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Ultrashort long-wave infrared (LWIR) laser pulses can resonantly excite vibrations in N2 and O2 through a two-photon transition. The absorptive, vibrational component of the ultrafast optical nonlinearity grows in time, starting smaller…
The interaction of intense, ultra-short laser pulses with nanostructures offers promising avenues for spatiotemporal light control. While enhanced optical transmission through subwavelength apertures has been extensively studied in the…
Saturable absorption is a nonlinear effect where a material's ability to absorb light is frustrated due to a high influx of photons and the creation of electron vacancies. Experimentally induced saturable absorption in copper revealed a…
High peak power ultrafast lasers are widely used in nonlinear spectroscopy but often limit its spectral resolution because of the broad frequency bandwidth of ultrashort laser pulses. Improving the resolution by achieving spectrally narrow…
The numerical simulations of an ultrashort pulse propagation in a one-dimensional nonlinear photonic crystal are carried out. It is known that the relaxation of cubic nonlinearity is the reason for the effect of pulse self-trapping in such…
Nonlinear amplification is a powerful technique for generating ultrashort laser pulses with high peak power in fiber systems. However, the diversity of nonlinear amplification approaches and their inherent complexities present significant…
We exploit the effect of light-induced atomic desorption to produce high atomic densities ($n\gg k^3$) in a rubidium vapor cell. An intense off-resonant laser is pulsed for roughly one nanosecond on a micrometer-sized sapphire-coated cell,…
We show that the modulation of the phases of the laser beams of ultra-short pulses leads to modulation of the two photon fluorescence intensity. The phase modulation technique when used in multi-photon microscopy can improve the signal to…
Multi-photon microscopy has played a significant role in biological imaging since it allows to observe living tissues with improved penetration depth and excellent sectioning effect. Multi-photon microscopy relies on multi-photon…
We experimentally investigate fluctuations in the spectrum of ultrashort laser pulses propagating in air, close to the critical power for filamentation. Increasing the laser peak power broadens the spectrum while the beam approaches the…
Propagation of ultrarelativistically intense laser pulse in a self-trapping mode in a near critical density plasma makes it possible to produce electron bunches of extreme parameters appropriate for different state of art applications.…
Ultrashort (femtosecond, fs) laser pulses have fascinating properties as they allow to confine optical energy on extreme scales in space and time. Such fs-laser pulsed beams can be seen as spatially thin slices of intense light that are…
It is known that rare-gas or metal clusters absorb incident laser energy very efficiently. However, due to the intricate dependencies on all the laser and cluster parameters it is difficult to predict under which circumstances ionization…
Through resonant backward Raman scattering, the plasma wave mediates the energy transfer between long pump and short seed laser pulses. These mediation can result in pulse compression at extraordinarily high powers. However, both the…
The ability to manipulate the spectral-temporal waveform of optical pulses has enabled a wide range of applications from ultrafast spectroscopy to high-speed communications. Extending these concepts to quantum light has the potential to…
We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS's photon absorption spectrum. Tuning and controlling the emission and the absorption is of much interest e.g.\ for the…
We derive upper and lower bounds on the absorption of ultraintense laser light by solids as a function of fundamental laser and plasma parameters. These limits emerge naturally from constrained optimization techniques applied to a…
Propagation of a weak probe pulse through a $\Lambda$ system in a resonant gain configuration is investigated. We employ the control field intensity that permits the amplification of probe pulse during propagation, without instability at…
We report on the response of graphene to high intensity mid-IR radiation and show that graphene exhibits saturable absorption and significant two-photon absorption in the spectral region from 1.55 $\mu$m to 3.50 $\mu$m (0.35 eV to 0.80 eV).…
The ability to control the spatial distribution of light, particularly in deep sub-wavelength areas, is important for a range of materials science, microscopy, and communications applications. Separately, materials science and…