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We present an analytical calculation of the complete $\alpha^6$ correction to energies of $nP$-levels of two-body systems consisting of the spin-$0$ or $1/2$ extended-size particles with arbitrary masses and magnetic moments. The obtained…

Atomic Physics · Physics 2026-02-19 Vojtěch Patkóš , Vladimir A. Yerokhin , Krzysztof Pachucki

We perform ab initio calculations of the QED effects of order $m\alpha^7$ for the $2^3S$ and $2^3P$ states of He-like ions. The computed effects are combined with previously calculated energies from [V. A. Yerokhin and K. Pachucki, Phys.…

Atomic Physics · Physics 2023-02-01 Vladimir A. Yerokhin , Vojtěch Patkóš , Krzysztof Pachucki

The pair potential for helium has been computed with accuracy improved by an order of magnitude relative to the best previous determination. For the well region, its uncertainties are now below 1 millikelvin. The main improvement is due to…

Chemical Physics · Physics 2017-09-27 Michal Przybytek , Wojciech Cencek , Bogumil Jeziorski , Krzysztof Szalewicz

Formulas and expectation values which are need to determine the lowest-order QED corrections ($\sim \alpha^3$) and corresponding recoil (or finite mass) corrections in the two-electron helium-like ions are presented. Other important…

Atomic Physics · Physics 2015-09-22 Alexei M. Frolov

The nonrelativistic energy of low lying rovibrational levels of HT, DT, and \T\ is determined to an absolute accuracy of $10^{-7}-10^{-8}$ cm$^{-1}$ using the variational method with the four-body nonadiabatic James-Coolidge functions. The…

Chemical Physics · Physics 2023-01-11 Krzysztof Pachucki , Jacek Komasa

With this work we start a project of calculating the QED contribution of order $\alpha^7m$ to the $2^3P$-$2^3S$ transition energy in helium, aiming for an accurate determination of the nuclear charge radius $r_E$ from measurements of the…

Atomic Physics · Physics 2021-02-16 Vladimir A. Yerokhin , Vojtěch Patkóš , Krzysztof Pachucki

The technique of quantum electrodynamics (QED) calculations of energy levels in the helium atom is reviewed. The calculations start with the solution of the Schr\"odinger equation and account for relativistic and QED effects by perturbation…

Atomic Physics · Physics 2021-07-14 Vladimir A. Yerokhin , Vojtech Patkos , Krzysztof Pachucki

We investigate the finite nuclear mass corrections in the helium atom in order to resolve a significant disagreement between the $2^3S - 2^3P$ and $2^3S - 2^1S$ transition isotope shifts. These two transitions lead to discrepant results for…

Atomic Physics · Physics 2017-01-31 V. Patkos , V. A. Yerokhin , K. Pachucki

Quantum electrodynamical (QED) calculations of ionization energies of the $1snd\,D$ states are performed for the helium atom. We reproduce the previously known relativistic and QED effects up to order $m\alpha^5$ and extend the theory by…

Atomic Physics · Physics 2020-07-14 Vladimir A. Yerokhin , Vojtěch Patkóš , Mariusz Puchalski , Krzysztof Pachucki

Calculational results are presented for the fine-structure splitting of the 2^3P state of helium and helium-like ions with the nuclear charge Z up to 10. Theoretical predictions are in agreement with the latest experimental results for the…

Atomic Physics · Physics 2015-05-20 Krzysztof Pachucki , Vladimir A. Yerokhin

We report the potential energy curve, the diagonal Born-Oppenheimer, non-adiabatic mass, relativistic, and leading-order QED corrections for the ground electronic state of the helium dimer cation; the higher-order QED and finite-nuclear…

Chemical Physics · Physics 2026-02-25 Edit Mátyus , Ádám Margócsy

The non-additive three-body interaction potential for helium was computed using the coupled-cluster theory and the full configuration interaction method. The obtained potential comprises an improved nonrelativistic Born--Oppenheimer energy…

Relativistic, quantum electrodynamics, as well as non-adiabatic corrections and couplings, are computed for the b $^3\Pi_\mathrm{g}$ and c $^3\Sigma_\mathrm{g}^+$ electronic states of the helium dimer. The underlying Born-Oppenheimer…

Chemical Physics · Physics 2025-09-03 Balázs Rácsai , Péter Jeszenszki , Ádám Margócsy , Edit Mátyus

The radium atom is a promising system for studying parity and time invariance violating weak interactions. However, available experimental spectroscopic data for radium is insufficient for designing an optimal experimental setup. We…

Atomic Physics · Physics 2009-11-13 V. A. Dzuba , V. V. Flambaum

We consider the uncertainty of theoretical calculations for a specific difference of the hyperfine intervals in the 1s and 2s states in a light hydrogen-like atom. For a number of crucial radiative corrections the result for hydrogen atom…

High Energy Physics - Phenomenology · Physics 2009-11-11 Savely G. Karshenboim , Vladimir G. Ivanov

It is shown that the non-relativistic ground state energy of helium-like and lithium-like ions with static nuclei can be interpolated in full physics range of nuclear charges $Z$ with accuracy of not less than 6 decimal digits (d.d.) or 7-8…

Atomic Physics · Physics 2017-11-27 Alexander V. Turbiner , Juan C. Lopez Vieyra , Horacio Olivares Pilon

For heliumlike uranium, the energies of the singly-excited $1sns$, $1snp$, and $1snd$ states with $n\leq 4$ and the probabilities of the one-photon $1s3d\to 1s2p$, $1s3p\to 1s2s$, $1s3p\to 1s2p$ and $1s4d\to 1s2p$ transitions are evaluated.…

Atomic Physics · Physics 2024-01-17 N. K. Dulaev , M. Y. Kaygorodov , A. V. Malyshev , I. I. Tupitsyn , V. M. Shabaev

We present a new computational method for the determination of energy levels in four-particle systems like H$_2$, HD, and HeH$^+$ using explicitly correlated exponential basis functions and analytic integration formulas. In solving the…

Chemical Physics · Physics 2018-02-14 Krzysztof Pachucki , Jacek Komasa

Extensive variational computations are reported for the ground state energy of the non-relativistic two-electron atom. Several different sets of basis functions were systematically explored, starting with the original scheme of Hylleraas.…

Atomic Physics · Physics 2009-11-07 Charles Schwartz

Results are presented for highly accurate ab initio variational calculation of the rotation - vibration energy levels of H2O2 in its electronic ground state. These results use a recently computed potential energy surface and the variational…

Earth and Planetary Astrophysics · Physics 2014-06-27 Oleg L. Polyansky , Igor N. Kozin , Roman I. Ovsyannikov , Pawel Malyszek , Jacek Koput , Jonathan Tennyson , Sergei N. Yurchenko