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Producing large samples of slow molecules from thermal-velocity ensembles is a formidable challenge. Here we employ a centrifugal force to produce a continuous molecular beam with a high flux at near-zero velocities. We demonstrate…

Chemical Physics · Physics 2018-12-04 S. Chervenkov , X. Wu , J. Bayerl , A. Rohlfes , T. Gantner , M. Zeppenfeld , G. Rempe

A new type of decelerator is presented where polar neutral molecules are guided and decelerated using the principle of traveling electric potential wells, such that molecules are confined in stable three-dimensional traps throughout. This…

Atomic Physics · Physics 2010-05-24 Andreas Osterwalder , Samuel A. Meek , Georg Hammer , Henrik Haak , Gerard Meijer

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

Atomic Physics · Physics 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

We model sympathetic cooling of ground-state CaF molecules by ultracold Li and Rb atoms. The molecules are moving in a microwave trap, while the atoms are trapped magnetically. We calculate the differential elastic cross sections for CaF-Li…

Atomic Physics · Physics 2015-11-18 Jongseok Lim , Matthew D. Frye , Jeremy M. Hutson , M. R. Tarbutt

A recent progress on laser cooling of molecules is summarized. Since the development during 1980s for atomic species, laser cooling has been the very beginning step to cool and trap atoms for frontier research on quantum simulations,…

Atomic Physics · Physics 2023-03-29 Eunmi Chae

In the last years, it was demonstrated that neutral molecules can be loaded on a microchip directly from a supersonic beam. The molecules are confined in microscopic traps that can be moved smoothly over the surface of the chip. Once the…

Atomic Physics · Physics 2015-09-15 Gabriele Santambrogio

We demonstrate the mixing of rotational states in the ground electronic state using microwave radiation to enhance optical cycling in the molecule yttrium (II) monoxide (YO). This mixing technique is used in conjunction with a frequency…

Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…

Atomic Physics · Physics 2017-04-05 S. Truppe , H. J. Williams , N. J. Fitch , M. Hambach , T. E. Wall , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

Atomic Physics · Physics 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

When the scattering length is proportional to the distance from the center of the system, two particles are shown to be trapped about the center. Furthermore, their spectrum exhibits discrete scale invariance, whose scale factor is…

Quantum Gases · Physics 2015-03-20 Yusuke Nishida , Dean Lee

A quantum simulator based on ultracold optically trapped atoms for simulating the physics of atoms and molecules in ultrashort intense laser fields is introduced. The slowing down by about 13 orders of magnitude allows to watch in slow…

Atomic Physics · Physics 2017-02-01 Simon Sala , Johann Förster , Alejandro Saenz

We describe a method for cooling neutral molecules that have magnetic and electric dipole moments using collisions with cold ions. An external magnetic field is used to split the ground rovibrational energy levels of the molecule. The…

Atomic Physics · Physics 2014-08-22 F. Robicheaux

Sympathetic cooling with ultracold atoms and atomic ions enables ultralow temperatures in systems where direct laser or evaporative cooling is not possible. It has so far been limited to the cooling of other microscopic particles, with…

We calculate the microwave spectra of ultracold KRb alkali metal dimers, including hyperfine interactions and in the presence of electric and magnetic fields. We show that microwave transitions may be used to transfer molecules between…

Chemical Physics · Physics 2015-05-13 J. Aldegunde , Hong Ran , Jeremy M. Hutson

Stable ultracold ensembles of dipolar molecules hold great promise for many-body quantum physics, but high inelastic loss rates have been a long-standing challenge. Recently, it was shown that gases of fermionic molecules can be effectively…

We investigate the efficiency of cooling the vibrations of a nano-mechanical resonator, constituted by a partially suspended Carbon-nanotube and operating as double-quantum dot. The motion is brought to lower temperatures by tailoring the…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Stefano Zippilli , Adrian Bachtold , Giovanna Morigi

YbF has been identified as a molecule that can be used to investigate charge-parity symmetry violations that are beyond the Standard Model of particle physics. Cooling to sub-milli-Kelvin is advantageous for experiments that probe…

Chemical Physics · Physics 2022-12-14 Thomas D. Persinger , Jiande Han , Anh T. Le , Timothy C. Steimle , Michael C. Heaven

We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires vacuum-ultraviolet laser light, while multielectron atoms need laser…

Quantum Physics · Physics 2009-11-10 David Kielpinski

The last few years have seen rapid progress in the application of laser cooling to molecules. In this review, we examine what kinds of molecules can be laser cooled, how to design a suitable cooling scheme, and how the cooling can be…

Atomic Physics · Physics 2021-12-14 N. J. Fitch , M. R. Tarbutt

We study the properties of a cryogenic buffer gas source that uses a low temperature two-stage buffer gas cell to produce very slow beams of ytterbium monofluoride molecules. The molecules are produced by laser ablation inside the cell and…

Atomic Physics · Physics 2024-11-19 A. D. White , S. Popa , J. Mellado-Munoz , N. J. Fitch , B. E. Sauer , J. Lim , M. R. Tarbutt