Related papers: High-resolution hyperfine spectroscopy of excited …
Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…
This study analyzed the optical techniques for high resolution, low-noise spectroscopy of a hyperfine structure (HFS) made of ytterbium-isotope 171 ions ($^{171}\mathrm{Yb}^{3+}$:$\mathrm{Y}_2\mathrm{SiO}_5$). Large energy spacings in…
We report experimental observations of interference between three-photon and one-photon excitations, and phase control of light attenuation/transmission in a four-level system. Either constructive interference or destructive interference…
In this paper, we report theoretical calculations of the photo-induced absorption (PA) spectrum of naphthalene and anthracene, with the aim of understanding those excited states, which are invisible in the linear optical absorption. The…
Rydberg molecules, often exemplified by long-range "trilobite" molecules, are a subject of much recent interest at high principal quantum number $n$. States that use the same bonding mechanism can exist at much lower $n$ and less-extreme…
Observation of internal quantum dynamics relies on correlations between the system being observed and the measurement apparatus. We propose using the center-of-mass (c.m.) degrees of freedom of atoms and molecules as a "built-in" monitoring…
The coherent superposition of two-atomic levels induced by coherent population trapping is employed in a standard $\Lambda$ type scheme to form a tripod-like system. A weak probe pulse scanning across the system is shown to experience a…
We investigate, theoretically and experimentally, the transmission of light through a thermal vapour of three-level ladder-type atoms, in the presence of 2 counter-propagating control fields. A simple theoretical model predicts the presence…
The excited state dynamics of chromophores in complex environments determine a range of vital biological and energy capture processes. Time-resolved, multidimensional optical spectroscopies provide a key tool to investigate these processes.…
Transient absorption (TA) spectroscopy has long been an invaluable tool for determining the energetics and dynamics of excited states in atomic, molecular, and solid-state systems. When pump pulse intensities are sufficiently high, the…
We consider a method for efficient parametric generation of a laser pulse. A single laser field is injected to a three-level medium which has two lower states and one excited state. The lower states are prepared initially in a…
Intersystem crossings between singlet and triplet states represent a crucial relaxation pathway in photochemical processes. Herein, we probe the intersystem crossing in hexafluoro-acetylacetone with ultrafast X-ray transient absorption…
Optical driving of materials has emerged as a versatile tool to control their properties, with photo-induced superconductivity being among the most fascinating examples. In this work, we show that light or lattice vibrations coupled to an…
We experimentally demonstrate a detection scheme suitable for state analysis of single optically trapped atoms in less than 1 {\mu}s with an overall detection efficiency {\eta} exceeding 98%. The method is based on hyperfine-state-selective…
Superradiance typically requires preparation of atoms in highly entangled multi-particle states, the so-called Dicke states. In this paper we discuss an alternative route where we prepare such states from initially uncorrelated atoms by a…
We present a scheme to controllably improve the accuracy of tight-binding Hamiltonian matrices derived by projecting the solutions of plane-wave ab initio calculations on atomic orbital basis sets. By systematically increasing the…
Electronic states and their dynamics are of critical importance for electronic and optoelectronic applications. Here, we probe various relevant electronic states in monolayer MoS2, such as multiple excitonic Rydberg states and free-particle…
We propose and experimentally verify a scheme to engineer arbitrary states of traveling light field up to the two-photon level. The desired state is remotely prepared in the signal channel of spontaneous parametric down-conversion by means…
We report the first observation of electromagnetically induced transparency (EIT) in an isotopically purified Nd$^{3+}$:YLiF$_4$ crystal. This crystal demonstrates inhomogeneous broadening of optical transitions of about 35 MHz. EIT is…
We study the excitation spectroscopy of few-electron, parallel coupled double quantum dots (QDs). By applying a finite source drain voltage to a double QD (DQD), the first excited states observed in nonequilibrium charging diagrams can be…