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We study the properties of convex functionals which have been proposed for the simulation of charged molecular systems within the Poisson-Boltzmann approximation. We consider the extent to which the functionals reproduce the true…

Statistical Mechanics · Physics 2015-01-12 Justine S. Pujos , A. C. Maggs

We present a density functional scheme for calculating the pair density (PD) by means of the correlated wave function. This scheme is free from both of problems related to PD functional theory, i.e., (a) the need to constrain the…

Strongly Correlated Electrons · Physics 2015-06-25 Masahiko Higuchi , Katsuhiko Higuchi

We formulate a time-dependent density functional theory for the coupled dynamics of electrons and nuclei that goes beyond the Born-Oppenheimer (BO) approximation. We prove that the time-dependent marginal nuclear probability density…

Chemical Physics · Physics 2025-11-14 Chen Li , Ryan Requist , E. K. U. Gross

Extracting molecular properties from a wave function can be done through the linear response (LR) formalism or, equivalently, the equation of motion (EOM) formalism. For a simple model system, He in a 6-31G basis, it is here shown that…

The electron density $n(\rb,t)$, which is the central tool of time-dependent density functional theory, is presently considered to be derivable from a one-body time-dependent potential $V(\rb,t)$, via one-electron wave functions satisfying…

Quantum Physics · Physics 2009-04-28 Thomas A. Niehaus , Norman H. March

A random matrix theory approach is applied in order to analyze the localization properties of local spectral density for a generic system of coupled quantum states with strong static imperfection in the unperturbed energy levels. The system…

Quantum Physics · Physics 2009-11-07 V. S. Starovoitov

Long range frequency chirping of Bernstein-Greene-Kruskal modes, whose existence is determined by the fast particles, is investigated in cases where these particles do not move freely and their motion is bounded to restricted orbits. An…

Plasma Physics · Physics 2017-10-11 H. Hezaveh , Z. S. Qu , B. Layden , M. J. Hole

Brueckner-Hartree-Fock calculations are performed for nuclear matter with an exact treatment of the Pauli exclusion operator in the Bethe-Goldstone equation. The differences in the calculated binding energy, compared to the angle-average…

Nuclear Theory · Physics 2014-11-18 E. Schiller , H. Müther , P. Czerski

Correlator product states (CPS) are a class of tensor network wavefunctions applicable to strongly correlated problems in arbitrary dimensions. Here, we present a method for optimizing and evaluating the energy of the CPS wavefunction that…

Strongly Correlated Electrons · Physics 2015-04-13 Eric Neuscamman , Hitesh Changlani , Jesse Kinder , Garnet Kin-Lic Chan

The modified local spin density functional and the related local potential for excited states is tested by employing the ionization potential theorem. The functional is constructed by splitting $k$-space. Since its functional derivative…

Chemical Physics · Physics 2014-05-23 M. Hemanadhan , Md. Shamim , Manoj K. Harbola

Current-carrying and superconducting systems can be treated within density-functional theory if suitable additional density variables (the current density and the superconducting order parameter, respectively) are included in the…

Materials Science · Physics 2009-11-07 K. Capelle , G. Vignale

Faithful representations of atomic environments and general models for regression can be harnessed to learn electron densities that are close to the ground state. One of the applications of data-derived electron densities is to orbital-free…

Materials Science · Physics 2019-03-01 Andrew T. Fowler , Chris J. Pickard , James A. Elliott

Local density approximation (LDA) to the density functional theory (DFT) has continuous derivative of total energy as a number of electrons function and continuous exchange-correlation potential, while in exact DFT both should be…

Strongly Correlated Electrons · Physics 2010-06-28 V. I. Anisimov , A. V. Kozhevnikov , M. A. Korotin , A. V. Lukoyanov , D. A. Khafizullin

The symmetric nuclear matter and pure neutron matter are investigated by the relativistic Brueckner-Hartree-Fock (RBHF) theory with the covariant chiral nuclear forces up to the next-to-leading order~(NLO). A fitting scheme to ensure the…

Nuclear Theory · Physics 2025-06-24 Wei-Jiang Zou , Yi-Long Yang , Jun-Xu Lu , Peng-Wei Zhao , Li-Sheng Geng , Jie Meng

The one-body density matrix is derived within the Extended Thomas-Fermi approximation. This has been done starting from the Wigner-Kirkwood distribution function for a non-local single-particle potential. The links between this new approach…

Nuclear Theory · Physics 2009-10-31 V. B. Soubbotin , X. Vinas

In approximate Kohn-Sham density-functional theory, self-interaction manifests itself as the dependence of the energy of an orbital on its fractional occupation. This unphysical behavior translates into qualitative and quantitative errors…

Materials Science · Physics 2010-09-28 Ismaila Dabo , Andrea Ferretti , Nicolas Poilvert , Yanli Li , Nicola Marzari , Matteo Cococcioni

Based on a generalization of Hohenberg-Kohn's theorem, we propose a ground state theory for bosonic quantum systems. Since it involves the one-particle reduced density matrix $\gamma$ as a natural variable but still recovers quantum…

We explore a new class of computationally feasible approximations of the two-body density matrix as a finite sum of tensor products of single-particle operators. Physical symmetries then uniquely determine the two-body matrix in terms of…

Materials Science · Physics 2009-09-25 Gabor Csanyi , T. A. Arias

The Quark--Meson--Coupling (QMC) model self-consistently relates the dynamics of the internal quark structure of a hadron to the relativistic mean fields arising in nuclear matter. It offers a natural explanation to some open questions in…

In this brief note, the configurational density of states of a system of particles interacting via power-law pair potentials is computed exactly. The result is consistent with a constant microcanonical heat capacity. The well-known form of…

Statistical Mechanics · Physics 2025-08-04 Sergio Davis