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We measure the statistical polarization of quadrupolar nuclear spins in a sub-micrometer (0.6 um^3) particle of GaAs using magnetic resonance force microscopy. The crystalline sample is cut out of a GaAs wafer and attached to a…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 Fei Xue , D. P. Weber , P. Peddibhotla , M. Poggio

We applied the recently developed technique of force-detected nuclear magnetic resonance (NMR) to observe 71Ga, 69Ga, and 75As in GaAs. The nuclear spin-lattice relaxation time is 21$\pm$5 min for 69Ga at $\sim 5$ K and 4.6 Tesla. We have…

Materials Science · Physics 2009-11-07 Kent R. Thurber , Lee E. Harrell , Raul Fainchtein , Doran D. Smith

Magnetic resonance imaging, based on the manipulation and detection of nuclear spins, is a powerful imaging technique that typically operates on the scale of millimeters to microns. Using magnetic resonance force microscopy, we have…

Other Condensed Matter · Physics 2007-06-27 H. J. Mamin , M. Poggio , C. L. Degen , D. Rugar

We exploit ferromagnetic imprinting to create complex laterally defined regions of nuclear spin polarization in lithographically patterned MnAs/GaAs epilayers grown by molecular beam epitaxy (MBE). A time-resolved Kerr rotation microscope…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 J. Stephens , R. K. Kawakami , J. Berezovsky , M. Hanson , D. P. Shepherd , A. C. Gossard , D. D. Awschalom

We review recent efforts to detect small numbers of nuclear spins using magnetic resonance force microscopy. Magnetic resonance force microscopy (MRFM) is a scanning probe technique that relies on the mechanical measurement of the weak…

Mesoscale and Nanoscale Physics · Physics 2010-08-03 M. Poggio , C. L. Degen

The photoluminescence polarizations of (In,Ga)As/GaAs quantum dots annealed at different temperatures are studied as a function of external magnetic field (Hanle curves). In these dependencies, remarkable resonant features appear due to…

We use a 1.0-um-wide patterned Cu wire with an integrated nanomagnetic tip to measure the statistical nuclear polarization of 19F in CaF2 by magnetic resonance force microscopy (MRFM). With less than 350 uW of dissipated power, we achieve…

Other Condensed Matter · Physics 2007-06-27 M. Poggio , C. L. Degen , C. T. Rettner , H. J. Mamin , D. Rugar

When probing nuclear spins in materials on the nanometer scale, random fluctuations of the spin polarization will exceed the mean Boltzmann polarization for sample volumes below about (100nm)^3. In this work, we use magnetic resonance force…

Mesoscale and Nanoscale Physics · Physics 2008-01-14 C. L. Degen , M. Poggio , H. J. Mamin , D. Rugar

A method for high-field optically detected nuclear magnetic resonance (ODNMR) is developed sensitive to 10**8 nuclei. Nuclear spin transitions are induced using a radio frequency coil and detected through Faraday rotation spectroscopy.…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Poggio , D. D. Awschalom

Understanding and manipulating spin polarization and transport in the vicinity of semiconductor-hosted defects is a problem of present technological and fundamental importance. Here, we use high-field magnetic resonance to monitor the…

Mesoscale and Nanoscale Physics · Physics 2014-01-14 Yunpu Li , Jonathan P. King , Jeffrey A. Reimer , Carlos A. Meriles

Magnetic Resonance Force Microscopy (MRFM) enables three-dimensional imaging of nuclear spin densities in nanoscale objects. Based on numerical simulations, we evaluate the performance of strained SiN resonators as force sensors and show…

Applied Physics · Physics 2026-04-15 Nils Prumbaum , Christian L. Degen , Alexander Eichler

Magnetic noise of atomic nuclear spins is a major problem for solid state spin qubits. Highly-polarized nuclei would not only overcome this obstacle, but also make nuclear spins a useful quantum information resource. However, achieving…

A room temperature nuclear magnetic resonance force microscope (MRFM), fitted in a $^1$Tesla electromagnet, is used to measure the nuclear spin relaxation of $^1$H in a micron-size (70ng) crystal of ammonium sulfate. NMR sequences,…

Condensed Matter · Physics 2009-10-31 O. Klein , V. V. Naletov , H. Alloul

We study light-induced nuclear spin-polarization in a thin film of Ga1-xMnxAs (x 0.04), a dilute ferromagnetic semiconductor, grown on a GaAs substrate. High-field inductively-detected Ga-71 NMR was performed with samples immersed in…

Magnetic spin resonance is a key non-invasive sensing and imaging technique across the life-, material- and fundamental sciences with further medical and commercial applications. Recent advances using paramagnetic color centers enable…

Mesoscale and Nanoscale Physics · Physics 2018-07-24 Florestan Ziem , Marwa Garsi , Helmut Fedder , Jörg Wrachtrup

We investigate the dynamic nuclear polarization from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins coupled to them in semiconductor nanostructures. We derive the time and position dependence of the…

Materials Science · Physics 2007-05-23 Ionel Tifrea , Michael E. Flatte

We demonstrate a scheme for optically patterning nuclear spin polarization in semiconductor/ferromagnet heterostructures. A scanning time-resolved Kerr rotation microscope is used to image the nuclear spin polarization that results when…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 J. Stephens , J. Berezovsky , R. K. Kawakami , A. C. Gossard , D. D. Awschalom

Mechanical resonators operating in the megahertz range have become a versatile platform for fundamental and applied quantum research. Their exceptional properties, such as low mass and high quality factor, make them also appealing for force…

Mesoscale and Nanoscale Physics · Physics 2026-04-20 Diego A. Visani , Letizia Catalini , Christian L. Degen , Alexander Eichler , Javier del Pino

We report the use of an atomic magnetometer based on nonlinear magneto-optical rotation with frequency modulated light (FM NMOR) to detect nuclear magnetization of xenon gas. The magnetization of a spin-exchange-polarized xenon sample ($1.7…

Nuclear spin polarization dynamics are measured in optically pumped individual GaAs/AlGaAs interface quantum dots by detecting the time-dependence of the Overhauser shift in photoluminescence (PL) spectra. Long nuclear polarization decay…

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