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The relativistic two-particle quantum mixtures are studied from the topological point of view. The mixture field variables can be transformed in such a way that a kinematical decoupling of both particle degrees of freedom takes place with a…

High Energy Physics - Theory · Physics 2007-05-23 S. Pruss-Hunzinger , S. Rupp , M. Sorg

Roles of electron correlation effects in the determination of attachment energies, magnetic dipole hyperfine structure constants and electric dipole (E1) matrix elements of the low-lying states in the singly charged cadmium ion (Cd$^+$)…

Atomic Physics · Physics 2018-03-14 Cheng-Bin Li , Yan-Mei Yu , B. K. Sahoo

We have developed an all particle Fock-space relativistic coupled-cluster method for two-valence atomic systems. We then describe a scheme to employ the coupled-cluster wave function to calculate atomic properties. Based on these…

Atomic Physics · Physics 2011-01-11 B. K. Mani , D. Angom

Quantum periodic cluster methods for strongly correlated electron systems are reformulated and developed. The reformulation and development are based on a canonical transformation which periodizes the fermions in the cluster space. The…

Strongly Correlated Electrons · Physics 2007-05-23 Tran Minh-Tien

We present several coupled-cluster calculations of ground and excited states of 4He and 16O employing methods from quantum chemistry. A comparison of coupled cluster results with the results of exact diagonalization of the hamiltonian in…

We propose a new formulation of time-dependent coupled cluster with adaptive basis functions and division of the one-particle space into active and secondary subspaces. The formalism is fully bivariational in the sense of a real-valued…

Chemical Physics · Physics 2024-02-20 Mads Greisen Højlund , Ove Christiansen

We have carried out a detailed and systematic study of the correlation energies of inert gas atoms Ne, Ar, Kr and Xe using relativistic many-body perturbation theory and relativistic coupled-cluster theory. In the relativistic…

Atomic Physics · Physics 2009-12-29 B. K. Mani , D. Angom

We describe a quantitative construction of almost-normal diffeomorphisms between embedded orientable manifolds with boundary to be used in the study of geometric variational problems with stratified singular sets. We then apply this…

Analysis of PDEs · Mathematics 2015-06-09 Marco Cicalese , Gian Paolo Leonardi , Francesco Maggi

Time-dependent response theories are foundational to the development of algorithms that determine quantum properties of electronic excited states of molecules and periodic systems. They are employed in wave-function, density-functional, and…

Chemical Physics · Physics 2022-11-23 Martín A. Mosquera

We demonstrate a method of creating photonic two-dimensional cluster states that is considerably more efficient than previously proposed approaches. Our method uses only local unitaries and type-I fusion operations. The increased efficiency…

Quantum Physics · Physics 2009-11-11 Gerald Gilbert , Michael Hamrick , Yaakov S. Weinstein

Finite temperature disordered solid solutions and magnetic materials are difficult to study directly using first principles calculations, due to the large unit cells and many independent samples that are required. In this work, we develop a…

Materials Science · Physics 2019-05-22 Kevin F. Garrity

We introduce a range-separation approximation to coupled cluster doubles (CCD) theory that successfully overcomes limitations of regular CCD when applied to the uniform electron gas. We combine the short-range ladder channel with the…

Chemical Physics · Physics 2014-05-07 James J. Shepherd , Thomas M. Henderson , Gustavo E. Scuseria

A general technique is presented for constructing a quantum theory of a finite number of interacting particles satisfying Poincar\'e invariance, cluster separability, and the spectral condition. Irreducible representations and…

Nuclear Theory · Physics 2015-06-26 W. N. Polyzou

In truncated coupled-cluster (CC) theories, non-variational and/or generally complex ground-state energies can occur. This is due to the non-Hermitian nature of the similarity transformed Hamiltonian matrix in combination with CC…

Chemical Physics · Physics 2023-09-22 Tanner Culpitt , Erik I. Tellgren , Fabijan Pavosevic

We consider a new formulation of the stochastic coupled cluster method in terms of the similarity transformed Hamiltonian. We show that improvement in the granularity with which the wavefunction is represented results in a reduction in the…

Chemical Physics · Physics 2016-02-02 Ruth S. T. Franklin , James S. Spencer , Alberto Zoccante , Alex J. W. Thom

The variational quantum eigensolver has been proposed as a low-depth quantum circuit that can be employed to examine strongly correlated systems on today's noisy intermediate-scale quantum computers. We examine details associated with the…

Quantum Physics · Physics 2020-08-26 Luogen Xu , Joseph T. Lee , J. K. Freericks

Hyperfine constants and anomalies of ground as well as few low lying excited states of $^{113,115,117}$In III are studied with highly correlated relativistic coupled-cluster theory. The ground state hyperfine splitting of $^{115}$In III is…

Atomic Physics · Physics 2015-06-18 Sourav Roy , Narendra Nath Dutta , Sonjoy Majumder

The electronic properties of one-dimensional clusters of N atoms or molecules have been studied. The model used is similar to the Kronig-Penney model with the potential offered by each ion being approximated by an attractive delta function.…

Other Condensed Matter · Physics 2015-06-25 S N Behera , S Gayen , G V Ravi Prasad , S M Bose

The lifetime of a system of connected units under some natural assumptions can be represented as a random variable Y defined as a weighted lattice polynomial of random lifetimes of its components. As such, the concept of a random variable Y…

Probability · Mathematics 2008-05-28 Alexander Dukhovny , Jean-Luc Marichal

In this work a calculation of the cluster decomposable formalism for relativistic scattering as developed by Lindesay, Markevich, Noyes, and Pastrana (LMNP) is made for an ultra-light quantum model. After highlighting areas of the theory…

Nuclear Theory · Physics 2022-10-12 Marcus Alfred , James Lindesay