Related papers: Charge-Induced Fragmentation of Sodium Clusters
Computer simulations yield evidence of superfluid behavior of nanoscale size clusters of parahydrogen adsorbed on a graphite substrate at low temperature ($T\lesssim 0.25 \text{ K}$). Clusters with a number of molecules between 7 and 12…
In the first part of thesis, we shall deal with fragment emission in central collisions studied as a function of beam energy and system mass. Central collisions are also important candidate in view of exploring collective expansion and…
Coherent grazing-incidence small-angle X-ray scattering is used to investigate the average kinetics and the fluctuation dynamics during self-organized nanopatterning of silicon by Ar$^+$ bombardment at 65$^{\circ}$ polar angle. At early…
We propose a method for quantifying charge-driven instabilities in clusters, based on equilibrium simulations under confinement at constant external pressure. This approach makes no assumptions about the mode of decay and allows different…
We report a systematic study of the $c$ lattice parameter in the Na$_{x}$CoO$_{2}$ phases versus Na content $x>0.5$, in which sodium always displays ordered arrangements. This allows us to single out the first phase which exhibits an AF…
Large density fluctuations of charged particles are the promising signatures for exploring the QCD phase transition and critical point in heavy ion collisions. These fluctuations are expected to exhibit fractal and scale invariant…
This paper provides new insights concerning the simulation of plasmon driven chemical reactions using real-time TDDFT based on the tight-binding electronic structure code DFTB+, with applications to the dissociation of H$_2$ on octahedral…
While largely studied on the macroscopic scale, the dynamics leading to nucleation and fission processes in atmospheric aerosols are still poorly understood at the molecular level. Here, we present a joint experimental-theoretical study of…
The fragmentation of quasi-projectiles from the nuclear reaction 40Ca + 12C at 25 MeV/nucleon was used to produce alpha-emission sources. From a careful selection of these sources provided by a complete detection and from comparisons with…
Density--functional simulations have been performed on Na$_{55}$, Na$_{92}$ and Na$_{142}$ clusters in order to understand the experimentally observed melting properties [M. Schmidt \textit{et al.}, Nature (London) \textbf{393}, 238…
The decay of $^{56}Ni^*$, formed in $^{32}S+^{24}Mg$ reaction at the incident energies $E_{cm}$=51.6 and 60.5 MeV, is calculated as a cluster decay process within the Preformed Cluster-decay Model (PCM) of Gupta et al. re-formulated for hot…
The generation of highly charged Xe$^{q+}$ ions up to {$q=24$} is observed in Xe clusters embedded in helium nanodroplets and exposed to intense femtosecond laser pulses ($\lambda$=800 nm). Laser intensity resolved measurements show that…
Massive clumps tend to fragment into clusters of cores and condensations, some of which form high-mass stars. In this work, we study the structure of massive clumps at different scales, analyze the fragmentation process, and investigate the…
We investigate the impact of dissipation on the energy balance in the electron dynamics of metal clusters excited by strong electro-magnetic pulses. The dynamics is described theoretically by Time-Dependent Density-Functional Theory (TDDFT)…
The inclusive energy distributions of complex fragments (3 $\leq$Z $\leq$ 9) emitted in the reactions $^{20}$Ne (145, 158, 200, 218 MeV) + $^{27}$Al have been measured in the angular range 10$^{o}$ - 50$^{o}$. The fusion-fission and the…
The melting-like transition in sodium clusters Na_N, with N=55, 92, and 142 is studied by using constant-energy molecular dynamics simulations. An orbital-free version of the Car-Parrinello technique is used which scales linearly with…
We present energy- and charge-resolved measurements of low and hyperthermal energy Na+ ions scattered from a Ag(001) surface. With the primary ion beam oriented along the [110] crystal direction, distinct peaks in the energy distributions…
The nucleation and structure of silicon nanocrystals formed by different preparation conditions and silicon concentration (28 - 70 area %) have been studied using Transmission Electron Microscopy (TEM), Energy Filtered TEM (EFTEM) and…
Context. The abundance inhomogeneities of light elements observed in Globular Clusters (GCs), and notably the ubiquitous Na-O anti-correlation, are generally interpreted as evidence that GCs comprise several generations of stars. There is…
We investigate the size distribution of electrically charged nanodroplets. The droplets were generated using nano- and micro- scale silicon tips. A brief voltage pulse results in a "snapshot" of charged nanodroplets on a metal surface.…