Related papers: High-resolution hyperfine spectroscopy of excited …
We analyze a model where a closed $V$ system is excited by two uncorrelated partially coherent fields. We use a collisionally broadened CW laser, which is a good model for an experimentally realizable partially coherent field, and show that…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
The concept of mode locking in laser is applied to a two-photon state with frequency entanglement. Cavity enhanced parametric down-conversion is found to produce exactly such a state. The mode-locked two-photon state exhibits a comb-like…
We investigate the prospects of using two-mode intensity squeezed twin-beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof of principle demonstration,…
Entanglement in high-dimensional quantum systems, where one or more degrees of freedom of light are involved, offers increased information capacities and enables new quantum protocols. Here, we demonstrate a functional source of…
Quantum phenomena such as entanglement can improve fundamental limits on the sensitivity of a measurement probe. In optical interferometry, a probe consisting of $N$ entangled photons provides up to a $\sqrt{N}$ enhancement in phase…
In a two level atom, real-time quantum state holography is performed through interferences between quantum states created by a reference pulse and a chirped pulse resulting in coherent transients. A sequence of several measurements allows…
Conical intersections serve as critical gateways in photochemical reactions, enabling rapid nonradiative transitions between potential energy surfaces that underpin fundamental processes such as photosynthesis or vision. Their calculation…
Recently, integrated photonic circuits have brought new capabilities to electron microscopy and been used to demonstrate efficient electron phase modulation and electron-photon correlations. Here, we quantitatively analyze the feasibility…
Fast beam collinear laser spectroscopy is the established method to investigate nuclear ground state properties such as the spin, the electromagnetic moments, and the charge radius of exotic nuclei. These are extracted with high precision…
We investigate the role of excited states in High-order Harmonic Generation by studying the spectral, spatial and temporal characteristics of the radiation produced near the ionization threshold of argon by few-cycle laser pulses. We show…
We demonstrate theoretically that electromagnetically induced transparency can be achieved in metamaterials, in which electromagnetic radiation is interacting resonantly with mesoscopic oscillators rather than with atoms. We describe novel…
The development of high-intensity ultrashort laser pulses unlocks the potential of pump-probe spectroscopy in sub-femtosecond timescale. Notably, subcycle pump pulses can generate electronic states unreachable by conventional multicycle…
We present a phase induced transparency based scheme to generate structured beam patterns in a closed four level atomic system. We employ phase structured probe beam and a transverse magnetic field (TMF) to create phase dependent medium…
We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2}…
Using a linear optical elements and post-selection, we construct an entangled polarization state of three photons in the same spatial mode. This state is analogous to a ``photon-number path entangled state'' and can be used for…
Surface enhanced Raman spectroscopy, is a technique of fundamental importance to analytical science and technology where the amplified Raman spectrum of analytes is used for chemical fingerprinting. Here, we showcase an engineered…
Ultrafast photoexcitation offers a novel approach to manipulating quantum materials. One of the long-standing goals in this field is to achieve optical control over topological properties. However, the impact on their electronic structures,…
The photoexcited state in superconducting metals and alloys was studied via pump-probe spectroscopy. A pulsed Ti:sapphire laser was used to create the non-equilibrium state and the far-infrared pulses of a synchrotron storage ring, to which…
The resonant state expansion (RSE), a rigorous perturbative method in electrodynamics, is applied to two-dimensional open optical systems. The analytically solvable homogeneous dielectric cylinder is used as unperturbed system, and its…