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High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron

Using time-dependent density functional theory, high-harmonic generation (HHG) is studied in one-dimensional structures of sizes from a single nucleus up to hundreds of nuclei. The HHG cutoff is observed to extent linearly with the system…

Atomic Physics · Physics 2018-04-27 Kenneth K. Hansen , Dieter Bauer , Lars Bojer Madsen

We investigate the high-order harmonic generation (HHG) in doped semiconductors. The HHG is simulated with the single-electron time-dependent Schr\"{o}dinger equation (TDSE). The results show that the high-order harmonics in the second…

Optics · Physics 2017-11-22 Tengfei Huang , Xiaosong Zhu , Liang Li , Xi Liu , Pengfei Lan , Peixiang Lu

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

Atomic Physics · Physics 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive High Harmonic Generation (HHG). The mixing of beams with different OAM allows to generate two laser foci tightly spaced to study…

Chemical Physics · Physics 2019-07-24 Jan Troßand Carlos A. Trallero-Herrero

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

Toroidal vortex is a kind of novel and exotic structured light with potential applications in photonic topology and quantum information. Here, we present the study on high harmonic generation (HHG) from the interaction of the intense…

Optics · Physics 2024-10-10 Zijian Lyu , Yiqi Fang , Yunquan Liu

We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…

We report a detailed study of high-order harmonic generation (HHG) in helium. When comparing predictions from a single-active-electron model with those from all-electron simulations, such as ATTOMESA and R-matrix with time-dependence, which…

Atomic Physics · Physics 2024-03-06 A. T. Bondy , S. Saha , J. C. del Valle , A. Harth , N. Douguet , K. R. Hamilton , K. Bartschat

Orbital angular momentum (OAM) light beams for high-order harmonic generation (HHG) provide an additional degree of freedom to study the light-matter interaction at ultrafast timescales. A more sophisticated configuration is a perfect…

Optics · Physics 2024-10-01 Bikash Kumar Das , C. Granados , M. Krüger , Marcelo F. Ciappina

We present an analytical framework for the emergence of nonclassical radiation in strongly laser-driven quantum systems, with a focus on high-order harmonic generation (HHG). Starting from a Pauli-Fierz description, we employ a parametric…

Quantum Physics · Physics 2026-04-23 Ivan Gonoskov , Christian Hünecke , Stefanie Gräfe

We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

High harmonic generation (HHG) in solid and gaseous targets has been proven to be a powerful avenue for the generation of attosecond pulses, whereas the influence of electron-phonon scattering on HHG is a critical outstanding problem. Here…

Optics · Physics 2022-06-02 Tao-Yuan Du , Chao Ma

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

Atomic Physics · Physics 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

Quantum Physics · Physics 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

Non-perturbative high-harmonic generation (HHG) has recently been observed in the liquid phase, where it was demonstrated to have a different physical mechanism compared to gas and solid phases of matter. The currently best physical picture…

We investigate the photoelectron angular emission distributions obtained by strong field dissociative ionization of H$_2$ using cold target recoil ion momentum spectroscopy. In case of employing laser light with an ellipticity close to 0.9…

High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…

Quantum Physics · Physics 2025-07-04 J. Rivera-Dean , P. Stammer , M. F. Ciappina , M. Lewenstein