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The pursuit of ever more precise measures of time and frequency is likely to lead to the eventual redefinition of the second in terms of an optical atomic transition. To ensure continuity with the current definition, based on a microwave…

We have measured the 1S - 2S transition frequency in atomic hydrogen via two photon spectroscopy on a 5.8 K atomic beam. We obtain $f_{1S-2S} = 2 466 061 413 187 035 (10)$ Hz for the hyperfine centroid. This is a fractional frequency…

We report a precise measurement of the hyperfine interval in the ${2P}_{1/2}$ state of $^{7}$Li. The transition from the ground state ($D_1$ line) is accessed using a diode laser and the technique of saturated-absorption spectroscopy in hot…

Atomic Physics · Physics 2015-05-19 Alok K. Singh , Lal Muanzuala , Vasant Natarajan

We report a direct measurement of the 0-1 R(0) vibrational transition frequency in ground-state hydrogen deuteride (HD) using infrared-ultraviolet double resonance spectroscopy in a molecular beam. Ground-state molecules are vibrationally…

Atomic Physics · Physics 2020-07-14 Arthur Fast , Samuel A. Meek

We report the first absolute frequency measurements for the $5s5p^{3}$P$_{0}\to5s6d^{3}$D$_{1}$ transition at 394 nm for all the stable strontium isotopes by utilizing repumping induced spectroscopy in a magneto-optical trap. Absolute…

Atomic Physics · Physics 2024-11-25 S. Zhang , B. T. Tiwari , S. Ganesh , Y. Singh , V. V. Flambaum

In 2003 we have measured the absolute frequency of the $(1S, F=1, m_F=\pm 1) \leftrightarrow (2S, F'=1, m_F'=\pm 1)$ two-photon transition in atomic hydrogen. We observed a variation of $(-29\pm 57)$ Hz over a 44 months interval separating…

Precision determination of the hyperfine splitting of cadmium ions is essential to study space-time variation of fundamental physical constants and isotope shifts. In this work, we present the precision frequency measurement of the…

Atomic Physics · Physics 2025-01-24 Ying Zheng , Yanmei Yu , Yiting Chen , Shengnan Miao , Wenxin Shi , Jianwei Zhang , Lijun Wang

High-precision quasi-simultaneous collinear/anticollinear laser spectroscopy was performed to measure the $5s$ $^2S_{1/2}\rightarrow 5p$ $^2P_{1/2}$ (D1), the $5s$ $^2S_{1/2}\rightarrow 5p$ $^2P_{3/2}$ (D2), and the three $4d\rightarrow 5p$…

We report on the absolute frequency determination of the 5s5p $^1P_1$ - 5s5d $^1D_2$ transition in atomic strontium, achieved through frequency comb-referenced laser-induced-fluorescence (LIF) spectroscopy. We excite the 5s$^2$ $^1S_0$ -…

Atomic Physics · Physics 2024-03-28 Ana Cipriš , Ivana Puljić , Damir Aumiler , Ticijana Ban , Neven Šantić

We report the direct frequency measurement of the visible 5s$^2$ $^1$S$_0$-5s 5p$^3$P$_1$ intercombination line of strontium that is considered a possible candidate for a future optical frequency standard. The frequency of a…

Atomic Physics · Physics 2007-05-23 G. Ferrari , P. Cancio , R. Drullinger , G. Giusfredi , N. Poli , M. Prevedelli , C. Toninelli , G. M. Tino

A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…

Atomic Physics · Physics 2009-11-11 Adela Marian , Matthew C. Stowe , Daniel Felinto , Jun Ye

The hyperfine structure and isotope shifts of the 3s23p2 3P2 to 3s3p3 3Do3 transition in silicon have been measured. The transition at 221.7 nm was studied by laser induced fluorescence in an atomic Si beam. For 29Si, the hyperfine A…

Atomic Physics · Physics 2015-05-20 Siu Au Lee , William Fairbank

The frequency comb created by a femtosecond mode-locked laser and a microstructured fiber is used to phase coherently measure the frequencies of both the Hg^+ and Ca optical standards with respect to the SI second as realized at NIST. We…

We developed a novel technique for frequency measurement and synthesis, based on the operation of a femtosecond comb generator as transfer oscillator. The technique can be used to measure frequency ratios of any optical signals throughout…

Optics · Physics 2009-11-07 Jörn Stenger , Harald Schnatz , Christian Tamm , Harald R. Telle

The absolute frequency measurement for all of the hyperfine transitions of 6P1/2 -> 7S1/2 using a self-referencing frequency comb is reported. This transition can be used as a bench marker for the accurate atomic wave function, and then…

Atomic Physics · Physics 2013-03-22 Tzu-Ling Chen , Isaac Fan , Chang-Yi Lin , Hsuan-Chen Chen , Shih-En Chen , Jow-Tsong Shy , Yi-Wei Liu

We have carried absolute frequency measurements of the $(6s^{2})\,^{1}S_{0}$ $-$ $(6s6p)\,^{3}P_{1}$ transition in $^{171}$Yb (the intercombination line), where the spin-1/2 isotope yields two hyperfine lines. The measurements rely on…

Atomic Physics · Physics 2023-05-23 Daniel M. Jones , Frank van Kann , John J. McFerran

We present a method to precisly measure the frequencies of transitions to high-$n$ Rydberg states of the hydrogen atom which are not subject to uncontrolled systematic shifts caused by stray electric fields. The method consists in recording…

Atomic Physics · Physics 2024-01-09 Simon Scheidegger , Josef A. Agner , Hansjürg Schmutz , Frédéric Merkt

High-resolution spectroscopy on the $A^2\Pi$ - $X^2\Sigma^+$ electronic system of $^{138}$Ba$^{19}$F is performed using a cold molecular beam produced by a buffer gas source. The hyperfine structure in both $X^2\Sigma^+$ ground and $A^2\Pi$…

We present a measurement of the hydrogen $2$S$_{1/2}-8$D$_{5/2}$ transition performed with a cryogenic atomic beam. The measured resonance frequency is $\nu=770649561570.9(2.0)$ kHz, which corresponds to a relative uncertainty of…

Atomic Physics · Physics 2022-01-26 A. D. Brandt , S. F. Cooper , C. Rasor , Z. Burkley , D. C. Yost , A. Matveev

An efficient $\lambda/2$-method ($\lambda$ is the resonant wavelength of laser radiation) based on nanometric-thickness cell filled with rubidium is implemented to study the splitting of hyperfine transitions of $^{85}$Rb and $^{87}$Rb…

Atomic Physics · Physics 2015-06-19 A. Sargsyan , A. Tonoyan , G. Hakhumyan , C. Leroy , Y. Pashayan-Leroy , D. Sarkisyan