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We present maps of the 6 cm and 1.3 mm transitions of formaldehyde toward three cold, dense pre-protostellar cores: L1498, L1512, and L1544. The 6 cm transition is a unique probe of high density gas at low temperature. However, our models…

Astrophysics · Physics 2009-11-10 Kaisa E. Young , Jeong-Eun Lee , Neal J. Evans , Paul F. Goldsmith , Steven D. Doty

Simultaneous two-dimensional trapping of neutral dipolar molecules in low- and high-field seeking states is analyzed. A trapping potential of the order of 20 mK can be produced for molecules like ND3 with time-dependent electric fields. The…

Chemical Physics · Physics 2009-11-10 T. Junglen , T. Rieger , S. A. Rangwala , P. W. H. Pinkse , G. Rempe

Reaching high densities is a key step towards cold-collision experiments with polyatomic molecules. We use a cryofuge to load up to 2$\times10^7$ CH$_3$F molecules into a box-like electric trap, achieving densities up to 10$^7$/cm$^3$ at…

Atomic Physics · Physics 2022-05-18 M. Koller , F. Jung , J. Phrompao , M. Zeppenfeld , I. M. Rabey , G. Rempe

Formaldehyde (H2CO) is often observed at centimeter wavelengths as an absorption line against the cosmic microwave background (CMB). This is possible when energy level populations are cooled to the point where line excitation temperatures…

Astrophysics of Galaxies · Physics 2019-04-02 Jeremy Darling

We conducted series of experiments on observing a Stark-type effect in superfluid $^4$He in presence of relative laminar flows of the normal and superfluid components. It is designed a measurement cell which allows us to simultaneously…

We report a compact (<20cm3), robust source for producing a bright flux of cold atoms, which can be loaded efficiently into a magnetic guide. A continuous flux of up to 8 x 109 87Rb atoms/s have been produced from this 2D+ vapor cell MOT.…

Atomic Physics · Physics 2015-06-26 R. S. Conroy , Y. Xiao , M. Vengalattore , W. Rooijakkers , M. Prentiss

We present an \textit{ab initio} auxiliary field quantum Monte Carlo method for studying the electronic structure of molecules, solids, and model Hamiltonians at finite temperature. The algorithm marries the \textit{ab initio} phaseless…

Strongly Correlated Electrons · Physics 2018-11-13 Yuan Liu , Minsik Cho , Brenda Rubenstein

Helium nanodroplets doped with polar molecules are studied by electrostatic deflection. This broadly applicable method allows even polyatomic molecules to attain sub-Kelvin temperatures and nearly full orientation in the field. The…

Atomic and Molecular Clusters · Physics 2019-07-26 John W. Niman , Benjamin S. Kamerin , Daniel J. Merthe , Lorenz Kranabetter , Vitaly V. Kresin

We demonstrate experimentally the guiding of cold and slow ND3 molecules along a thin charged wire over a distance of ~0.34 m through an entire molecular beam apparatus. Trajectory simulations confirm that both linear and quadratic…

Atomic and Molecular Clusters · Physics 2011-12-19 M. Strebel , S. Spieler , F. Stienkemeier , M. Mudrich

Ro-vibrational Stark-associated phenomena of small polyatomic molecules are modelled using extensive spectroscopic data generated as part of the ExoMol project. The external field Hamiltonian is built from the computed ro-vibrational line…

The strengths and short-comings of the point-dipole model for polar fluids of spherical molecules are illustrated by considering the physically more relevant case of extended dipoles formed by two opposite charges $\pm q$ separated by a…

Statistical Mechanics · Physics 2009-11-10 V. Ballenegger , J. P. Hansen

Electrostatic velocity filtering is a technique for the production of continuous guided beams of slow polar molecules from a thermal gas. We extended this technique to produce pulses of slow molecules with a narrow velocity distribution…

We propose an array of ultracold polar molecules as a platform to study alignment transport between molecules. We envision a polar molecule being aligned with an intense off-resonant laser field whose alignment migrates to a nearby molecule…

Chemical Physics · Physics 2024-02-27 Jonathan Smucker , Jesus Pérez-Ríos

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

Atomic Physics · Physics 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal…

Carbon monoxide molecules in their electronic, vibrational, and rotational ground state are highly attractive for trapping experiments. The optical or ac electric traps that can be envisioned for these molecules will be very shallow,…

Continuously operating atom-light interfaces represent a key prerequisite for steady-state quantum sensors and efficient quantum processors. Here, we demonstrate continuous accumulation of sub-Doppler-cooled atoms in a shallow intracavity…

Quantum Physics · Physics 2025-12-17 Edward Gheorghita , Sebastian Wald , Andrea Pupić , Onur Hosten

We propose a simple and reliable method to study the translational relaxation of 'hot' H atoms following their production by chemical mechanisms. The problem is relevant to PDR's, shocks, photospheres, atmospheric entry problems. We show…

Plasma Physics · Physics 2015-05-30 A. Panarese , S. Longo

We present precision spectroscopy on electrically trapped formaldehyde (H$_2$CO), demonstrating key attributes which will enable molecular spectroscopy with unprecedented precision. Our method makes use of a microstructured electric trap…

Atomic Physics · Physics 2018-07-19 Alexander Prehn , Martin Ibrügger , Gerhard Rempe , Martin Zeppenfeld

The ground-state properties of two-dimensional liquid $^4$He at zero temperature are studied by means of a quadratic diffusion Monte Carlo method. As interatomic potential we use a revised version of the HFDHE2 Aziz potential which is…

Condensed Matter · Physics 2009-10-28 S. Giorgini , J. Boronat , J. Casulleras