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Above 54.4 eV, two-photon double ionization of helium is dominated by a sequential absorption process, producing characteristic behavior in the single and triple differential cross sections. We show that the signature of this process is…

Atomic Physics · Physics 2009-11-13 D. A. Horner , T. N. Rescigno , C. W. McCurdy

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

We develop an approximate model for the process of direct (nonsequential) two-photon double ionization of atoms. Employing the model, we calculate (generalized) total cross sections as well as energy-resolved differential cross sections of…

Quantum Physics · Physics 2016-08-17 Morten Førre , Sølve Selstø , Raymond Nepstad

Both uncorrelated ("sequential") and correlated ("nonsequential") processes contribute to the double ionization of the helium atom in strong laser pulses. The double ionization probability has a characteristic "knee" shape as a function of…

Chaotic Dynamics · Physics 2011-12-12 François Mauger , Cristel Chandre , T. Uzer

We explore the influence of elliptical polarization on the (non)sequential two-photon double ionization of atomic helium with ultrashort extreme ultraviolet (XUV) light fields using time-dependent full ab-initio simulations. The energy and…

Atomic Physics · Physics 2019-02-20 Stefan Donsa , Iva Brezinova , Hongcheng Ni , Johannes Feist , Joachim Burgdörfer

We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…

Atomic Physics · Physics 2020-03-24 Fengzheng Zhu , Genliang Li , Aihua Liu

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We report on a kinematically complete experiment on strong field double ionization of helium using laser pulses with a wavelength of 394\,nm and intensities of $3.5-5.7\times10^{14}\,W/cm^2$. Our experiment reaches the most complete level…

Double photo-electron momentum spectra of the Helium atom are calculated \textit{ab initio} at extreme ultra-violet and near infrared wavelengths. At short wavelengths two-photon double ionization yields, two-electron energy spectra, and…

Computational Physics · Physics 2016-02-17 Alejandro Zielinski , Vinay Pramod Majety , Armin Scrinzi

We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our…

Atomic Physics · Physics 2008-05-07 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schroedinger equation. We present details of the method and calculate (generalized) cross…

Atomic Physics · Physics 2010-06-11 R. Nepstad , T. Birkeland , M. Førre

Triple-differential cross sections for two-photon double ionization of molecular hydrogen are presented for a central photon energy of 30 eV. The calculations are based on a fully {\it ab initio}, nonperturbative, approach to the…

Atomic Physics · Physics 2016-11-17 Xiaoxu Guan , Klaus Bartschat , Barry I. Schneider

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime…

Atomic Physics · Physics 2010-01-19 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We present a theoretical study of atomic laser-assisted photoionization emission (LAPE). We consider an atom driven by a linearly polarized XUV laser in two different scenarios: i) a single attosecond pulse (in both the streaking and…

Atomic Physics · Physics 2020-10-21 Renata Della Picca , Marcelo F. Ciappina , Maciej Lewenstein , Diego G. Arbó

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

Non-perturbative resonant multiphoton ionization $(1+1)$ is studied using the resolvent operator technique. Scaling parameters for effective two-level Hamiltonians are computed for hydrogen and helium atoms to provide a quantitative…

Atomic Physics · Physics 2023-09-25 Edvin Olofsson , Jan Marcus Dahlström

We investigate single photon double ionization (PDI) of helium at photon energies of 440 and 800 eV. We observe doubly charged ions with close to zero momentum corresponding to electrons emitted back-to-back with equal energy. These slow…

We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT…

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos
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