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An electron diffraction study of nucleation and growth of the hcp phase in large pure Ar and mixed Ar-Kr clusters formed by supersonic jet expansion is carried out. The threshold cluster size corresponding to the appearance of an hcp phase…

Atomic and Molecular Clusters · Physics 2014-11-18 O. G. Danylchenko , S. I. Kovalenko , O. P. Konotop , V. N. Samovarov

An electron diffraction diagnostics of substrate-free clusters formed in N2-Kr binary jets expanding through a supersonic nozzle into vacuum was carried out. Gas mixtures contained 0.5, 1, and 6 mol.% krypton, the measured average sizes of…

Atomic and Molecular Clusters · Physics 2022-12-06 O. P. Konotop , O. G. Danylchenko

A quantitative phase analysis of substrate-free single-component and binary clusters of the Ar-Kr system obtained by adiabatic expansion of gas into vacuum through a supersonic nozzle was performed. The studies were carried out in-situ…

Atomic and Molecular Clusters · Physics 2026-01-06 O. G. Danylchenko , O. P. Konotop

We propose a new approach to analysis of cathodoluminescence spectra of substrate-free nanoclusters of argon produced in a supersonic jet expanding into a vacuum. It is employed to analyze intensities of the luminescence bands of neutral…

Atomic and Molecular Clusters · Physics 2016-01-28 Yu. S. Doronin , V. L. Vakula , G. V. Kamarchuk , A. A. Tkachenko , V. N. Samovarov

Size and composition of clusters produced by adiabatic expansion of binary gas mixtures (Ar-Kr, Kr-Xe, and N2-Ar) with various component concentrations are studied by using electron-diffraction technique. The resulting homogeneous and…

Atomic and Molecular Clusters · Physics 2014-10-06 O. P. Konotop , S. I. Kovalenko , O. G. Danylchenko , V. N. Samovarov

The master equation for the cluster-size distribution function is solved numerically to investigate the electron-hole droplet formation claimed to be discovered in the direct-gap CuCl excited by picosecond laser pulses [Nagai {\em et al.},…

Condensed Matter · Physics 2009-11-10 L. Jiang , M. W. Wu , M. Nagai , M. Kuwata-Gonokami

The article presents an original spectroscopic method for determining the initial stage of the clustering process in supersonic jets. The technique has been tested on a supersonic argon jet excited by electrons at a distance of 30…

Atomic and Molecular Clusters · Physics 2026-02-04 Yu. S. Doronin , A. A. Tkachenko , V. L. Vakula , G. V. Kamarchuk

We study the nucleation of crystalline cluster phases in the generalized exponential model with exponent n=4. Due to the finite value of this pair potential for zero separation, at high densities the system forms cluster crystals with…

Soft Condensed Matter · Physics 2016-09-01 Christian Leitold , Christoph Dellago

Previous x-ray diffraction studies have reported Eu to transform from the hcp structure to a new phase, Eu-III, at 18 GPa. Using x-ray powder diffraction we have determined that Eu remains hcp up to 33 GPa, and that the extra peaks that…

Materials Science · Physics 2013-01-16 R. J. Husband , I. Loa , G. W. Stinton , S. R. Evans , G. J. Ackland , M. I. McMahon

In this paper, electron diffraction and optical methods are used together for the first time to study the problem of phase equilibrium in binary clusters of heavy rare gases. For the argon-xenon system, a new effect of its decay into pure…

Atomic and Molecular Clusters · Physics 2007-05-23 O. G. Danylchenko , Yu. S. Doronin , S. I. Kovalenko , V. N. Samovarov

We study the distribution of hydrogen and various hydride configurations in realistic models of a-Si:H for two different concentration generated via experimentally constrained molecular relaxation approach (ECMR) [1]. The microstructure…

Materials Science · Physics 2015-05-14 Rajendra Timilsina , Parthapratim Biswas

We construct an electron optical system to investigate Bragg diffraction (the crystal lattice plane, $10^{-2}$-$10^{-3}$ rad) with the objective lens turned off by adjusting the current in the intermediate lenses. A crossover was located on…

Materials Science · Physics 2019-11-06 Hiroshi Nakajima , Atsuhiro Kotani , Ken Harada , Shigeo Mori

A new method for determining the condensate fraction and cluster density in absolute units has been proposed and tested for a supersonic argon jet, which can also be applied to supersonic jets of other gases. The method is based on…

Atomic and Molecular Clusters · Physics 2025-06-10 Yu. S. Doronin , A. A. Tkachenko , V. L. Vakula , G. V. Kamarchuk

Aberration-corrected scanning electron microscopy (AC-STEM) can provide valuable information on the atomic structure of nanoclusters, an essential input for gaining an understanding of their physical and chemical properties. A systematic…

Materials Science · Physics 2021-05-11 Kusse S. Bersha , Alejandro Peña-Torres , Hannes Jónsson

Energy spectra and angular distributions have been measured of electrons that are emitted upon disassembly of $Xe_{150000}$ following irradiation by intense (10$^{15}-10^{16}$ W cm$^{-2}$) laser pulses whose durations are varied over the…

Atomic and Molecular Clusters · Physics 2009-11-07 V. Kumarappan , M. Krishnamurthy , D. Mathur

A theoretical approach for the interpretation of reflectance spectra of opal photonic crystals with fcc structure and (111) surface orientation is presented. It is based on the calculation of photonic bands and density of states…

Other Condensed Matter · Physics 2009-11-11 E. Pavarini , L. C. Andreani , C. Soci , M. Galli , F. Marabelli , D. Comoretto

Atomic clusters presents an isolated system that models the bulk materials whose mechanism of HHG remains uncertain, and a promising medium to produce HHG beyond the limited conversion efficiency for gaseous atoms. Here we reveal that the…

Optics · Physics 2016-06-07 Na Li , Peng Liu , Ya Bai , Peng Peng , Ruxin Li , Zhizhan Xu

We report on an experimental study on the interaction of a high-contrast 40 fs duration 2.5 TW laser pulse with an argon cluster target. A high-charge, homogeneous, large divergence electron beam with moderate kinetic energy (~2 MeV) is…

Electronic transitions of jet-cooled FeC$_n$ clusters ($n = 3 - 6$) were measured between 230 and 300 nm by a mass-resolved 1+1 resonant two-photon ionization technique. Rotational profiles were simulated based on previous calculations of…

Chemical Physics · Physics 2015-02-19 Mathias Steglich , Xiaojing Chen , Anatoly Johnson , John P. Maier

A numerically cheap way to obtain structural information about clusters of rare gas atoms at low temperatures is developed. The semiclassical frozen Gaussian imaginary time propagator is extended such that it can account for the mean values…

Atomic and Molecular Clusters · Physics 2015-12-02 Holger Cartarius
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