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We exploit spin noise spectroscopy (SNS) to directly observe build-up of dynamic nuclear polarization and relaxation of a perturbed nuclear spin-system to its equilibrium state in a single-shot experiment. The SNS experiments were performed…

We report the observation of nuclear magnetic resonance (NMR) in a ferromagnet-semiconductor heterostructure in the presence of a spin-polarized current. Spin-polarized electrons injected from a metallic ferromagnet generate a large nuclear…

Condensed Matter · Physics 2009-11-10 J. Strand , B. D. Schultz , A. F. Isakovic , X. Lou , C. J. Palmstrom , P. A. Crowell

We attract attention to the fact that the ultimate (shot-noise-limited) polarimetric sensitivity can be enhanced by orders of magnitude leaving the photon flux incident onto the photodetector on the same low level. This opportunity is of…

Mesoscale and Nanoscale Physics · Physics 2014-03-14 P. Glasenapp , A. Greilich , I. I. Ryzhov , V. S. Zapasskii , D. R. Yakovlev , G. G. Kozlov , M. Bayer

We present a new method for high-resolution nanoscale magnetic resonance imaging (nano-MRI) that combines the high spin sensitivity of nanowire-based magnetic resonance detection with high spectral resolution nuclear magnetic resonance…

Mesoscale and Nanoscale Physics · Physics 2018-03-07 William Rose , Holger Haas , Angela Q. Chen , Nari Jeon , Lincoln J. Lauhon , David G. Cory , Raffi Budakian

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

We report a method for nanometer-scale pulsed nuclear magnetic resonance imaging and spectroscopy. Periodic radiofrequency pulses are used to create temporal correlations in the statistical polarization of a solid organic sample. The spin…

Mesoscale and Nanoscale Physics · Physics 2013-10-01 John M. Nichol , Tyler R. Naibert , Eric R. Hemesath , Lincoln J. Lauhon , Raffi Budakian

We report achieving enhanced nuclear magnetization in a magnetic resonance force microscope experiment at 0.6 tesla and 4.2 kelvin using the dynamic nuclear polarization (DNP) effect. In our experiments a microwire coplanar waveguide…

Interest in the magnetism of organic compounds is growing because of new organic magnets, spin-based electronics and the diverse properties of magnetic edge states in graphene nanoribbons. Electron spin resonance spectroscopy combined with…

Mesoscale and Nanoscale Physics · Physics 2025-04-28 Gregory Czap , Christoph Wolf , Jose Reina-Gálvez , Mark H. Sherwood , Christopher P. Lutz

We implement magnetic resonance force microscopy (MRFM) in an experimental geometry, where the long axis of the cantilever is normal to both the external magnetic field and the RF microwire source. Measurements are made of the statistical…

Mesoscale and Nanoscale Physics · Physics 2015-03-19 Fei Xue , P. Peddibhotla , M. Montinaro , D. Weber , M. Poggio

Soon after the first measurements of nuclear magnetic resonance (NMR) in a condensed matter system, Bloch predicted the presence of statistical fluctuations proportional to $1/\sqrt{N}$ in the polarization of an ensemble of $N$ spins. First…

Mesoscale and Nanoscale Physics · Physics 2013-10-07 P. Peddibhotla , F. Xue , H. I. T. Hauge , S. Assali , E. P. A. M. Bakkers , M. Poggio

Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 Sahand Tabatabaei , Pritam Priyadarsi , Namanish Singh , Pardis Sahafi , Daniel Tay , Andrew Jordan , Raffi Budakian

Recently reported optical nuclear orientation in the $n$-doped GaAs microcavity under pumping in nominal transparency region of the crystal [Appl. Phys. Lett. $\mathbf{106}$, 242405 (2015)] has arisen a number of questions, the main of them…

Deep cooling of electron and nuclear spins is equivalent to achieving polarization degrees close to 100% and is a key requirement in solid state quantum information technologies. While polarization of individual nuclear spins in diamond and…

Mesoscale and Nanoscale Physics · Physics 2017-10-11 E. A. Chekhovich , A. Ulhaq , E. Zallo , F. Ding , O. G. Schmidt , M. S. Skolnick

Magnetic resonance force microscopy (MRFM) is a scanning probe technique capable of detecting MRI signals from nanoscale sample volumes, providing a paradigm-changing potential for structural biology and medical research. Thus far, however,…

The study of nuclear magnetic resonance and nuclear spin-lattice relaxation was conducted in an asymmetrically doped to $n\sim1.8\times10^{11}$ cm$^{-2}$ 16 nm AlAs quantum well grown in the $[001]$-direction. Dynamic polarization of…

Mesoscale and Nanoscale Physics · Physics 2016-12-22 A. V. Shchepetilnikov , D. D. Frolov , Yu. A. Nefyodov , I. V. Kukushkin , D. S. Smirnov , L. Tiemann , C. Reichl , W. Dietsche , W. Wegscheider

We report on Magnetic Resonance Force Microscopy measurements of the Boltzmann polarization of the nuclear spins in copper by detecting the frequency shift of a soft cantilever. We use the time-dependent solution of the Bloch equations to…

Mesoscale and Nanoscale Physics · Physics 2019-07-23 Martin de Wit , Gesa Welker , Jelmer Wagenaar , Freek Hoekstra , Tjerk Oosterkamp

The nuclear spin fluctuations (NSF) as well as the dynamic nuclear polarization (DNP) and their effects on the electron spins in negatively charged (In,Ga)As/GaAs quantum dots have been studied by polarized pump-probe and photoluminescence…

We report a method for accelerated nanoscale nuclear magnetic resonance imaging by detecting several signals in parallel. Our technique relies on phase multiplexing, where the signals from different nuclear spin ensembles are encoded in the…

Mesoscale and Nanoscale Physics · Physics 2015-08-11 B. A. Moores , A. Eichler , Y. Tao , H. Takahashi , P. Navaretti , C. L. Degen

We demonstrate an interface-sensitive NMR in a semiconducting nanostructure, where an NMR signal from the minute heterojunction region of a model heterojunction structure (In$_{0.48}$Ga$_{0.52}$P/GaAs) is detected by using nuclear…

Mesoscale and Nanoscale Physics · Physics 2017-12-13 Atsushi Goto , Kenjiro Hashi , Shinobu Ohki , Tadashi Shimizu

Heat capacity of the nuclear spin system (NSS) in GaAs-based microstructures has been shown to be much greater than expected from dipolar coupling between nuclei, thus limiting the efficiency of NSS cooling by adiabatic demagnetization. It…

Mesoscale and Nanoscale Physics · Physics 2024-03-26 M. Vladimirova , S. Cronenberger , A. Colombier , D. Scalbert , V. M. Litvyak , K. V. Kavokin , A. Lemaître