics 2009-01-22 Brian C. Sawyer , Benjamin K. Stuhl , Dajun Wang , Mark Yeo , Jun Ye

The precise measurement of molecular vibrational transition frequencies is useful in the search for variation in the proton-to-electron mass ratio {\mu}. Homonuclear diatomic molecules are particularly advantageous for precise measurement…

Atomic Physics · Physics 2017-03-01 Masatoshi Kajita

We report absolute optical frequencies of electronic transitions from the $X\, ^2\Pi_{3/2},v''=0,J''=3/2$ rovibronic ground state to the 12 lowest levels of the $A\, ^2\Sigma^+,v'=0$ vibronic state in $^{16}$OH, as well as to the 16 lowest…

Atomic Physics · Physics 2018-12-05 Arthur Fast , John E. Furneaux , Samuel A. Meek

Theories unifying gravity with other interactions suggest spatial and temporal variation of fundamental ``constants'' in the Universe. A change in the fine structure constant, alpha, could be detected via shifts in the frequencies of atomic…

Precise molecular transition frequencies are of great interest in the test of fundamental physics and also in various applications. Two well isolated ro-vibrational transitions of $^{12}$C$^{16}$O at 1.57 $\mu$m, R(9) and R(10) in the…

Atomic Physics · Physics 2017-10-11 Jin Wang , Yu R. Sun , Lei-Gang Tao , An-Wen Liu , Shui-Ming Hu

Precision measurements with ultracold molecules require development of robust and sensitive techniques to produce and interrogate the molecules. With this goal, we theoretically analyze factors that affect frequency measurements between…

Quantum Physics · Physics 2009-11-13 S. Kotochigova , T. Zelevinsky , Jun Ye

We have detected the four 18cm OH lines from the $z \sim 0.765$ gravitational lens toward PMN J0134-0931. The 1612 and 1720 MHz lines are in conjugate absorption and emission, providing a laboratory to test the evolution of fundamental…

The hydroxyl radical, hereafter referred to as the OH molecule (OHM), carries both electric and magnetic dipole moments and, as a diatomic molecule, admits a comparatively simple and accurate model. This makes it a natural quantum probe for…

Quantum Physics · Physics 2026-05-01 Luca Previdi , Francesco Albarelli , Matteo G. A. Paris

Rapid progress in cooling and trapping of molecules has enabled first experiments on high resolution spectroscopy of trapped diatomic molecules, promising unprecedented precision. Extending this work to polyatomic molecules provides unique…

Atomic Physics · Physics 2021-10-22 Alexander Prehn , Martin Ibrügger , Gerhard Rempe , Martin Zeppenfeld

A new method for examining the possible space-time variation of the fine structure constant ($\alpha$) is proposed. The technique uses a relatively simple measurement with an optical resonator to compare atom-stabilized optical frequency…

Atomic Physics · Physics 2007-05-23 J. R. Torgerson

Precise radial velocity measurements (delta v/c ~ 10^{-7}) of FeII lines in damped Ly-alpha systems from very high quality VLT/UVES spectra of quasars HE0515-4414 and Q1101-264 are used to probe cosmological time dependence of the fine…

Precision comparisons of different atomic frequency standards over a period of a few years can be used for a sensitive search for temporal variations of fundamental constants. We present recent frequency measurements of the 688 THz…

Atomic Physics · Physics 2008-11-25 E. Peik , B. Lipphardt , H. Schnatz , Chr. Tamm , S. Weyers , R. Wynands

Weak transitions in the (2,0) overtone band of the HD molecule at $\lambda = 1.38 \, \mu$m were measured in saturated absorption using the technique of noise-immune cavity-enhanced optical heterodyne molecular spectroscopy. Narrow…

Atomic Physics · Physics 2018-04-18 F. M. J. Cozijn , P. Dupre , E. J. Salumbides , K. S. E. Eikema , W. Ubachs

We report new precise H$(e,e^\prime p)\pi^0$ measurements at the $\Delta(1232)$ resonance at $Q^2= 0.127$ (GeV/c)$^2$ using the MIT/Bates out-of-plane scattering (OOPS) facility. The data reported here are particularly sensitive to the…

Nuclear Experiment · Physics 2009-11-10 N. F. Sparveris , OOPS Collaboration

Star-forming galaxies at high redshifts are the ideal targets to probe the hypothetical variation of the fine-structure constant alpha over cosmological time scales. We propose a modification of the alkali doublets method which allows us to…

Cosmology and Nongalactic Astrophysics · Physics 2017-05-10 S. A. Levshakov , M. G. Kozlov

Theories unifying gravity with other interactions suggest spatial and temporal variation of fundamental "constants" in the Universe. A change in the fine structure constant, alpha, could be detected via shifts in the frequencies of atomic…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-20 J. C. Berengut , V. A. Dzuba , V. V. Flambaum , J. A. King , M. G. Kozlov , M. T. Murphy , J. K. Webb

We report the measurement of hyperfine splitting in the $7d$ $^{2}D_{3/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy in a Cs vapor cell. We determine the hyperfine coupling constants $A = 7.3509(9)$ MHz…

Atomic Physics · Physics 2022-10-05 Bubai Rahaman , Sourav Dutta